Thucydides on early Greek history

This chapter studies Thucydides’ account of early Greek history in the “Archaeology” (1.1.2–1.21.2). It shows that Thucydides’ criteria of development and his reconstruction of history are heavily influenced by power relations in Greece during the early stages of the Peloponnesian War. Comparison with other sources for both the legendary and the historical past reveals the extent to which Thucydides, by means of omission, selective emphasis, and skewed interpretation, manipulates traditions that were well known to Athenian audiences, in order to create his distinctive vision of history as reaching a peak of military and economic development and “modernity” in the Greece of his own day. The chapter concludes by exploring the ways in which Thucydides’ influential model of Greek history fails to do justice to the historical realities of archaic Greece

Spin-Dependent Electron Transmission Model for Chiral Molecules in Mesoscopic Devices

Various device-based experiments have indicated that electron transfer in certain chiral molecules may be spin-dependent, a phenomenon known as the Chiral Induced Spin Selectivity (CISS) effect. However, due to the complexity of these devices and a lack of theoretical understanding, it is not always clear to what extent the chiral character of the molecules actually contributes to the magnetic-field-dependent signals in these experiments. To address this issue, we report here an electron transmission model that evaluates the role of the CISS effect in two-terminal and multi-terminal linear-regime electron transport experiments. Our model reveals that for the CISS effect, the chirality-dependent spin transmission is accompanied by a spin-flip electron reflection process. Furthermore, we show that more than two terminals are required in order to probe the CISS effect in the linear regime. In addition, we propose two types of multi-terminal nonlocal transport measurements that can distinguish the CISS effect from other magnetic-field-dependent signals. Our model provides an effective tool to review and design CISS-related transport experiments, and to enlighten the mechanism of the CISS effect itself

Circuit-Model Analysis for Spintronic Devices with Chiral Molecules as Spin Injectors

Recent research discovered that charge transfer processes in chiral molecules can be spin selective and named the effect chiral-induced spin selectivity (CISS). Follow-up work studied hybrid spintronic devices with conventional electronic materials and chiral (bio)molecules. However, a theoretical foundation for the CISS effect is still in development and the spintronic signals were not evaluated quantitatively. We present a circuit-model approach that can provide quantitative evaluations. Our analysis assumes the scheme of a recent experiment that used photosystem~I (PSI) as spin injectors, for which we find that the experimentally observed signals are, under any reasonable assumptions on relevant PSI time scales, too high to be fully due to the CISS effect. We also show that the CISS effect can in principle be detected using the same type of solid-state device, and by replacing silver with graphene, the signals due to spin generation can be enlarged four orders of magnitude. Our approach thus provides a generic framework for analyzing this type of experiments and advancing the understanding of the CISS effect

Injection of Ballistic Hot Electrons and Cool Holes in a Two-Dimensional Electron Gas

We have constructed a novel magnetic spectrometer to study the dynamics of hot electrons and cool missing electron states injected by quantum point contacts in the two-dimensional electron gas of a GaAs-AlxGa1-xAs heterostructure. The mean free path of these quasi-particles is found to be longer than recent theoretical estimates. The injection energy of the particles is found to be anomalously low as the point contact approaches pinch-off, and also for high bias voltages.

Unified description of bulk and interface-enhanced spin pumping

The dynamics of non-equilibrium spin accumulation generated in metals or semiconductors by rf magnetic field pumping is treated within a diffusive picture. The dc spin accumulation produced in a uniform system by a rotating applied magnetic field or by a precessing magnetization of a weak ferromagnet is in general given by a (small) fraction of hbar omega, where omega is the rotation or precession frequency. With the addition of a neighboring, field-free region and allowing for the diffusion of spins, the spin accumulation is dramatically enhanced at the interface, saturating at the universal value hbar omega in the limit of long spin relaxation time. This effect can be maximized when the system dimensions are of the order of sqrt(2pi D omega), where D is the diffusion constant. We compare our results to the interface spin pumping theory of A. Brataas et al. [Phys. Rev. B 66, 060404(R) (2002)]

Bistable hysteresis and resistance switching in hydrogen gold junctions

Current-voltage characteristics of H2-Au molecular junctions exhibit intriguing steps around a characteristic voltage of 40 mV. Surprisingly, we find that a hysteresis is connected to these steps with a typical time scale > 10 ms. This time constant scales linearly with the power dissipated in the junction beyond an ofset power P_s = IV_s. We propose that the hysteresis is related to vibrational heating of both the molecule in the junction and a set of surrounding hydrogen molecules. Remarkably, we can engineer our junctions such that the hysteresis' characteristic time becomes >days. We demonstrate that reliable switchable devices can be built from such junctions.Comment: Submitted to Phys. Rev. Let