640 research outputs found
Extremely Small Energy Gap in the Quasi-One-Dimensional Conducting Chain Compound SrNbO
Resistivity, optical, and angle-resolved photoemission experiments reveal
unusual one-dimensional electronic properties of highly anisotropic
SrNbO. Along the conducting chain direction we find an extremely small
energy gap of only a few meV at the Fermi level. A discussion in terms of
typical 1D instabilities (Peierls, Mott-Hubbard) shows that neither seems to
provide a satisfactory explanation for the unique properties of SrNbO.Comment: 4 pages, 3 figure
Ag-coverage-dependent symmetry of the electronic states of the Pt(111)-Ag-Bi interface: The ARPES view of a structural transition
We studied by angle-resolved photoelectron spectroscopy the strain-related
structural transition from a pseudomorphic monolayer (ML) to a striped
incommensurate phase in an Ag thin film grown on Pt(111). We exploited the
surfactant properties of Bi to grow ordered Pt(111)-xMLAg-Bi trilayers with 0 <
x < 5 ML, and monitored the dispersion of the Bi-derived interface states to
probe the structure of the underlying Ag film. We find that their symmetry
changes from threefold to sixfold and back to threefold in the Ag coverage
range studied. Together with previous scanning tunneling microscopy and
photoelectron diffraction data, these results provide a consistent microscopic
description of the coverage-dependent structural transition.Comment: 10 pages, 9 figure
Transition from a Tomonaga-Luttinger liquid to a Fermi liquid in potassium intercalated bundles of single wall carbon nanotubes
We report on the first direct observation of a transition from a
Tomonaga-Luttinger liquid to a Fermi liquid behavior in potassium intercalated
mats of single wall carbon nanotubes (SWCNT). Using high resolution
photoemission spectroscopy an analysis of the spectral shape near the Fermi
level reveals a Tomonaga-Luttinger liquid power law scaling in the density of
states for the pristine sample and for low dopant concentration. As soon as the
doping is high enough to fill bands of the semiconducting tubes a distinct
transition to a bundle of only metallic SWCNT with a scaling behavior of a
normal Fermi liquid occurs. This can be explained by a strong screening of the
Coulomb interaction between charge carriers and/or an increased hopping matrix
element between the tubes.Comment: 5 pages, 4 figure
Silicon surface with giant spin-splitting
We demonstrate the induction of a giant Rashba-type spin-splitting on a
semiconducting substrate by means of a Bi trimer adlayer on a Si(111) wafer.
The in-plane inversion symmetry is broken so that the in-plane potential
gradient induces a giant spin-splitting with a Rashba energy of about 140 meV,
which is more than an order of magnitude larger than what has previously been
reported for any semiconductor heterostructure. The separation of the
electronic states is larger than their lifetime broadening, which has been
directly observed with angular resolved photoemission spectroscopy. The
experimental results are confirmed by relativistic first-principles
calculations. We envision important implications for basic phenomena as well as
for the semiconductor based technology
Tunable Polaronic Conduction in Anatase TiO2
Oxygen vacancies created in anatase TiO2 by UV photons (80–130 eV) provide an effective electron-doping mechanism and induce a hitherto unobserved dispersive metallic state. Angle resolved photoemission reveals that the quasiparticles are large polarons. These results indicate that anatase can be tuned from an insulator to a polaron gas to a weakly correlated metal as a function of doping and clarify the nature of conductivity in this material.open1192sciescopu
Nodal Landau Fermi-Liquid Quasiparticles in Overdoped LaSrCuO
Nodal angle resolved photoemission spectra taken on overdoped
LaSrCuO are presented and analyzed. It is proven that the
low-energy excitations are true Landau Fermi-liquid quasiparticles. We show
that momentum and energy distribution curves can be analyzed self-consistently
without quantitative knowledge of the bare band dispersion. Finally, by
imposing Kramers-Kronig consistency on the self-energy , insight into
the quasiparticle residue is gained. We conclude by comparing our results to
quasiparticle properties extracted from thermodynamic, magneto-resistance, and
high-field quantum oscillation experiments on overdoped
TlBaCuO.Comment: Accepted for publication in Phys. Rev.
Electronic Instability in a Zero-Gap Semiconductor: The Charge-DensityWave in (TaSe4)(2)I
We report a comprehensive study of the paradigmatic quasi-1D compound (TaSe4)(2)I performed by means of angle-resolved photoemission spectroscopy (ARPES) and first-principles electronic structure calculations. We find it to be a zero-gap semiconductor in the nondistorted structure, with non-negligible interchain coupling. Theory and experiment support a Peierls-like scenario for the charge-density wave formation below T-CDW = 263 K, where the incommensurability is a direct consequence of the finite interchain coupling. The formation of small polarons, strongly suggested by the ARPES data, explains the puzzling semiconductor-to-semiconductor transition observed in transport at T-CDW.open114sciescopu
The electronic structure of the high-symmetry perovskite iridate Ba2IrO4
We report angle-resolved photoemission (ARPES) measurements, density
functional and model tight-binding calculations on BaIrO (Ba-214), an
antiferromagnetic ( K) insulator. Ba-214 does not exhibit the
rotational distortion of the IrO octahedra that is present in its sister
compound SrIrO (Sr-214), and is therefore an attractive reference
material to study the electronic structure of layered iridates. We find that
the band structures of Ba-214 and Sr-214 are qualitatively similar, hinting at
the predominant role of the spin-orbit interaction in these materials.
Temperature-dependent ARPES data show that the energy gap persists well above
, and favour a Mott over a Slater scenario for this compound.Comment: 13 pages, 9 figure
Spin-Orbit-Induced Orbital Excitations in Sr2RuO4 and Ca2RuO4: A Resonant Inelastic X-ray Scattering Study
High-resolution resonant inelastic X-ray scattering (RIXS) at the oxygen
K-edge has been used to study the orbital excitations of Ca2RuO4 and Sr2RuO4.
In combination with linear dichroism X-ray absorption spectroscopy, the
ruthenium 4d-orbital occupation and excitations were probed through their
hybridization with the oxygen p-orbitals. These results are described within a
minimal model, taking into account crystal field splitting and a spin-orbit
coupling \lambda_{so}=200~meV. The effects of spin-orbit interaction on the
electronic structure and implications for the Mott and superconducting ground
states of (Ca,Sr)2RuO4 are discussed.Comment: accepted in PRB 201
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