2,399 research outputs found
Field dependent anisotropy change in a supramolecular Mn(II)-[3x3] grid
The magnetic anisotropy of a novel Mn(II)-[3x3] grid complex was investigated
by means of high-field torque magnetometry. Torque vs. field curves at low
temperatures demonstrate a ground state with S > 0 and exhibit a torque step
due to a field induced level-crossing at B* \approx 7.5 T, accompanied by an
abrupt change of magnetic anisotropy from easy-axis to hard-axis type. These
observations are discussed in terms of a spin Hamiltonian formalism.Comment: 4 pages, 4 figures, to be published in Phys. Rev. Let
Approximating parabolas as natural bounds of Heisenberg spectra: Reply on the comment of O. Waldmann
O. Waldmann has shown that some spin systems, which fulfill the condition of
a weakly homogeneous coupling matrix, have a spectrum whose minimal or maximal
energies are rather poorly approximated by a quadratic dependence on the total
spin quantum number. We comment on this observation and provide the new
argument that, under certain conditions, the approximating parabolas appear as
natural bounds of the spectrum generated by spin coherent states.Comment: 2 pages, accepted for Europhysics Letter
Low temperature magnetization and the excitation spectrum of antiferromagnetic Heisenberg spin rings
Accurate results are obtained for the low temperature magnetization versus
magnetic field of Heisenberg spin rings consisting of an even number N of
intrinsic spins s = 1/2, 1, 3/2, 2, 5/2, 3, 7/2 with nearest-neighbor
antiferromagnetic (AF) exchange by employing a numerically exact quantum Monte
Carlo method. A straightforward analysis of this data, in particular the values
of the level-crossing fields, provides accurate results for the lowest energy
eigenvalue E(N,S,s) for each value of the total spin quantum number S. In
particular, the results are substantially more accurate than those provided by
the rotational band approximation. For s <= 5/2, data are presented for all
even N <= 20, which are particularly relevant for experiments on finite
magnetic rings. Furthermore, we find that for s > 1 the dependence of E(N,S,s)
on s can be described by a scaling relation, and this relation is shown to hold
well for ring sizes up to N = 80 for all intrinsic spins in the range 3/2 <= s
<= 7/2. Considering ring sizes in the interval 8 <= N <= 50, we find that the
energy gap between the ground state and the first excited state approaches zero
proportional to 1/N^a, where a = 0.76 for s = 3/2 and a = 0.84 for s = 5/2.
Finally, we demonstrate the usefulness of our present results for E(N,S,s) by
examining the Fe12 ring-type magnetic molecule, leading to a new, more accurate
estimate of the exchange constant for this system than has been obtained
heretofore.Comment: Submitted to Physical Review B, 10 pages, 10 figure
The Little Fishermaiden : Waltz
https://digitalcommons.library.umaine.edu/mmb-ps/1694/thumbnail.jp
Field-induced level crossings in spin clusters: Thermodynamics and magneto-elastic instability
Quantum spin clusters with dominant antiferromagnetic Heisenberg exchange
interactions typically exhibit a sequence of field-induced level crossings in
the ground state as function of magnetic field. For fields near a level
crossing, the cluster can be approximated by a two-level Hamiltonian at low
temperatures. Perturbations, such as magnetic anisotropy or spin-phonon
coupling, sensitively affect the behavior at the level-crossing points. The
general two-level Hamiltonian of the spin system is derived in first-order
perturbation theory, and the thermodynamic functions magnetization, magnetic
torque, and magnetic specific heat are calculated. Then a magneto-elastic
coupling is introduced and the effective two-level Hamilitonian for the
spin-lattice system derived in the adiabatic approximation of the phonons. At
the level crossings the system becomes unconditionally unstable against lattice
distortions due to the effects of magnetic anisotropy. The resultant
magneto-elastic instabilities at the level crossings are discussed, as well as
the magnetic behavior.Comment: 13 pages, 8 figures, REVTEX
Magnetic relaxation studies on a single-molecule magnet by time-resolved inelastic neutron scattering
Time-resolved inelastic neutron scattering measurements on an array of
single-crystals of the single-molecule magnet Mn12ac are presented. The data
facilitate a spectroscopic investigation of the slow relaxation of the
