Determining the Electron-Phonon Coupling Strength in Correlated Electron Systems from Resonant Inelastic X-ray Scattering

We show that high resolution Resonant Inelastic X-ray Scattering (RIXS) provides direct, element-specific and momentum-resolved information on the electron-phonon (e-p) coupling strength. Our theoretical analysis demonstrates that the e-p coupling can be extracted from RIXS spectra by determining the differential phonon scattering cross section. An alternative, very direct manner to extract the coupling is to use the one and two-phonon loss ratio, which is governed by the e-p coupling strength and the core-hole life-time. This allows measurement of the e-p coupling on an absolute energy scale.Comment: 4 pages, 3 figure

Hamiltonian for coupled flux qubits

An effective Hamiltonian is derived for two coupled three-Josephson-junction (3JJ) qubits. This is not quite trivial, for the customary "free" 3JJ Hamiltonian is written in the limit of zero inductance L. Neglecting the self-flux is already dubious for one qubit when it comes to readout, and becomes untenable when discussing inductive coupling. First, inductance effects are analyzed for a single qubit. For small L, the self-flux is a "fast variable" which can be eliminated adiabatically. However, the commonly used junction phases are_not_ appropriate "slow variables", and instead one introduces degrees of freedom which are decoupled from the loop current to leading order. In the quantum case, the zero-point fluctuations (LC oscillations) in the loop current diverge as L->0. Fortunately, they merely renormalize the Josephson couplings of the effective (two-phase) theory. In the coupled case, the strong zero-point fluctuations render the full (six-phase) wave function significantly entangled in leading order. However, in going to the four-phase theory, this uncontrollable entanglement is integrated out completely, leaving a computationally usable mutual-inductance term of the expected form as the effective interaction.Comment: REVTeX4, 16pp., one figure. N.B.: "Alec" is my first, and "Maassen van den Brink" my family name. Informal note. v2: completely rewritten; correction of final result and major expansion. v3: added numerical verification plus a discussion of Ref. [2

Orbital excitations in LaMnO3_3

We study the recently observed orbital excitations, orbitons, and treat electron-electron correlations and lattice dynamics on equal footing. It is shown that the orbiton energy and dispersion are determined by both correlations and lattice-vibrations. The electron-phonon coupling causes satellite structures in the orbiton spectral function and the elementary excitations of the system are mixed modes with both orbital and phonon character. It is proposed that the satellite structures observed in recent Raman-scattering experiments on LaMnO$_3$ are actually orbiton derived satellites in the phonon spectral function, caused by the phonon-orbiton interaction.Comment: 4 pages, 3 figures embedde

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Excitonic quasiparticles in a spin-orbit Mott insulator

In condensed matter systems, out of a large number of interacting degrees of freedom emerge weakly coupled particles, in terms of which most physical properties are described. For example, Landau quasiparticles (QP) determine all electronic properties of a normal metal. The lack of identification of such QPs is major barrier for understanding myriad exotic properties of correlated electrons, such as unconventional superconductivity and non-Fermi liquid behaviours. Here, we report the observation of a composite particle in a Mott insulator Sr2IrO4---and exciton dressed with magnons---that propagates with the canonical characteristics of a QP: a finite QP residue and a lifetime longer than the hopping time scale. The dynamics of this charge-neutral bosonic excitation mirrors the fundamental process of the analogous one-hole propagation in the background of ordered spins, for which a well-defined QP has never been observed. The much narrower linewidth of the exciton reveals the same intrinsic dynamics that is obscured for the hole and is intimately related to the mechanism of high temperature superconductivity.Comment: submitted versio

Reentrant metallic transition at a temperature above Tc at the breakdown of cooperative Jahn-Teller orbital order in perovskite manganites

We report an interesting reentrant metallic resistivity pattern beyond a characteristic temperature T* which is higher than other such characteristic transition temperatures like T(c)(Curie point), T(N) (Neel point), T(CO) (charge order onset point) or T(OO) (orbital order onset point) in a range of rare-erath perovskite manganites (RE(1-x)A(x)MnO(3); RE = La, Nd, Y; A = Sr, Ca; x = 0.0-0.5). Such a behavior is normally observed in doped manganites with doping level (x) higher than the critical doping level x(c) (= 0.17-0.22) required for the metallic ground state to emerge and hence in a system where cooperative Jahn-Teller orbital order has already undergone a breakdown. However, the observation made in the La(1-x)Ca(x)MnO(3) (x = 0.0-0.5) series turns out to be an exception to this general trend.Comment: 15 pages including 3 figures; pdf onl

Interface-induced d-wave pairing

We discuss a scenario for interface-induced superconductivity involving pairing by dipolar excitations proximate to a two-dimensional electron system controlled by a transverse electric field. If the interface consists of transition metal oxide materials, the repulsive on-site Coulomb interaction is typically strong and a superconducting state is formed via exchange of non-local dipolar excitations in the d-wave channel. Perspectives to enhance the superconducting transition temperature are discussed.Comment: 4 pages, 3 figure

New light on magnetic excitations: indirect resonant inelastic X-ray scattering on magnons

Recent experiments show that indirect resonant inelastic X-ray scattering (RIXS) is a new probe of spin dynamics. Here I derive the cross-section for magnetic RIXS and determine the momentum dependent four-spin correlation function that it measures. These results show that this technique offers information on spin dynamics that is complementary to e.g. neutron scattering. The RIXS spectrum of Heisenberg antiferromagnets is calculated. It turns out that only scattering processes that involve at least two magnons are allowed. Other selection rules imply that the scattering intensity vanishes for specific transferred momenta ${\bf q}$, in particular for ${\bf q}=0$. The calculated spectra agree very well with the experimental data.Comment: 4 pages, 3 figure