6,779 research outputs found

    From Chemistry to Functionality: Trends for the Length Dependence of the Thermopower in Molecular Junctions

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    We present a systematic ab-initio study of the length dependence of the thermopower in molecular junctions. The systems under consideration are small saturated and conjugated molecular chains of varying length attached to gold electrodes via a number of different binding groups. Different scenarios are observed: linearly increasing and decreasing thermopower as function of the chain length as well as positive and negative values for the contact thermopower. Also deviation from the linear behaviour is found. The trends can be explained by details of the transmission, in particular the presence, position and shape of resonances from gateway states. We find that these gateway states do not only determine the contact thermopower, but can also have a large influence on the length-dependence itself. This demonstrates that simple models for electron transport do not apply in general and that chemical trends are hard to predict. Furthermore, we discuss the limits of our approach based on Density Functional Theory and compare to more sophisticated methods like self-energy corrections and the GW theory

    Atom-molecule theory of broad Feshbach resonances

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    We derive the atom-molecule theory for an atomic gas near a broad Feshbach resonance, where the energy dependence of the atom-molecule coupling becomes crucial for understanding experimental results. We show how our many-body theory incorporates the two-atom physics exactly. In particular, we calculate the magnetic moment of a two-component gas of ^{6}Li atoms for a wide range of magnetic fields near the broad Feshbach resonance at about 834 Gauss. We find excellent agreement with the experiment of Jochim et al. [Phys. Rev. Lett. 91, 240402 (2003)].Comment: 4 pages, 2 figure

    Quantum annealing and the Schr\"odinger-Langevin-Kostin equation

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    We show, in the context of quantum combinatorial optimization, or quantum annealing, how the nonlinear Schr\"odinger-Langevin-Kostin equation can dynamically drive the system toward its ground state. We illustrate, moreover, how a frictional force of Kostin type can prevent the appearance of genuinely quantum problems such as Bloch oscillations and Anderson localization which would hinder an exhaustive search.Comment: 5 pages, 4 figures. To appear on Physical Review

    Crossover temperature of Bose-Einstein condensation in an atomic Fermi gas

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    We show that in an atomic Fermi gas near a Feshbach resonance the crossover between a Bose-Einstein condensate of diatomic molecules and a Bose-Einstein condensate of Cooper pairs occurs at positive detuning, i.e., when the molecular energy level lies in the two-atom continuum. We determine the crossover temperature as a function of the applied magnetic field and find excellent agreement with the experiment of Regal et al. [Phys. Rev. Lett. 92, 040403 (2004)] that has recently observed this crossover temperature.Comment: 4 pages, 2 figure

    Natural Disasters and Preferences for the Environment: Evidence from the Impressionable Years

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    Do generations affected by natural disasters during the critical years of adolescence and early adulthood form different preferences towards the environment than generations who are not? Consistent with the theories of social psychology, we show that an environmental shock experienced during the impressionable years (18-25 years old) help shape positive environmental preferences. Individuals tend not to change beliefs in response to natural disasters experienced in other age ranges. Using information from the General Social Survey and World Values Survey, we exploit yearly natural disasters variation both within the US and across countries to identify these effects

    Natural Disasters and Preferences for the Environment: Evidence from the Impressionable Years

    Get PDF
    Do generations a˙ected by natural disasters during the critical years of adolescence and early adulthood form di˙erent preferences towards the environment than generations who are not? Consistent with the theories of social psychology, we show that an environmental shock experienced during the impressionable years (18-25 years old) help shape positive environmental preferences. Individuals tend not to change beliefs in response to natural disasters experienced in other age ranges. Using information from the General Social Survey and World Values Survey, we exploit yearly natural disasters variation both within the US and across countries to identify these effects
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