263 research outputs found
Magnetic properties of nanoscale compass-Heisenberg planar clusters
We study a model of spins 1/2 on a square lattice, generalizing the quantum
compass model via the addition of perturbing Heisenberg interactions between
nearest neighbors, and investigate its phase diagram and magnetic excitations.
This model has motivations both from the field of strongly correlated systems
with orbital degeneracy and from that of solid-state based devices proposed for
quantum computing. We find that the high degeneracy of ground states of the
compass model is fragile and changes into twofold degenerate ground states for
any finite amplitude of Heisenberg coupling. By computing the spin structure
factors of finite clusters with Lanczos diagonalization, we evidence a rich
variety of phases characterized by Z2 symmetry, that are either ferromagnetic,
C-type antiferromagnetic, or of Neel type, and analyze the effects of quantum
fluctuations on phase boundaries. In the ordered phases the anisotropy of
compass interactions leads to a finite excitation gap to spin waves. We show
that for small nanoscale clusters with large anisotropy gap the lowest
excitations are column-flip excitations that emerge due to Heisenberg
perturbations from the manifold of degenerate ground states of the compass
model. We derive an effective one-dimensional XYZ model which faithfully
reproduces the exact structure of these excited states and elucidates their
microscopic origin. The low energy column-flip or compass-type excitations are
robust against decoherence processes and are therefore well designed for
storing information in quantum computing. We also point out that the dipolar
interactions between nitrogen-vacancy centers forming a rectangular lattice in
a diamond matrix may permit a solid-state realization of the anisotropic
compass-Heisenberg model.Comment: 24 pages, 18 figure
Photoemission spectra of LaMnO3 controlled by orbital excitations
We investigate the spectral function of a hole moving in the orbital-ordered
ferromagnetic planes of LaMnO, and show that it depends critically on the
type of orbital ordering. While the hole does not couple to the spin
excitations, it interacts strongly with the excitations of orbitals
(orbitons), leading to new type of quasiparticles with a dispersion on the
orbiton energy scale and with strongly enhanced mass and reduced weight.
Therefore we predict a large redistribution of spectral weight with respect to
the bands found in local density approximation (LDA) or in LDA+U.Comment: 4 pages, 4 figures, 3 figures embedded, figure 3 correcte
Ab initio calculation of resonant X-ray scattering in Manganites
We study the origin of the resonant x-ray signal in manganites and generalize
the resonant cross-section to the band structure framework. With {\it ab
initio} LSDA and LSDA+U calculations we determine the resonant x-ray spectrum
of LaMnO. The calculated spectrum and azimuthal angle dependence at the Mn
-edge reproduce the measured data without adjustable parameters. The
intensity of this signal is directly related to the orthorhombicity of the
lattice. We also predict a resonant x-ray signal at the La -edge, caused by
the tilting of the MnO octahedra. This shows that the resonant x-ray signal
in the hard x-ray regime can be understood in terms of the band structure of a
material and is sensitive to the fine details of crystal structure.Comment: 4 pages, 4 figures, accepted for publication in Phys. Rev.
