821 research outputs found
Deflection of field-free aligned molecules
We consider deflection of polarizable molecules by inhomogeneous optical
fields, and analyze the role of molecular orientation and rotation in the
scattering process. It is shown that molecular rotation induces spectacular
rainbow-like features in the distribution of the scattering angle. Moreover, by
pre-shaping molecular angular distribution with the help of short and strong
femtosecond laser pulses, one may efficiently control the scattering process,
manipulate the average deflection angle and its distribution, and reduce
substantially the angular dispersion of the deflected molecules. This opens new
ways for many applications involving molecular focusing, guiding and trapping
by optical and static fields.Comment: 4 pages, 4 figure
Radiative orbital electron capture by the atomic nucleus
The rate for the photon emission accompanying orbital 1S electron capture by
the atomic nucleus is recalculated. While a photon can be emitted by the
electron or by the nucleus, the use of the length gauge significantly
suppresses the nuclear contribution. Our calculations resolve the long standing
discrepancy of theoretical predictions with experimental data for
forbidden transitions. We illustrate the results by comparison with the data
established experimentally for the first forbidden unique decays of Ca
and Tl.Comment: 18 pages, 2 figures, submitted to Phys. Rev.
Optimal molecular alignment and orientation through rotational ladder climbing
We study the control by electromagnetic fields of molecular alignment and
orientation, in a linear, rigid rotor model. With the help of a monotonically
convergent algorithm, we find that the optimal field is in the microwave part
of the spectrum and acts by resonantly exciting the rotation of the molecule
progressively from the ground state, i.e., by rotational ladder climbing. This
mechanism is present not only when maximizing orientation or alignment, but
also when using prescribed target states that simultaneously optimize the
efficiency of orientation/alignment and its duration. The extension of the
optimization method to consider a finite rotational temperature is also
presented.Comment: 14 pages, 12 figure
Radiative electron capture in the first forbidden unique decay of 81Kr
The photon spectrum accompanying the orbital K-electron capture in the first
forbidden unique decay of 81Kr was measured. The total radiation intensity for
the photon energies larger than 50 keV was found to be 1.47(6) x 10^{-4} per
K-capture. Both the shape of the spectrum and its intensity relative to the
ordinary, non-radiative capture rate, are compared to theoretical predictions.
The best agreement is found for the recently developed model which employs the
length gauge for the electromagnetic field.Comment: 7 pages, 6 figure
Controlling Molecular Scattering by Laser-Induced Field-Free Alignment
We consider deflection of polarizable molecules by inhomogeneous optical
fields, and analyze the role of molecular orientation and rotation in the
scattering process. It is shown that molecular rotation induces spectacular
rainbow-like features in the distribution of the scattering angle. Moreover, by
preshaping molecular angular distribution with the help of short and strong
femtosecond laser pulses, one may efficiently control the scattering process,
manipulate the average deflection angle and its distribution, and reduce
substantially the angular dispersion of the deflected molecules. We provide
quantum and classical treatment of the deflection process. The effects of
strong deflecting field on the scattering of rotating molecules are considered
by the means of the adiabatic invariants formalism. This new control scheme
opens new ways for many applications involving molecular focusing, guiding and
trapping by optical and static fields
Laser-induced nuclear excitation
An analysis is presented of the Coulomb excitation of low lying nuclear levels by the electrons produced by strong field ionization of atoms. It is shown that the resulting short lived radioactivity can be as high as on the order of 10³Ci for certain isotopes excited by using modern laser systems. Relativistic effects are demonstrated that substantially increase radioactivity as compared tothat predicted by nonrelativistic theory resultsyesBelgorod State Universit
Stern-Gerlach deflection of field-free aligned paramagnetic molecules
The effects of laser-induced prealignment on the deflection of paramagnetic
molecules by inhomogeneous static magnetic field are studied. Depending on the
relevant Hund's coupling case of the molecule, two different effects were
identified: either suppression of the deflection by laser pulses (Hund's
coupling case (a) molecules, such as ClO), or a dramatic reconstruction of the
broad distribution of the scattering angles into several narrow peaks (for
Hund's coupling case (b) molecules, such as O2 or NH). These findings are
important for various applications using molecular guiding, focusing and
trapping with the help of magnetic fields
Self-Energy Correction to the Two-Photon Decay Width in Hydrogenlike Atoms
We investigate the gauge invariance of the leading logarithmic radiative
correction to the two-photon decay width in hydrogenlike atoms. It is shown
that an effective treatment of the correction using a Lamb-shift "potential"
leads to equivalent results in both the length as well as the velocity gauges
provided all relevant correction terms are taken into account. Specifically,
the relevant radiative corrections are related to the energies that enter into
the propagator denominators, to the Hamiltonian, to the wave functions, and to
the energy conservation condition that holds between the two photons; the form
of all of these effects is different in the two gauges, but the final result is
shown to be gauge invariant, as it should be. Although the actual calculation
only involves integrations over nonrelativistic hydrogenic Green functions, the
derivation of the leading logarithmic correction can be regarded as slightly
more complex than that of other typical logarithmic terms. The dominant
radiative correction to the 2S two-photon decay width is found to be -2.020536
(alpha/pi) (Zalpha)^2 ln[(Zalpha)^-2] in units of the leading nonrelativistic
expression. This result is in agreement with a length-gauge calculation [S. G.
Karshenboim and V. G. Ivanov, e-print physics/9702027], where the coefficient
was given as -2.025(1).Comment: 9 pages, RevTe
Electric Deflection of Rotating Molecules
We provide a theory of the deflection of polar and non-polar rotating
molecules by inhomogeneous static electric field. Rainbow-like features in the
angular distribution of the scattered molecules are analyzed in detail.
Furthermore, we demonstrate that one may efficiently control the deflection
process with the help of short and strong femtosecond laser pulses. In
particular the deflection process may by turned-off by a proper excitation, and
the angular dispersion of the deflected molecules can be substantially reduced.
We study the problem both classically and quantum mechanically, taking into
account the effects of strong deflecting field on the molecular rotations. In
both treatments we arrive at the same conclusions. The suggested control scheme
paves the way for many applications involving molecular focusing, guiding, and
trapping by inhomogeneous fields
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