1,246 research outputs found
On the morphology of ammonium nitrate (III): theory and observation
The aim of this paper is to derive on a theoretical basis the morphology of crystals of ammonium nitrate, phase III, and to compare the results with experimental growth forms. The theory used is based on the concepts of periodic bond chain (PBC), F face and connected net, developed by Hartman and Perdok. Further an Ising model is used to determine roughening temperatures. Based on different criteria theoretical growth forms are predicted and compared with experiments
A simple model for magnetism in itinerant electron systems
A new lattice model of interacting electrons is presented. It can be viewed
as a classical Hubbard model in which the energy associated to electron
itinerance is proportional to the total number of possible electron jumps.
Symmetry properties of the Hubbard model are preserved. In the half-filled band
with strong interaction the model becomes the Ising model. The main features of
the magnetic behavior of the model in the one-dimensional and mean-field cases
are studied.Comment: 9 pages, 3 figures, to be published in Physica
Interfaces with a single growth inhomogeneity and anchored boundaries
The dynamics of a one dimensional growth model involving attachment and
detachment of particles is studied in the presence of a localized growth
inhomogeneity along with anchored boundary conditions. At large times, the
latter enforce an equilibrium stationary regime which allows for an exact
calculation of roughening exponents. The stochastic evolution is related to a
spin Hamiltonian whose spectrum gap embodies the dynamic scaling exponent of
late stages. For vanishing gaps the interface can exhibit a slow morphological
transition followed by a change of scaling regimes which are studied
numerically. Instead, a faceting dynamics arises for gapful situations.Comment: REVTeX, 11 pages, 9 Postscript figure
Frequency-dependent magnetotransport and particle dynamics in magnetic modulation systems
We analyze the dynamics of a charged particle moving in the presence of
spatially-modulated magnetic fields. From Poincare surfaces of section and
Liapunov exponents for characteristic trajectories we find that the fraction of
pinned and runaway quasiperiodic orbits {\em vs}. chaotic orbits depends
strongly on the ratio of cyclotron radius to the structure parameters, as well
as on the amplitude of the modulated field. We present a complete
characterization of the dynamical behavior of such structures, and investigate
the contribution to the magnetoconductivity from all different orbits using a
classical Kubo formula. Although the DC conductivity of the system depends
strongly on the pinned and runaway trajectories, the frequency response
reflects the topology of all different orbits, and even their unusual temporal
behavior.Comment: Submitted to PRB - 14 figure files - REVTEX tex
Kinetics and Jamming Coverage in a Random Sequential Adsorption of Polymer Chains
Using a highly efficient Monte Carlo algorithm, we are able to study the
growth of coverage in a random sequential adsorption (RSA) of self-avoiding
walk (SAW) chains for up to 10^{12} time steps on a square lattice. For the
first time, the true jamming coverage (theta_J) is found to decay with the
chain length (N) with a power-law theta_J propto N^{-0.1}. The growth of the
coverage to its jamming limit can be described by a power-law, theta(t) approx
theta_J -c/t^y with an effective exponent y which depends on the chain length,
i.e., y = 0.50 for N=4 to y = 0.07 for N=30 with y -> 0 in the asymptotic limit
N -> infinity.Comment: RevTeX, 5 pages inclduing figure
Tight-binding g-Factor Calculations of CdSe Nanostructures
The Lande g-factors for CdSe quantum dots and rods are investigated within
the framework of the semiempirical tight-binding method. We describe methods
for treating both the n-doped and neutral nanostructures, and then apply these
to a selection of nanocrystals of variable size and shape, focusing on
approximately spherical dots and rods of differing aspect ratio. For the
negatively charged n-doped systems, we observe that the g-factors for
near-spherical CdSe dots are approximately independent of size, but show strong
shape dependence as one axis of the quantum dot is extended to form rod-like
