9,279 research outputs found

    Lamellar phase separation and dynamic competition in La0.23Ca0.77MnO3

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    We report the coexistence of lamellar charge-ordered (CO) and charge-disordered (CD) domains, and their dynamical behavior, in La0.23Ca0.77MnO3. Using high resolution transmission electron microscopy (TEM), we show that below Tcd~170K a CD-monoclinic phase forms within the established CO-orthorhombic matrix. The CD phase has a sheet-like morphology, perpendicular to the q vector of the CO superlattice (a axis of the Pnma structure). For temperatures between 64K and 130K, both the TEM and resistivity experiments show a dynamic competition between the two phases: at constant T, the CD phase slowly advances over the CO one. This slow dynamics appears to be linked to the magnetic transitions occurring in this compound, suggesting important magnetoelastic effects.Comment: 4 pages, 4 figure

    Correlation effects in the ground state charge density of Mott-insulating NiO: a comparison of ab-initio calculations and high-energy electron diffraction measurements

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    Accurate high-energy electron diffraction measurements of structure factors of NiO have been carried out to investigate how strong correlations in the Ni 3d shell affect electron charge density in the interior area of nickel ions and whether the new ab-initio approaches to the electronic structure of strongly correlated metal oxides are in accord with experimental observations. The generalized gradient approximation (GGA) and the local spin density approximation corrected by the Hubbard U term (LSDA+U) are found to provide the closest match to experimental measurements. The comparison of calculated and observed electron charge densities shows that correlations in the Ni 3d shell suppress covalent bonding between the oxygen and nickel sublattices.Comment: 6 pages, LaTeX and 5 figures in the postscript forma

    Induced Growth of Asymmetric Nanocantilever Arrays on Polar Surfaces

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    ©2003 The American Physical Society. The electronic version of this article is the complete one and can be found online at: http://link.aps.org/doi/10.1103/PhysRevLett.91.185502DOI: 10.1103/PhysRevLett.91.185502We report that the Zn-terminated ZnO (0001) polar surface is chemically active and the oxygenterminated (0001) polar surface is inert in the growth of nanocantilever arrays. Longer and wider "comblike" nanocantilever arrays are grown from the (0001)-Zn surface, which is suggested to be a self-catalyzed process due to the enrichment of Zn at the growth front. The chemically inactive (0001)-O surface typically does not initiate any growth, but controlling experimental conditions could lead to the growth of shorter and narrower nanocantilevers from the intersections between (0001)-O with (0110) surfaces

    Su(3) Algebraic Structure of the Cuprate Superconductors Model based on the Analogy with Atomic Nuclei

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    A cuprate superconductor model based on the analogy with atomic nuclei was shown by Iachello to have an su(3)su(3) structure. The mean-field approximation Hamiltonian can be written as a linear function of the generators of su(3)su(3) algebra. Using algebraic method, we derive the eigenvalues of the reduced Hamiltonian beyond the subalgebras u(1)⨂u(2)u(1)\bigotimes u(2) and so(3)so(3) of su(3)su(3) algebra. In particular, by considering the coherence between s- and d-wave pairs as perturbation, the effects of coherent term upon the energy spectrum are investigated

    Electron release of rare gas atom clusters under an intense laser pulse

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    Calculating the energy absorption of atomic clusters as a function of the laser pulse length TT we find a maximum for a critical T∗T^*. We show that T∗T^* can be linked to an optimal cluster radius R∗R^*. The existence of this radius can be attributed to the enhanced ionization mechanism originally discovered for diatomic molecules. Our findings indicate that enhanced ionization should be operative for a wide class of rare gas clusters. From a simple Coulomb explosion ansatz, we derive an analytical expression relating the maximum energy release to a suitably scaled expansion time which can be expressed with the pulse length T∗T^*.Comment: 4 pages, 5 figure
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