Controlling single diamond NV color center photoluminescence spectrum with a Fabry-Perot microcavity

We present both theoretical and experimental results on fluorescence of single defect centers in diamond nanocrystals embedded in a planar dielectric microcavity. From a theoretical point of view, we show that the overall fluorescence collection efficiency using moderate numerical aperture microscope objective can be enhanced by using a low quality factor microcavity. This could be used in particular for low temperature applications where the numerical aperture of collection microscope objectives is limited due to the experimental constraints. We experimentally investigate the control of the fluorescence spectrum of the emitted light from a single center. We show the simultaneous narrowing of the room temperature broadband emission spectrum and the increase of the fluorescence spectral density.Comment: 22 pages, 10 figure

Frequency tuning of the whispering gallery modes of silica microspheres for CQED and spectroscopy

We have tuned the whispering gallery modes of a fused silica microresonator over nearly 1 nm at 800 nm, i.e. over 0.5 FSR or 10^6 linewidths of the resonator. This has been achieved by a new method based on the stretching of a two-stem microsphere. The devices described below will permit new Cavity-QED experiments with this high-Q optical resonator when it is desirable to optimize its coupling to emitters with given transition frequencies. The tuning capability demonstrated here is compatible with both UHV and low temperature operation, which should be useful for future experiments with laser cooled atoms or single quantum dots.Comment: ReVTeX, 4 pages, 3 figure

Narrow-band single-photon emission in the near infrared for quantum key distribution

We report on the observation of single colour centers in natural diamond samples emitting in the near infrared region when optically excited. Photoluminescence of these single emitters have several striking features, such as a narrow-band fully polarized emission (FWHM 2 nm) around 780 nm, a short excited-state lifetime of about 2 ns, and perfect photostability at room temperature under our excitation conditions. We present a detailed study of their photophysical properties. Development of a triggered single-photon source relying on this single colour centre is discussed in the prospect of its application to quantum key distribution.Comment: 9 page

Direct Measurement of the Photon Statistics of a Triggered Single Photon Source

We studied intensity fluctuations of a single photon source relying on the pulsed excitation of the fluorescence of a single molecule at room temperature. We directly measured the Mandel parameter Q(T) over 4 orders of magnitude of observation timescale T, by recording every photocount. On timescale of a few excitation periods, subpoissonian statistics is clearly observed and the probablility of two-photons events is 10 times smaller than Poissonian pulses. On longer times, blinking in the fluorescence, due to the molecular triplet state, produces an excess of noise.Comment: 4 pages, 3 figures, 1 table submitted to Physical Review Letter

Wheeler's delayed-choice thought experiment: Experimental realization and theoretical analysis

Wheeler has strikingly illustrated the wave-particle duality by the delayed-choice thought experiment, in which the configuration of a 2-path interferometer is chosen after a single-photon light-pulsed has entered it. We present a quantitative theoretical analysis of an experimental realization of Wheeler's proposal

Experimental realization of Wheeler's delayed-choice GedankenExperiment

The quantum "mystery which cannot go away" (in Feynman's words) of wave-particle duality is illustrated in a striking way by Wheeler's delayed-choice GedankenExperiment. In this experiment, the configuration of a two-path interferometer is chosen after a single-photon pulse has entered it : either the interferometer is \textit{closed} (\textit{i.e.} the two paths are recombined) and the interference is observed, or the interferometer remains \textit{open} and the path followed by the photon is measured. We report an almost ideal realization of that GedankenExperiment, where the light pulses are true single photons, allowing unambiguous which-way measurements, and the interferometer, which has two spatially separated paths, produces high visibility interference. The choice between measuring either the 'open' or 'closed' configuration is made by a quantum random number generator, and is space-like separated -- in the relativistic sense -- from the entering of the photon into the interferometer. Measurements in the closed configuration show interference with a visibility of 94%, while measurements in the open configuration allow us to determine the followed path with an error probability lower than 1%