Long-range Energy Transfer and Ionization in Extended Quantum Systems Driven by Ultrashort Spatially Shaped Laser Pulses

The processes of ionization and energy transfer in a quantum system composed of two distant H atoms with an initial internuclear separation of 100 atomic units (5.29 nm) have been studied by the numerical solution of the time-dependent Schr\"odinger equation beyond the Born-Oppenheimer approximation. Thereby it has been assumed that only one of the two H atoms was excited by temporally and spatially shaped laser pulses at various laser carrier frequencies. The quantum dynamics of the extended H-H system, which was taken to be initially either in an unentangled or an entangled ground state, has been explored within a linear three-dimensional model, including two z coordinates of the electrons and the internuclear distance R. An efficient energy transfer from the laser-excited H atom (atom A) to the other H atom (atom B) and the ionization of the latter have been found. It has been shown that the physical mechanisms of the energy transfer as well as of the ionization of atom B are the Coulomb attraction of the laser driven electron of atom A by the proton of atom B and a short-range Coulomb repulsion of the two electrons when their wave functions strongly overlap in the domain of atom B.Comment: 11 pages, 7 figure

Electronic dynamics and frequency-dependent effects in circularly polarized strong-field physics

We analyze, quantum mechanically, the dynamics of ionization with a strong, circularly polarized, laser field. We show that the main source for non-adiabatic effects is connected to an effective barrier lowering due to the laser frequency. Such non-adiabatic effects manifest themselves through ionization rates and yields that depart up to more than one order of magnitude from a static-field configuration. Beyond circular polarization, these results show the limits of standard instantaneous - static-field like - interpretation of laser-matter interaction and the great need for including time dependent electronic dynamics

Analysis of strong-field enhanced ionization of molecules using Bohmian trajectories

We theoretically investigate the mechanism of enhanced ionization in two-electron molecules by analyzing Bohmian trajectories for a one-dimensional H2 in an intense laser field. We identify both types of ionizing trajectories corresponding to the ejection from the up-field and down-field cores. The trajectories of the two electrons are correlated with each other in the former while correlation is negligible in the latter. The contributions from the two ionization types, though depending on laser intensity and internuclear distance, are comparable to each other.Comment: 9 pages, 9 figure

Circularly Polarized Molecular High Harmonic Generation Using a Bicircular Laser

We investigate the process of circularly polarized high harmonic generation in molecules using a bicircular laser field. In this context, we show that molecules offer a very robust framework for the production of circularly polarized harmonics, provided their symmetry is compatible with that of the laser field. Using a discrete time-dependent symmetry analysis, we show how all the features (harmonic order and polarization) of spectra can be explained and predicted. The symmetry analysis is generic and can easily be applied to other target and/or field configurations

Resonantly enhanced pair production in a simple diatomic model

A new mechanism for the production of electron-positron pairs from the interaction of a laser field and a fully stripped diatomic molecule in the tunneling regime is presented. When the laser field is turned off, the Dirac operator has resonances in both the positive and the negative energy continua while bound states are in the mass gap. When this system is immersed in a strong laser field, the resonances move in the complex energy plane: the negative energy resonances are pushed to higher energies while the bound states are Stark shifted. It is argued here that there is a pair production enhancement at the crossing of resonances by looking at a simple 1-D model: the nuclei are modeled simply by Dirac delta potential wells while the laser field is assumed to be static and of finite spatial extent. The average rate for the number of electron-positron pairs produced is evaluated and the results are compared to the single nucleus and to the free cases. It is shown that positrons are produced by the Resonantly Enhanced Pair Production (REPP) mechanism, which is analogous to the resonantly enhanced ionization of molecular physics. This phenomenon could be used to increase the number of pairs produced at low field strength, allowing the study of the Dirac vacuum.Comment: 11 pages, 4 figure