Signatures of Hund Metal and Fermi Liquid Behavior in Sr2_2RuO4_4 Revealed by Electronic Raman Scattering

We investigate the electronic Raman scattering of Sr$_2$RuO$_4$ using a material-realistic dynamical mean-field theory approach. We identify the low-energy Fermi liquid behavior and point out that the enhanced Raman response at higher energies displays clear signatures of Hund metals physics. These signatures originate in the two-stage coherence of Hund metals and associated quasiparticle 'unrenormalization'. In agreement with recent experimental observations we find a strong dichotomy between the $\mathrm{B}_{1g}$ and $\mathrm{B}_{2g}$ response, but our calculations suggest a novel interpretation of this dichotomy. The $\mathrm{B}_{1g}$ response is dominated by the $xy$ orbital and the $\mathrm{B}_{2g}$ response receives contributions from all orbitals and is strongly affected by interband nesting at finite frequencies.Comment: 7 pages, 4 figures. SM: 5 pages, 8 figure

Magnetic phase diagram of the infinite- U Hubbard model with nearest- and next-nearest-neighbor hoppings

We study the infinite-U Hubbard model on ladders of two, four, and six legs with nearest- (t) and next-nearest- (t′) neighbor hoppings by means of the density-matrix renormalization group algorithm. In particular, we analyze the stability of the Nagaoka state for several values of t′ when we vary the electron density ρ from half filling to the low-density limit. We build the two-dimensional phase diagram, where the fully spin polarized and paramagnetic states prevail. We find that the inclusion of a nonfrustrating next-nearest-neighbor hopping stabilizes the fully spin polarized phase up until |t′/t|=0.5. Surprisingly, for this value of t′, the ground state is fully spin polarized for almost any electron density 1 ρ 0, connecting the Nagaoka state to itinerant ferromagnetism at low density. Also, we find that the previously found checkerboard insulator phase at t′=0 and ρ=0.75 is unstable against t′.Fil: Blesio, Germán Gabriel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Gonzalez, Matías Gabriel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Lisandrini, Franco Thomas. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; Argentin

Iron phthalocyanine on Au(111) is a “non-Landau” Fermi liquid

The paradigm of Landau’s Fermi liquid theory has been challenged with the finding of a strongly interacting Fermi liquid that cannot be adiabatically connected to a non-interacting system. A spin-1 two-channel Kondo impurity with anisotropy D has a quantum phase transition between two topologically different Fermi liquids with a peak (dip) in the Fermi level for D Dc). Extending this theory to general multi-orbital problems with finite magnetic field, we reinterpret in a unified and consistent fashion several experimental studies of iron phthalocyanine molecules on Au(111) that were previously described in disconnected and conflicting ways. The differential conductance shows a zero-bias dip that widens when the molecule is lifted from the surface (reducing the Kondo couplings) and is transformed continuously into a peak under an applied magnetic field. We reproduce all features and propose an experiment to induce the topological transition.Fil: Zitko, R.. University Of Ljubljana; EsloveniaFil: Blesio, Germán Gabriel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Manuel, Luis Oscar. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Aligia, Armando Ángel. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Unidad Ejecutora Instituto de Nanociencia y Nanotecnología. Unidad Ejecutora Instituto de Nanociencia y Nanotecnología - Nodo Bariloche | Comisión Nacional de Energía Atómica. Unidad Ejecutora Instituto de Nanociencia y Nanotecnología. Unidad Ejecutora Instituto de Nanociencia y Nanotecnología - Nodo Bariloche; Argentin

Topological quantum phase transition between Fermi liquid phases in an Anderson impurity model

We study a generalized Anderson model that mixes two localized configurations-one formed by two degenerate doublets and the other by a triplet with single-ion anisotropy DSz2-by means of two degenerate conduction channels. The model has been derived for a single Ni impurity embedded into an O-doped Au chain. Using the numerical renormalization group, we find a topological quantum phase transition, at a finite value Dc, between two regular Fermi liquid phases of high (low) conductance and topological number 2IL/π=0 (+1) for DDc), where IL is the well-known Luttinger integral. At finite temperature the two phases are separated by a non-Fermi liquid phase with fractional impurity entropy 12ln2 and other properties which are similar to those of the two-channel Kondo model.Fil: Blesio, Germán Gabriel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Manuel, Luis Oscar. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Roura Bas, Pablo Gines. Comisión Nacional de Energía Atómica. Gerencia del Área de Energía Nuclear. Instituto Balseiro; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaFil: Aligia, Armando Ángel. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Comisión Nacional de Energía Atómica. Gerencia del Área de Energía Nuclear. Instituto Balseiro; Argentin

Fully compensated Kondo effect for a two-channel spin S=1 impurity

We study the low-temperature properties of the generalized Anderson impurity model in which two localized configurations, one with two doublets and the other with a triplet, are mixed by two degenerate conduction channels. By using the numerical renormalization group and the noncrossing approximation, we analyze the impurity entropy, its spectral density, and the equilibrium conductance for several values of the model parameters. Marked differences with respect to the conventional one-channel spin s=1/2 Anderson model, which can be traced as hallmarks of an impurity spin S=1, are found in the Kondo temperature, the width and position of the charge-transfer peak, and the temperature dependence of the equilibrium conductance. Furthermore, we analyze the rich effects of a single-ion magnetic anisotropy D on the Kondo behavior. In particular, as shown before, for large enough positive D the system behaves as a "non-Landau" Fermi liquid that cannot be adiabatically connected to a noninteracting system turning off the interactions. For negative D the Kondo effect is strongly suppressed. While the model is suitable for the description of a single Ni impurity embedded in an O-doped Au chain, it is a generic one for S=1 and two channels and might be realized in other nanoscopic systems.Fil: Blesio, Germán Gabriel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Manuel, Luis Oscar. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Aligia, Armando Angel. Comisión Nacional de Energía Atómica. Gerencia del Área de Energía Nuclear. Instituto Balseiro. Archivo Histórico del Centro Atómico Bariloche e Instituto Balseiro | Universidad Nacional de Cuyo. Instituto Balseiro. Archivo Histórico del Centro Atómico Bariloche e Instituto Balseiro; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Patagonia Norte; ArgentinaFil: Roura Bas, Pablo Gines. Comisión Nacional de Energía Atómica. Gerencia del Área de Energía Nuclear. Instituto Balseiro. Archivo Histórico del Centro Atómico Bariloche e Instituto Balseiro | Universidad Nacional de Cuyo. Instituto Balseiro. Archivo Histórico del Centro Atómico Bariloche e Instituto Balseiro; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Patagonia Norte; Argentin

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