15 research outputs found
Creation of Rydberg Polarons in a Bose Gas
We report spectroscopic observation of Rydberg polarons in an atomic Bose
gas. Polarons are created by excitation of Rydberg atoms as impurities in a
strontium Bose-Einstein condensate. They are distinguished from previously
studied polarons by macroscopic occupation of bound molecular states that arise
from scattering of the weakly bound Rydberg electron from ground-state atoms.
The absence of a -wave resonance in the low-energy electron-atom scattering
in Sr introduces a universal behavior in the Rydberg spectral lineshape and in
scaling of the spectral width (narrowing) with the Rydberg principal quantum
number, . Spectral features are described with a functional determinant
approach (FDA) that solves an extended Fr\"{o}hlich Hamiltonian for a mobile
impurity in a Bose gas. Excited states of polyatomic Rydberg molecules
(trimers, tetrameters, and pentamers) are experimentally resolved and
accurately reproduced with FDA.Comment: 5 pages, 3 figure
Theory of excitation of Rydberg polarons in an atomic quantum gas
We present a quantum many-body description of the excitation spectrum of
Rydberg polarons in a Bose gas. The many-body Hamiltonian is solved with
functional determinant theory, and we extend this technique to describe Rydberg
polarons of finite mass. Mean-field and classical descriptions of the spectrum
are derived as approximations of the many-body theory. The various approaches
are applied to experimental observations of polarons created by excitation of
Rydberg atoms in a strontium Bose-Einstein condensate.Comment: 14 pages, 9 figures. arXiv admin note: substantial text overlap with
arXiv:1706.0371
Structural and Morphological Evolution of Lead Dendrites during Electrochemical Migration
The electrochemical deposition and dissolution of lead on gold electrodes immersed in an aqueous solution of lead nitrate were studied in situ using a biasing liquid cell by transmission electron microscopy (TEM). We investigate in real time the growth mechanisms of lead dendrites as deposited on the electrodes under an applied potential. TEM images reveal that lead dendrites are developed by the fast protrusion of lead branches in the electrolyte and tip splitting. And, the fast growing tip of the dendritic branch is composed of polycrystalline nanograins and it develops into a single crystalline branch eventually. This study demonstrated unique electrochemical growth of single crystal dendrites through nucleation, aggregation, alignment and attachment of randomly oriented small grains. Additionally, we found the lead concentration in the electrolyte drastically influences the morphology of dendritic formation