405 research outputs found

    Incommensurate spin density modulation in a copper-oxide chain compound with commensurate charge order

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    Neutron diffraction has been used to determine the magnetic structure of Na8_8Cu5_5O10_{10}, a stoichiometric compound containing chains based on edge-sharing CuO4_4 plaquettes. The chains are doped with 2/5 hole per Cu site and exhibit long-range commensurate charge order with an onset well above room temperature. Below TN=23T_N = 23 K, the neutron data indicate long-range collinear magnetic order with a spin density modulation whose propagation vector is commensurate along and incommensurate perpendicular to the chains. Competing interchain exchange interactions are discussed as a possible origin of the incommensurate magnetic order

    Pressure induced magnetic phase separation in La0.75_{0.75}Ca0.25_{0.25}MnO3_{3} manganite

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    The pressure dependence of the Curie temperature TC(P)_{C}(P) in La0.75_{0.75}Ca0.25_{0.25}MnO3_{3} was determined by neutron diffraction up to 8 GPa, and compared with the metallization temperature TIM(P)_{IM}(P) \cite{irprl}. The behavior of the two temperatures appears similar over the whole pressure range suggesting a key role of magnetic double exchange also in the pressure regime where the superexchange interaction is dominant. Coexistence of antiferromagnetic and ferromagnetic peaks at high pressure and low temperature indicates a phase separated regime which is well reproduced with a dynamical mean-field calculation for a simplified model. A new P-T phase diagram has been proposed on the basis of the whole set of experimental data.Comment: 5 pages, 4 figure

    Magnetic structure of the edge-sharing copper oxide chain compound NaCu2O2

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    Single-crystal neutron diffraction has been used to determine the incommensurate magnetic structure of NaCu2O2, a compound built up of chains of edge-sharing CuO4 plaquettes. Magnetic structures compatible with the lattice symmetry were identified by a group-theoretical analysis, and their magnetic structure factors were compared to the experimentally observed Bragg intensities. In conjunction with other experimental data, this analysis yields an elliptical helix structure in which both the helicity and the polarization plane alternate among copper-oxide chains. This magnetic ground state is discussed in the context of the recently reported multiferroic properties of other copper-oxide chain compounds

    The Mixed Problem In L \u3csup\u3ep\u3c/sup\u3e For Some Two-dimensional Lipschitz Domains

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    We consider the mixed problem, {Δ u = 0 in Ω ∂u = f N on N u = fD on D in a class of Lipschitz graph domains in two dimensions with Lipschitz constant at most 1. We suppose the Dirichlet data, f D , has one derivative in L p (D) of the boundary and the Neumann data, f N , is in L p (N). We find a p 0 \u3e 1 so that for p in an interval (1, p 0), we may find a unique solution to the mixed problem and the gradient of the solution lies in L p

    Hall Effect in Nested Antiferromagnets Near the Quantum Critical Point

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    We investigate the behavior of the Hall coefficient in the case of antiferromagnetism driven by Fermi surface nesting, and find that the Hall coefficient should abruptly increase with the onset of magnetism, as recently observed in vanadium doped chromium. This effect is due to the sudden removal of flat portions of the Fermi surface upon magnetic ordering. Within this picture, the Hall coefficient should scale as the square of the residual resistivity divided by the impurity concentration, which is consistent with available data.Comment: published version; an accidental interchange in the quoting of sigmaxyzsigma_{xyz} analytic dependencies was correcte

    Magnetic excitations and phonons in the spin-chain compound NaCu2O2

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    We report an inelastic light scattering study of single-crystalline NaCu2_2O2_2, a spin-chain compound known to exhibit a phase with helical magnetic order at low temperatures. Phonon excitations were studied as a function of temperature and light polarization, and the phonon frequencies are compared to the results of ab-initio lattice dynamical calculations, which are also reported here. The good agreement between the observed and calculated modes allows an assignment of the phonon eigenvectors. Two distinct high-energy two-magnon features as well as a sharp low-energy one-magnon peak were also observed. These features are discussed in terms of the magnon modes expected in a helically ordered state. Their polarization dependence provides evidence of substantial exchange interactions between two closely spaced spin chains within a unit cell. At high temperatures, the spectral features attributable to magnetic excitations are replaced by a broad, quasielastic mode due to overdamped spin excitations