Applying HDACis to increase SSTR2 expression and radiolabeled DOTA-TATE uptake:from cells to mice
Aims: The aim of our study was to determine the effect of histone deacetylase (HDAC) inhibitors (HDACis) on somatostatin type-2 receptor (SSTR2) expression and [111In]In-/[177Lu]Lu-DOTA-TATE uptake in vitro and in vivo. Materials and methods: The human cell lines NCI-H69 (small-cell lung carcinoma) and BON-1 (pancreatic neuroendocrine tumor) were treated with HDACis (i.e. entinostat, mocetinostat (MOC), LMK-235, CI-994 or panobinostat (PAN)), and SSTR2 mRNA expression levels and [111In]In-DOTA-TATE uptake were measured. Furthermore, vehicle- and HDACi-treated NCI-H69 and BON-1 tumor-bearing mice were injected with radiolabeled DOTA-TATE followed by biodistribution studies. Additionally, SSTR2 and HDAC mRNA expression of xenografts, and of NCI-H69, BON-1, NCI-H727 (human pulmonary carcinoid) and GOT1 (human midgut neuroendocrine tumor) cells were determined. Key findings: HDACi treatment resulted in the desired effects in vitro. However, no significant increase in tumoral DOTA-TATE uptake was observed after HDACi treatment in NCI-H69 tumor-bearing animals, whereas tumoral SSTR2 mRNA and/or protein expression levels were significantly upregulated after treatment with MOC, CI-994 and PAN, i.e. a maximum of 2.1- and 1.3-fold, respectively. Analysis of PAN-treated BON-1 xenografts solely demonstrated increased SSTR2 mRNA expression levels. Comparison of HDACs and SSTR2 expression in BON-1 and NCI-H69 xenografts showed a significantly higher expression of 6/11 HDACs in BON-1 xenografts. Of these HDACs, a significant inverse correlation was found between HDAC3 and SSTR2 expression (Pearson r = −0.92) in the studied cell lines. Significance: To conclude, tumoral uptake levels of radiolabeled DOTA-TATE were not enhanced after HDACi treatment in vivo, but, depending on the applied inhibitor, increased SSTR2 expression levels were observed.</p
Four-qubit device with mixed couplings
We present the first experimental results on a device with more than two
superconducting qubits. The circuit consists of four three-junction flux
qubits, with simultaneous ferro- and antiferromagnetic coupling implemented
using shared Josephson junctions. Its response, which is dominated by the
ground state, is characterized using low-frequency impedance measurement with a
superconducting tank circuit coupled to the qubits. The results are found to be
in excellent agreement with the quantum-mechanical predictions.Comment: REVTeX 4, 5pp., 7 EPS figure files. N.B.: "Alec" is my first, and
"Maassen van den Brink" my family name. v2: final published version, with
changed title, different sample micrograph, and several clarification
Optical conductivity in doped manganites with planar x-y orbital order
We investigate a planar model for the ferromagnetic (FM) phase of manganites,
which develops orbital order of electrons with x-y-symmetry at
low temperature. The dynamic structure factor of orbital excitations and the
optical conductivity are studied with help of a
finite-temperature diagonalization method. Our calculations provide a
theoretical prediction for for the 2D FM state and are of
possible relevance for the recently found A-type phase of manganites at high
doping which consists of FM layers coupled antiferromagnetically. In the
x-y ordered regime shows both a Drude peak and a
gapped incoherent absorption due to a gap in the orbital excitations.Comment: 5 pages, 5 figures, to appear in Phys. Rev. Let
Orbital dynamics in ferromagnetic transition metal oxides
We consider a model of strongly correlated electrons interacting by
superexchange orbital interactions in the ferromagnetic phase of LaMnO. It
is found that the classical orbital order with alternating occupied
orbitals has a full rotational symmetry at orbital degeneracy, and the
excitation spectrum derived using the linear spin-wave theory is gapless. The
quantum (fluctuation) corrections to the order parameter and to the ground
state energy restore the cubic symmetry of the model. By applying a uniaxial
pressure orbital degeneracy is lifted in a tetragonal field and one finds an
orbital-flop phase with a gap in the excitation spectrum. In two dimensions the
classical order is more robust near the orbital degeneracy point and quantum
effects are suppressed. The orbital excitation spectra obtained using finite
temperature diagonalization of two-dimensional clusters consist of a
quasiparticle accompanied by satellite structures. The orbital waves found
within the linear spin-wave theory provide an excellent description of the
dominant pole of these spectra.Comment: 13 pages, 12 figures, to appear in Phys. Rev.
Manganites at Quarter Filling: Role of Jahn-Teller Interactions
We have analyzed different correlation functions in a realistic spin-orbital
model for half-doped manganites. Using a finite-temperature diagonalization
technique the CE phase was found in the charge-ordered phase in the case of
small antiferromagnetic interactions between electrons. It is shown
that a key ingredient responsible for stabilization of the CE-type spin and
orbital-ordered state is the cooperative Jahn-Teller (JT) interaction between
next-nearest Mn neighbors mediated by the breathing mode distortion of
Mn octahedra and displacements of Mn ions. The topological phase
factor in the Mn-Mn hopping leading to gap formation in one-dimensional models
for the CE phase as well as the nearest neighbor JT coupling are not able to
produce the zigzag chains typical for the CE phase in our model.Comment: 16 pages with 16 figures, contains a more detailed parameter estimate
based on the structural data by Radaelli et al. (accepted for publication in
Phys. Rev. B
- …