Bragg Reflection Waveguide: Anti-Mirror Reflection and Light Slowdown

The effect of the light group velocity reduction in dielectric Bragg reflection waveguide structures (SiO$_2$/TiO$_2$) in the vicinity of the cutoff frequency is studied experimentally. The effect of anti-mirror reflection, specific for the Bragg reflection waveguides, is described and employed for detection of "slow light". The experiments were performed with the use of the Ti:sapphire laser pulses ~ 100 fs in length. The group index $n_g \sim$ 30 with a fractional pulse delay (normalized to the pulse width) of $\sim$ 10 is demonstrated. The problems and prospects of implementation of the slow-light devices based on the Bragg reflection waveguide structures are discussed.Comment: 11 pages, in the previous version, we failed to insert figure

Spin noise of a halide perovskite

We report on first observation of spin noise in a strongly birefringent semiconductor -- halide perovskite single crystal MAPbI$_3$. The observed spin noise resonance is ascribed to free holes with a record spin dephasing time of 4 ns. The spin dynamics is found to be affected by the residual light absorption of the crystal providing renormalization of the Larmor frequency. Extended spin noise spectroscopy with rotating magnetic field allowed us not only to evaluate the $g$-factor anisotropy, but also to distinguish two different spin subsystems tentatively associated to twinning of the crystal.Comment: 14 pages, 11 figure

Photon echoes from (In,Ga)As quantum dots embedded in a Tamm-plasmon microcavity

We acknowledge the financial support by the Deutsche Forschungsgemeinschaft through the Collaborative Research Centre TRR 142 and the International Collaborative Research Centre 160. S.V.P. and Yu.V.K. thank the Russian Foundation of Basic Research for partial financial support (contracts no. ofi_m 16-29-03115 and no. 15-52-12016NNIO_a). M.B. acknowledges partial financial support from the Russian Ministry of Science and Education (contract no. 14.Z50.31.0021). Yu.V.K. acknowledges Saint Petersburg State University for a research grant 11.42.993.2016. The project SPANGL4Q acknowledges financial support from the Future and Emerging Technologies (FET) programme within the Seventh Framework Programme for Research of the European Commission, under FET-Open grant no. FP7-284743.We report on the coherent optical response from an ensemble of (In,Ga)As quantum dots (QDs) embedded in a planar Tamm-plasmon microcavity with a quality factor of approx. 100. Significant enhancement of the light-matter interaction is demonstrated under selective laser excitation of those quantum dots which are in resonance with the cavity mode. The enhancement is manifested through Rabi oscillations of the photon echo, demonstrating coherent control of excitons with picosecond pulses at intensity levels more than an order of magnitude smaller as compared with bare quantum dots. The decay of the photon echo transients is weakly changed by the resonator indicating a small decrease of the coherence time T2 which we attribute to the interaction with the electron plasma in the metal layer located close (40 nm) to the QD layer. Simultaneously we see a reduction of the population lifetime T1, inferred from the stimulated photon echo, due to an enhancement of the spontaneous emission by a factor of 2, which is attributed to the Purcell effect, while non-radiative processes are negligible as confirmed from time-resolved photoluminescence.PostprintPeer reviewe

Photon echo transients from an inhomogeneous ensemble of semiconductor quantum dots

We acknowledge the financial support by the Deutsche Forschungsgemeinschaft, Project ICRC TRR 160 and the Russian Foundation of Basic Research (RFBR) in the frame of the Project No. 15-52-12016 NNIO_a. The project SPANGL4Q acknowledges financial support from the Future and Emerging Technologies (FET) programme within the Seventh Framework Programme for Research of the European Commission, under FET-Open Grant No. FP7-284743. S.V.P. thanks the RFBR for partial financial support (Project No. 14-02-31735 mol_a). S.V.P. and I.A.Yu. acknowledge partial financial support from the Ministry of Education and Science of the Russian Federation (Grant No. 11.G34.31.0067) and St-Petersburg State University (SPbU) (Grant No. 11.38.213.2014). M.B. acknowledges support from the Ministry of Education and Science of the Russian Federation (Grant No. 14.Z50.31.0021).An ensemble of quantum dot excitons may be used for coherent information manipulation. Due to the ensemble inhomogeneity any optical information retrieval occurs in form of a photon echo. We show that the inhomogeneity can lead to a significant deviation from the conventional echo timing sequence. Variation of the area of the initial rotation pulse, which generates excitons in a dot subensemble only, reveals this complex picture of photon echo formation. We observe a retarded echo for π/2 pulses, while for 3π/2 the echo is advanced in time as evidenced through monitoring the Rabi oscillations in the time-resolved photon echo amplitude from (In,Ga)As/GaAs self-assembled quantum dot structures and confirmed by detailed calculations.PostprintPeer reviewe

Hybrid Organic–Inorganic Halide Post-Perovskite 3-Cyanopyridinium Lead Tribromide for Optoelectronic Applications

2D halide perovskite-like semiconductors are attractive materials for various optoelectronic applications, from photovoltaics to lasing. To date, the most studied families of such low-dimensional halide perovskite-like compounds are Ruddlesden–Popper, Dion–Jacobson, and other phases that can be derived from 3D halide perovskites by slicing along different crystallographic directions, which leads to the spatially isotropic corner-sharing connectivity type of metal-halide octahedra in the 2D layer plane. In this work, a new family of hybrid organic–inorganic 2D lead halides is introduced, by reporting the first example of the hybrid organic–inorganic post-perovskite 3-cyanopyridinium lead tribromide (3cp)PbBr3. The post-perovskite structure has unique octahedra connectivity type in the layer plane: a typical “perovskite-like” corner-sharing connectivity pattern in one direction, and the rare edge-sharing connectivity pattern in the other. Such connectivity leads to significant anisotropy in the material properties within the inorganic layer plane. Moreover, the dense organic cation packing results in the formation of 1D fully organic bands in the electronic structure, offering the prospects of the involvement of the organic subsystem into material's optoelectronic properties. The (3cp)PbBr3 clearly shows the 2D quantum size effect with a bandgap around 3.2 eV and typical broadband self-trapped excitonic photoluminescence at temperatures below 200 K