magnetization in this compound in the time domain.Comment: 3 pages, 4 figures, REVTEX4, to appear in Appl. Phys. Lett., for an
animation see also
http://www.dcb.unibe.ch/groups/guedel/members/ow2/trins.ht
Photometric stability analysis of the Exoplanet Characterisation Observatory
Photometric stability is a key requirement for time-resolved spectroscopic
observations of transiting extrasolar planets. In the context of the Exoplanet
Characterisation Observatory (EChO) mission design, we here present and
investigate means of translating spacecraft pointing instabilities as well as
temperature fluctuation of its optical chain into an overall error budget of
the exoplanetary spectrum to be retrieved. Given the instrument specifications
as of date, we investigate the magnitudes of these photometric instabilities in
the context of simulated observations of the exoplanet HD189733b secondary
eclipse.Comment: submitted to MNRA
Quantum Phase Interference and Neel-Vector Tunneling in Antiferromagnetic Molecular Wheels
The antiferromagnetic molecular wheel Fe18 of eighteen exchange-coupled
Fe(III) ions has been studied by measurements of the magnetic torque, the
magnetization, and the inelastic neutron scattering spectra. The combined data
show that the low-temperature magnetism of Fe18 is very accurately described by
the Neel-vector tunneling (NVT) scenario, as unfolded by semiclassical theory.
In addition, the magnetic torque as a function of applied field exhibits
oscillations that reflect the oscillations in the NVT tunnel splitting with
field due to quantum phase interference.Comment: 5 pages, 4 figures, REVTEX4, to appear in PR
ExoSim: the Exoplanet Observation Simulator
A new generation of exoplanet research beckons and with it the need for simulation tools that accurately predict signal and noise in transit spectroscopy observations. We developed ExoSim: an end-to-end simulator that models noise and systematics in a dynamical simulation. ExoSim improves on previous simulators in the complexity of its simulation, versatility of use and its ability to be generically applied to different instruments. It performs a dynamical simulation that can capture temporal effects such as correlated noise and systematics on the light curve. It has also been extensively validated, including against real results from the Hubble WFC3 instrument. We find ExoSim is accurate to within 5% in most comparisons. ExoSim can interact with other models which simulate specific time-dependent processes. A dedicated star spot simulator allows ExoSim to produce simulated observations that include spot and facula contamination. ExoSim has been used extensively in the Phase A and B design studies of the ARIEL mission, and has many potential applications in the field of transit spectroscopy
Detection of an atmosphere around the super-Earth 55 Cancri e
We report the analysis of two new spectroscopic observations of the
super-Earth 55 Cancri e, in the near infrared, obtained with the WFC3 camera
onboard the HST. 55 Cancri e orbits so close to its parent star, that
temperatures much higher than 2000 K are expected on its surface. Given the
brightness of 55 Cancri, the observations were obtained in scanning mode,
adopting a very long scanning length and a very high scanning speed. We use our
specialized pipeline to take into account systematics introduced by these
observational parameters when coupled with the geometrical distortions of the
instrument. We measure the transit depth per wavelength channel with an average
relative uncertainty of 22 ppm per visit and find modulations that depart from
a straight line model with a 6 confidence level. These results suggest
that 55 Cancri e is surrounded by an atmosphere, which is probably
hydrogen-rich. Our fully Bayesian spectral retrieval code, T-REx, has
identified HCN to be the most likely molecular candidate able to explain the
features at 1.42 and 1.54 m. While additional spectroscopic observations
in a broader wavelength range in the infrared will be needed to confirm the HCN
detection, we discuss here the implications of such result. Our chemical model,
developed with combustion specialists, indicates that relatively high mixing
ratios of HCN may be caused by a high C/O ratio. This result suggests this
super-Earth is a carbon-rich environment even more exotic than previously
thought.Comment: 10 pages, 10 figures, 4 tables, Accepted for publication in Ap
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