Nuclear structure investigations of Es 253-255 by laser spectroscopy

Laser resonance ionization spectroscopy was performed on the rare einsteinium isotopes Es253-255 at the RISIKO mass separator in Mainz. With low sample sizes ranging down to femtograms, the prominent 352 nm-ground-state transition was measured in all three einsteinium isotopes, and four additional ground-state transitions were measured in Es254. Hyperfine-structure analysis resulted in assigned spin values of I(Es254)=7 and I(Es255)=7/2. From the extracted coupling constants, nuclear magnetic dipole moments of μI(Es254)=3.42(7)μN and μI(Es255)=4.14(10)μN as well as spectroscopic electric quadrupole moments of Qs(Es254)=9.6(1.2)eb and Qs(Es255)=5.1(1.7)eb were derived. Our value for Es254 deviates from the value of |μI(Es254)|=4.35(41)μN extracted from the angular anisotropy of α-radiation emitted by Es254

Precision Measurement of the First Ionization Potential of Nobelium

One of the most important atomic properties governing an element's chemical behavior is the energy required to remove its least-bound electron, referred to as the first ionization potential. For the heaviest elements, this fundamental quantity is strongly influenced by relativistic effects which lead to unique chemical properties. Laser spectroscopy on an atom-at-a-time scale was developed and applied to probe the optical spectrum of neutral nobelium near the ionization threshold. The first ionization potential of nobelium is determined here with a very high precision from the convergence of measured Rydberg series to be 6.626 21±0.000 05  eV. This work provides a stringent benchmark for state-of-the-art many-body atomic modeling that considers relativistic and quantum electrodynamic effects and paves the way for high-precision measurements of atomic properties of elements only available from heavy-ion accelerator facilities.status: publishe

Experimental study of the U238(S36,3-5n)Hs269-271 reaction leading to the observation of Hs270

The deformed doubly magic nucleus Hs270 has so far only been observed as the four-neutron (4n) evaporation residue of the reaction Mg26+Cm248, where a maximum cross section of 3 pb was measured. Theoretical studies on the formation of Hs270 in the 4n evaporation channel of fusion reactions with different entrance channel asymmetry in the framework of a two-parameter Smoluchowski equation predict that the reactions Ca48+Ra226 and S36+U238 result in higher cross sections due to lower reaction Q values, in contrast to simple arguments based on the reaction asymmetry, which predict opposite trends. Calculations using hivap predict cross sections for the reaction S36+U238 that are similar to those of the Mg26+Cm248 reaction. Here, we report on the first measurement of evaporation residues formed in the complete nuclear fusion reaction S36+U238 and the observation of Hs270, which is produced in the 4n evaporation channel, with a measured cross section of 0.8-0.7+2.6 pb at 51-MeV excitation energy. The one-event cross-section limits (68% confidence level) for the 3n, 4n, and 5n evaporation channels at 39-MeV excitation energy are 2.9 pb, while the cross-section limits of the 3n and 5n channel at 51 MeV are 1.5 pb. This is significantly lower than the 5n cross section of the Mg26+Cm248 reaction at similar excitation energy. © 2010 The American Physical Society

Decay spectroscopy of element 115 daughters: Rg 280 → Mt 276 and Mt 276 → Bh 272

Forty-six decay chains, assigned to the decay of 115288, were produced using the Am243(Ca48,3n)115288 reaction at the Lawrence Berkeley National Laboratory 88-in. cyclotron. The resulting series of α decays were studied using α-photon and α-x-ray spectroscopies. Multiple α-photon coincidences were observed in the element 115 decay chain members, particularly in the third- and fourth-generation decays (presumed to be Rg280 and Mt276, respectively). Upon combining these data with those from 22 115288 decay chains observed in a similar experiment, updated level schemes in Mt276 and Bh272 (populated by the α decay of Rg280 and Mt276, respectively) are proposed. Photons were observed in the energy range expected for K x rays coincident with the α decay of both Rg280 and Mt276. However, Compton scattering of higher-energy γ rays and discrete transitions are present in the K x-ray region preventing a definitive Z identification to be made based on observation of characteristic K x-ray energies

Low-lying states in Ra 219 and Rn 215: Sampling microsecond α -decaying nuclei

Short-lived α-decaying nuclei "northeast" of Pb208 in the chart of nuclides were studied using the reaction Ca48+Am243 with the decay station TASISpec at TASCA, GSI Darmstadt. Decay energies and times from pile-up events were extracted with a tailor-made pulse-shape analysis routine and specific α-decay chains were identified in a correlation analysis. Decay chains starting with the even-even Ra220 and its odd-A neighbors, Fr219, and Ra221,219, with a focus on the Ra219→Rn215 decay, were studied by means of α-γ spectroscopy. A revised α-decay scheme of Ra219 is proposed, including a new decay branch from a previously not considered isomeric state at 17 keV excitation energy. Conclusions on nuclear structure are drawn from the experimental data, aided by Geant4 simulations and a discussion on theoretical calculations

Alpha-photon coincidence spectroscopy along element 115 decay chains

Produced in the reaction 48Ca+243Am, thirty correlated α-decay chains were observed in an experiment conducted at the GSI Helmholzzentrum für Schwerionenforschung, Darmstadt, Germany. The decay chains are basically consistent with previous findings and are considered to originate from isotopes of element 115 with mass numbers 287, 288, and 289. A set-up aiming specifically for high-resolution charged particle and photon coincidence spectroscopy was placed behind the gas-filled separator TASCA. For the first time, γ rays as well as X-ray candidates were observed in prompt coincidence with the α-decay chains of element 115