1,133 research outputs found
Phonon-mediated electron spin phase diffusion in a quantum dot
An effective spin relaxation mechanism that leads to electron spin
decoherence in a quantum dot is proposed. In contrast to the common
calculations of spin-flip transitions between the Kramers doublets, we take
into account a process of phonon-mediated fluctuation in the electron spin
precession and subsequent spin phase diffusion. Specifically, we consider
modulations in the longitudinal g-factor and hyperfine interaction induced by
the phonon-assisted transitions between the lowest electronic states. Prominent
differences in the temperature and magnetic field dependence between the
proposed mechanisms and the spin-flip transitions are expected to facilitate
its experimental verification. Numerical estimation demonstrates highly
efficient spin relaxation in typical semiconductor quantum dots.Comment: 5 pages, 1 figur
Hydrodynamic Modes in a Trapped Strongly Interacting Fermi Gases of Atoms
The zero-temperature properties of a dilute two-component Fermi gas in the
BCS-BEC crossover are investigated. On the basis of a generalization of the
variational Schwinger method, we construct approximate semi-analytical formulae
for collective frequencies of the radial and the axial breathing modes of the
Fermi gas under harmonic confinement in the framework of the hydrodynamic
theory. It is shown that the method gives nearly exact solutions.Comment: 11 page
The law of action and reaction for the effective force in a nonequilibrium colloidal system
We study a nonequilibrium Langevin many-body system containing two 'test'
particles and many 'background' particles. The test particles are spatially
confined by a harmonic potential, and the background particles are driven by an
external driving force. Employing numerical simulations of the model, we
formulate an effective description of the two test particles in a
nonequilibrium steady state. In particular, we investigate several different
definitions of the effective force acting between the test particles. We find
that the law of action and reaction does not hold for the total mechanical
force exerted by the background particles, but that it does hold for the
thermodynamic force defined operationally on the basis of an idea used to
extend the first law of thermodynamics to nonequilibrium steady states.Comment: 13 page
Activated Ion Electron Capture Dissociation (AI ECD) of proteins: synchronization of infrared and electron irradiation with ion magnetron motion.
Here, we show that to perform activated ion electron capture dissociation (AI-ECD) in a Fourier transform ion cyclotron resonance (FT-ICR) mass spectrometer equipped with a CO(2) laser, it is necessary to synchronize both infrared irradiation and electron capture dissociation with ion magnetron motion. This requirement is essential for instruments in which the infrared laser is angled off-axis, such as the Thermo Finnigan LTQ FT. Generally, the electron irradiation time required for proteins is much shorter (ms) than that required for peptides (tens of ms), and the modulation of ECD, AI ECD, and infrared multiphoton dissociation (IRMPD) with ion magnetron motion is more pronounced. We have optimized AI ECD for ubiquitin, cytochrome c, and myoglobin; however the results can be extended to other proteins. We demonstrate that pre-ECD and post-ECD activation are physically different and display different kinetics. We also demonstrate how, by use of appropriate AI ECD time sequences and normalization, the kinetics of protein gas-phase refolding can be deconvoluted from the diffusion of the ion cloud and measured on the time scale longer than the period of ion magnetron motion
Transport Phenomena in Complex Systems (part 1)
The issue, in two parts, is devoted to theoretical, computational and experimental studies of transport phenomena in various complex systems (in porous and composite media; systems with physical and chemical reactions and phase and structural transformations; in biological tissues and materials). Various types of these phenomena (heat and mass transfer; hydrodynamic and rheological effects; electromagnetic field propagation) are considered. Anomalous, relaxation and nonlinear transport, as well as transport induced by the impact of external fields and noise, is the focus of this issue. Modern methods of computational modelling, statistical physics and hydrodynamics, nonlinear dynamics and experimental methods are presented and discussed. Special attention is paid to transport phenomena in biological systems (such as haemodynamics in stenosed and thrombosed blood vessels magneto-induced heat generation and propagation in biological tissues, and anomalous transport in living cells) and to the development of a scientific background for progressive methods in cancer, heart attack and insult therapy (magnetic hyperthermia for cancer therapy, magnetically induced circulation flow in thrombosed blood vessels and non-contact determination of the local rate of blood flow in coronary arteries). The present issue includes works on the phenomenological study of transport processes, the derivation of a macroscopic governing equation on the basis of the analysis of a complicated internal reaction and the microscopic determination of macroscopic characteristics of the studied systems. This article is part of the theme issue 'Transport phenomena in complex systems (part 1)'. © 2021 The Author(s).Data accessibility. This article has no additional data. Authors’ contributions. All authors contributed equally to the present paper. Competing interests. We declare we have no competing interests. Funding. This work was supported by the Russian Science Foundation (project no. 18-19-00008)