    Helicoidal magnetic order in a clean copper oxide spin chain compound

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    We report susceptibility, specific heat, and neutron diffraction measurements on NaCu2_2O2_2, a spin-1/2 chain compound isostructural to LiCu2_2O2_2, which has been extensively investigated. Below 13 K, we find a long-range ordered, incommensurate magnetic helix state with a propagation vector similar to that of LiCu2_2O2_2. In contrast to the Li analogue, substitutional disorder is negligible in NaCu2_2O2_2. We can thus rule out that the helix is induced by impurities, as was claimed on the basis of prior work on LiCu2_2O2_2. A spin Hamiltonian with frustrated longer-range exchange interactions provides a good description of both the ordered state and the paramagnetic susceptibility.Comment: 4 pages, 4 figures Improved Fig.1 and 4. Minor rephrasing. Reference adde

    Competing magnetic fluctuations in Sr3Ru2O7 probed by Ti doping

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    We report the effect of nonmagnetic Ti4+ impurities on the electronic and magnetic properties of Sr3Ru2O7. Small amounts of Ti suppress the characteristic peak in magnetic susceptibility near 16 K and result in a sharp upturn in specific heat. The metamagnetic quantum phase transition and related anomalous features are quickly smeared out by small amounts of Ti. These results provide strong evidence for the existence of competing magnetic fluctuations in the ground state of Sr3Ru2O7. Ti doping suppresses the low temperature antiferromagnetic interactions that arise from Fermi surface nesting, leaving the system in a state dominated by ferromagnetic fluctuations.Comment: 5 pages, 4 figures, 1 tabl

    Understanding the effect of cognitive/brain reserve and depression on regional atrophy in early Alzheimer’s disease

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    Introduction: Depression in patients with mild cognitive impairment (MCI) and dementia of the Alzheimer’s type (AD) is associated with worse prognosis. Indeed, depressed MCI patients have worse cognitive performance and greater loss of gray-matter volume in several brain areas. To date, knowledge of the factors that can mitigate this detrimental effect is still limited. The aim of the present study was to understand in what way cognitive reserve/brain reserve and depression interact and are linked to regional atrophy in early stage AD. Methods: Depression was evaluated with the Patient Health Questionnaire-9 in 90 patients with early AD, and a cutoff of ≥ 5 was used to separate depressed (n = 44) from non-depressed (n = 46) patients. Each group was further stratified into high/low cognitive reserve/brain reserve. Cognitive reserve was calculated using years of education as proxy, while normalized parenchymal volumes were used to estimate brain reserve. Voxel-based morphometry was carried out to extract and analyze gray-matter maps. 2 × 2 ANCOVAs were run to test the effect of the reserve-by-depression interaction on gray matter. Age and hippocampal ratio were used as covariates. Composite indices of major cognitive domains were also analyzed with comparable models. Results: No reserve-by-depression interaction was found in the analytical models of gray matter. Depression was associated with less gray matter volume in the cerebellum and parahippocampal gyrus. The brain reserve-by-depression interaction was a significant predictor of executive functioning. Among those with high brain reserve, depressed patients had poorer executive skills. No significant results were found in association with cognitive reserve. Conclusion: These findings suggest that brain reserve may modulate the association between neurodegeneration and depression in patients with MCI and dementia of the AD type, influencing in particular executive functioning

    Dispersion of the odd magnetic resonant mode in near-optimally doped Bi2Sr2CaCu2O8+d

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    We report a neutron scattering study of the spin excitation spectrum in the superconducting state of slightly overdoped Bi2Sr2CaCu2O8+d system (Tc=87 K). We focus on the dispersion of the resonance peak in the superconducting state that is due to a S=1 collective mode. The measured spin excitation spectrum bears a strong similarity to the spectrum of the YBa2Cu3O6+x system for a similar doping level i.e. x= 0.95-1), which consists of intersecting upward- and downward-dispersing branches. A close comparison of the threshold of the electron-hole spin flip continuum, deduced from angle resolved photo-emission measurements in the same system, indicates that the magnetic response in the superconducting state is confined, in both energy and momentum, below the gapped Stoner continuum. In contrast to YBa2Cu3O6+x, the spin excitation spectrum is broader than the experimental resolution. In the framework of an itinerant-electron model, we quantitatively relate this intrinsic energy width to the superconducting gap distribution observed in scanning tunnelling microscopy experiments. Our study further suggests a significant in-plane anisotropy of the magnetic response.Comment: 10 figure
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