structures. In particular, there is a discontinuity in the magnitude of
g-factor and a transition from anisotropic to isotropic g-factor tensor at
aspect ratio ~1.3. For the neutral systems, we analyze the electron g-factor of
both the conduction and valence band electrons. We find that the behavior of
the electron g-factor in the neutral nanocrystals is generally similar to that
in the n-doped case, showing the same strong shape dependence and discontinuity
in magnitude and anisotropy. In smaller systems the g-factor value is dependent
on the details of the surface model. Comparison with recent measurements of
g-factors for CdSe nanocrystals suggests that the shape dependent transition
may be responsible for the observations of anomalous numbers of g-factors at
certain nanocrystal sizes.Comment: 15 pages, 6 figures. Fixed typos to match published versio
Rheological Chaos in a Scalar Shear-Thickening Model
We study a simple scalar constitutive equation for a shear-thickening
material at zero Reynolds number, in which the shear stress \sigma is driven at
a constant shear rate \dot\gamma and relaxes by two parallel decay processes: a
nonlinear decay at a nonmonotonic rate R(\sigma_1) and a linear decay at rate
\lambda\sigma_2. Here \sigma_{1,2}(t) =
\tau_{1,2}^{-1}\int_0^t\sigma(t')\exp[-(t-t')/\tau_{1,2}] {\rm d}t' are two
retarded stresses. For suitable parameters, the steady state flow curve is
monotonic but unstable; this arises when \tau_2>\tau_1 and
0>R'(\sigma)>-\lambda so that monotonicity is restored only through the
strongly retarded term (which might model a slow evolution of material
structure under stress). Within the unstable region we find a period-doubling
sequence leading to chaos. Instability, but not chaos, persists even for the
case \tau_1\to 0. A similar generic mechanism might also arise in shear
thinning systems and in some banded flows.Comment: Reference added; typos corrected. To appear in PRE Rap. Com
ERK1 as a therapeutic target for dendritic cell vaccination against high-grade gliomas
Glioma regression requires the recruitment of potent anti-tumor immune cells into the tumor microenvironment. Dendritic cells (DCs) play a role in immune responses to these tumors. The fact that DC vaccines do not effectively combat high-grade gliomas, however, suggests that DCs need to be genetically modified especially to promote their migration to tumor relevant sites. Previously, we identified extracellular signal-regulated kinase (ERK1) as a regulator of DC immunogenicity and brain autoimmunity. In the present study, we made use of modern magnetic resonance methods to study the role of ERK1 in regulating DC migration and tumor progression in a model of high-grade glioma. We found that ERK1-deficient mice are more resistant to the development of gliomas, and tumor growth in these mice is accompanied by a higher infiltration of leukocytes. ERK1-deficient DCs exhibit an increase in migration that is associated with sustained Cdc42 activation and increased expression of actin-associated cytoskeleton-organizing proteins. We also demonstrated that ERK1 deletion potentiates DC vaccination and provides a survival advantage in high-grade gliomas. Considering the therapeutic significance of these results, we propose ERK1-deleted DC vaccines as an additional means of eradicating resilient tumor cells and preventing tumor recurrence
Unconventional MBE Strategies from Computer Simulations for Optimized Growth Conditions
We investigate the influence of step edge diffusion (SED) and desorption on
Molecular Beam Epitaxy (MBE) using kinetic Monte-Carlo simulations of the
solid-on-solid (SOS) model. Based on these investigations we propose two
strategies to optimize MBE growth. The strategies are applicable in different
growth regimes: During layer-by-layer growth one can exploit the presence of
desorption in order to achieve smooth surfaces. By additional short high flux
pulses of particles one can increase the growth rate and assist layer-by-layer
growth. If, however, mounds are formed (non-layer-by-layer growth) the SED can
be used to control size and shape of the three-dimensional structures. By
controlled reduction of the flux with time we achieve a fast coarsening
together with smooth step edges.Comment: 19 pages, 7 figures, submitted to Phys. Rev.
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