Transport phenomena and phase transitions in soft and disordered systems
The present special issue is devoted to the experimental, theoretical and computational studies of fundamental features in transport phenomena, structural and phase transitions in various soft and disordered systems (polymers, colloids, glasses, amorphous, crystalline, and composite materials) involved in macroscopically non-equilibrium processes (hydrodynamic flows; non-stationary deformations, heat and mass transfer and so on). Special attention is focused on a detailed microscopical study of the effects of internal structural and phase transformations on macroscopic physical properties and phenomena in the systems under study. © 2022, The Author(s), under exclusive licence to EDP Sciences, Springer-Verlag GmbH Germany, part of Springer Nature.Russian Science Foundation, RSF: 20-61-46013This work was supported by the Russian Science Foundation (Grant number 20-61-46013)
Transport Phenomena in Complex Systems (part 2)
This theme issue, in two parts, continues research studies of transport phenomena in complex media published in the first part (Alexandrov & Zubarev 2021 Phil. Trans. R. Soc. A 379, 20200301. (doi:10.1098/rsta.2020.0301)). The issue is concerned with theoretical, numerical and experimental investigations of nonlinear transport phenomena in heterogeneous and metastable materials of different nature, including biological systems. The papers are devoted to the new effects arising in such systems (e.g. pattern and microstructure formation in materials, impacts of external processes on their properties and evolution and so on). State-of-the-art methods of numerical simulations, stochastic analysis, nonlinear physics and experimental studies are presented in the collection of issue papers. This article is part of the theme issue 'Transport phenomena in complex systems (part 2)'. © 2022 The Authors.This work was supported by the Russian Science Foundation (project no. 18-19-00008)
Universal Properties of Nonlinear Response Functions of Nonequilibrium Steady States
We derive universal properties of nonlinear response functions of
nonequilibrium steady states. In particular, sum rules and asymptotic behaviors
are derived. Their consequences are illustrated for nonlinear optical materials
and nonlinear electrical conductors.Comment: 10 pages, 1 figure; added a few sentences and references to explain
detail
Nonequilibrium mesoscopic transport: a genealogy
Models of nonequilibrium quantum transport underpin all modern electronic
devices, from the largest scales to the smallest. Past simplifications such as
coarse graining and bulk self-averaging served well to understand electronic
materials. Such particular notions become inapplicable at mesoscopic
dimensions, edging towards the truly quantum regime. Nevertheless a unifying
thread continues to run through transport physics, animating the design of
small-scale electronic technology: microscopic conservation and nonequilibrium
dissipation. These fundamentals are inherent in quantum transport and gain even
greater and more explicit experimental meaning in the passage to atomic-sized
devices. We review their genesis, their theoretical context, and their
governing role in the electronic response of meso- and nanoscopic systems.Comment: 21p
Generalized kinetic and evolution equations in the approach of the nonequilibrium statistical operator
The method of the nonequilibrium statistical operator developed by D. N.
Zubarev is employed to analyse and derive generalized transport and kinetic
equations. The degrees of freedom in solids can often be represented as a few
interacting subsystems (electrons, spins, phonons, nuclear spins, etc.).
Perturbation of one subsystem may produce a nonequilibrium state which is then
relaxed to an equilibrium state due to the interaction between particles or
with a thermal bath. The generalized kinetic equations were derived for a
system weakly coupled to a thermal bath to elucidate the nature of transport
and relaxation processes. It was shown that the "collision term" had the same
functional form as for the generalized kinetic equations for the system with
small interactions among particles. The applicability of the general formalism
to physically relevant situations is investigated. It is shown that some known
generalized kinetic equations (e.g. kinetic equation for magnons, Peierls
equation for phonons) naturally emerges within the NSO formalism. The
relaxation of a small dynamic subsystem in contact with a thermal bath is
considered on the basis of the derived equations. The Schrodinger-type equation
for the average amplitude describing the energy shift and damping of a particle
in a thermal bath and the coupled kinetic equation describing the dynamic and
statistical aspects of the motion are derived and analysed. The equations
derived can help in the understanding of the origin of irreversible behavior in
quantum phenomena.Comment: 21 pages, Revte
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