644 research outputs found
The malleability of uranium: manipulating the charge-density wave in epitaxial films
We report x-ray synchrotron experiments on epitaxial films of uranium,
deposited on niobium and tungsten seed layers. Despite similar lattice
parameters for these refractory metals, the uranium epitaxial arrangements are
different and the strains propagated along the a-axis of the uranium layers are
of opposite sign. At low temperatures these changes in epitaxy result in
dramatic modifications to the behavior of the charge-density wave in uranium.
The differences are explained with the current theory for the electron-phonon
coupling in the uranium lattice. Our results emphasize the intriguing
possibilities of producing epitaxial films of elements that have complex
structures like the light actinides uranium to plutonium.Comment: 6 pages, 6 figure
X-ray fiber diffraction evidence for neighbor exclusion binding of a platinum metallointercalation reagent to DNA.
Profile of the U 5f magnetization in U/Fe multilayers
Recent calculations, concerning the magnetism of uranium in the U/Fe
multilayer system have described the spatial dependence of the 5f polarization
that might be expected. We have used the x-ray resonant magnetic reflectivity
technique to obtain the profile of the induced uranium magnetic moment for
selected U/Fe multilayer samples. This study extends the use of x-ray magnetic
scattering for induced moment systems to the 5f actinide metals. The spatial
dependence of the U magnetization shows that the predominant fraction of the
polarization is present at the interfacial boundaries, decaying rapidly towards
the center of the uranium layer, in good agreement with predictions.Comment: 7 pages, 6 figure
The elevated Curie temperature and half-metallicity in the ferromagnetic semiconductor LaEuO
Here we study the effect of La doping in EuO thin films using SQUID
magnetometry, muon spin rotation (SR), polarized neutron reflectivity
(PNR), and density functional theory (DFT). The SR data shows that the
LaEuO is homogeneously magnetically ordered up to its
elevated . It is concluded that bound magnetic polaron behavior does
not explain the increase in and an RKKY-like interaction is
consistent with the SR data. The estimation of the magnetic moment by DFT
simulations concurs with the results obtained by PNR, showing a reduction of
the magnetic moment per LaEuO for increasing lanthanum doping.
This reduction of the magnetic moment is explained by the reduction of the
number of Eu-4 electrons present in all the magnetic interactions in EuO
films. Finally, we show that an upwards shift of the Fermi energy with La or Gd
doping gives rise to half-metallicity for doping levels as high as 3.2 %.Comment: 7 pages, 11 figure
On thermalization of magnetic nano-arrays at fabrication
We propose a model to predict and control the statistical ensemble of
magnetic degrees of freedom in Artificial Spin Ice (ASI) during thermalized
adiabatic growth. We predict that as-grown arrays are controlled by the
temperature at fabrication and by their lattice constant, and that they can be
described by an effective temperature. If the geometry is conducive to a phase
transition, then the lowest temperature phase is accessed in arrays of lattice
constant smaller than a critical value, which depends on the temperature at
deposition. Alternatively, for arrays of equal lattice constant, there is a
temperature threshold at deposition and the lowest temperature phase is
accessed for fabrication temperatures {\it larger rather than smaller} than
this temperature threshold. Finally we show how to define and control the
effective temperature of the as-grown array and how to measure critical
exponents directly. We discuss the role of kinetics at the critical point, and
applications to experiments, in particular to as-grown thermalized square ASI,
and to magnetic monopole crystallization in as-grown honeycomb ASI.Comment: 14 pages, 2 figures. A theoretical approach to experimental results
reported in: Morgan J P, Stein A, Langridge S and Marrows C (2010) Nature
Physics 7 7
Magnetic coupling in ferromagnetic semiconductor (Ga,Mn)As/(Al,Ga,Mn)As bilayers
We report on a study of ferromagnetic semiconductor (Ga,Mn)As/(Al,Ga,Mn)As bilayers using magnetometry and polarized neutron reflectivity (PNR). From depth-resolved characterization of the magnetic structure obtained by PNR, we concluded that the (Ga,Mn)As and (Al,Ga,Mn)As layers have in-plane and perpendicular-to-plane magnetic easy axes, respectively, with weak interlayer coupling. Therefore, the layer magnetizations align perpendicular to each other under low magnetic fields and parallel at high fields
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