High efficiency dark-to-bright exciton conversion in carbon nanotubes

We report that dark excitons can have a large contribution to the emission intensity in carbon nanotubes due to an efficient exciton conversion from a dark state to a bright state. Time-resolved photoluminescence measurements are used to investigate decay dynamics and diffusion properties of excitons, and we obtain intrinsic lifetimes and diffusion lengths of bright excitons as well as diffusion coefficients for both bright and dark excitons. We find that the dark-to-bright transition rates can be considerably high, and that more than half of the dark excitons can be transformed into the bright excitons. The state transition rates have a large chirality dependence with a family pattern, and the conversion efficiency is found to be significantly enhanced by adsorbed air molecules on the surface of the nanotubes. Our findings show the nontrivial significance of the dark excitons on the emission kinetics in low dimensional materials, and demonstrate the potential for engineering the dark-to-bright conversion process by using surface interactions.Comment: 7 pages, 4 figure

Single carbon nanotubes as ultrasmall all-optical memories

Performance improvements are expected from integration of photonic devices into information processing systems, and in particular, all-optical memories provide a key functionality. Scaling down the size of memory elements is desirable for high-density integration, and the use of nanomaterials would allow for devices that are significantly smaller than the operation wavelengths. Here we report on all-optical memory based on individual carbon nanotubes, where adsorbed molecules give rise to optical bistability. By exciting at the high-energy tail of the excitonic absorption resonance, nanotubes can be switched between the desorbed state and the adsorbed state. We demonstrate reversible and reproducible operation of the nanotube optical memory, and determine the rewriting speed by measuring the molecular adsorption and desorption times. Our results underscore the impact of molecular-scale effects on optical properties of nanomaterials, offering new design strategies for photonic devices that are a few orders of magnitude smaller than the optical diffraction limit.Comment: 8 pages, 6 figure

QED Radiative Corrections to the Non-annihilation Processes Using the Structure Function and the Parton Shower

Inclusion of the QED higher order radiative corrections in the two-photon process, e+e- -> e+e- mu+mu-, is examined by means of the structure function and the parton shower. Results are compared with the exact $O(\alpha)$ calculations and give a good agreement. These two methods should be universally applicable to any other non-annihilation processes like the single-W productions in the e+e- collisions. In this case, however, the energy scale for the evolution by the renormalization-group equation should be chosen properly depending on the dominant diagrams for the given process. A method to find the most suitable energy scale is proposed.Comment: 17 pages, LaTeX, 5 figure

Stark effect of excitons in individual air-suspended carbon nanotubes

We investigate electric-field induced redshifts of photoluminescence from individual single-walled carbon nanotubes. The shifts scale quadratically with field, while measurements with different excitation powers and energies show that effects from heating and relaxation pathways are small. We attribute the shifts to the Stark effect, and characterize nanotubes with different chiralities. By taking into account exciton binding energies for air-suspended tubes, we find that theoretical predictions are in quantitative agreement.Comment: 4 pages, 3 figure

QED Radiative Correction for the Single-W Production using a Parton Shower Method

A parton shower method for the photonic radiative correction is applied to the single W-boson production processes. The energy scale for the evolution of the parton shower is determined so that the correct soft-photon emission is reproduced. Photon spectra radiated from the partons are compared with those from the exact matrix elements, and show a good agreement. Possible errors due to a inappropriate energy-scale selection or due to the ambiguity of energy scale determination are also discussed, particularly for the measurements on triple gauge-couplings.Comment: 17 pages, 6 Postscript figure