35 research outputs found
Structural and magnetic dynamics of a laser induced phase transition in FeRh
We use time-resolved x-ray diffraction and magnetic optical Kerr effect to
study the laser induced antiferromagnetic to ferromagnetic phase transition in
FeRh. The structural response is given by the nucleation of independent
ferromagnetic domains (\tau_1 ~ 30ps). This is significantly faster than the
magnetic response (\tau_2 ~ 60ps) given by the subsequent domain realignment.
X-ray diffraction shows that the two phases co-exist on short time-scales and
that the phase transition is limited by the speed of sound. A nucleation model
describing both the structural and magnetic dynamics is presented.Comment: 5 pages, 3 figures - changed to reflect version accepted for PR
Ultrafast changes in lattice symmetry probed by coherent phonons
The electronic and structural properties of a material are strongly
determined by its symmetry. Changing the symmetry via a photoinduced phase
transition offers new ways to manipulate material properties on ultrafast
timescales. However, in order to identify when and how fast these phase
transitions occur, methods that can probe the symmetry change in the time
domain are required. We show that a time-dependent change in the coherent
phonon spectrum can probe a change in symmetry of the lattice potential, thus
providing an all-optical probe of structural transitions. We examine the
photoinduced structural phase transition in VO2 and show that, above the phase
transition threshold, photoexcitation completely changes the lattice potential
on an ultrafast timescale. The loss of the equilibrium-phase phonon modes
occurs promptly, indicating a non-thermal pathway for the photoinduced phase
transition, where a strong perturbation to the lattice potential changes its
symmetry before ionic rearrangement has occurred.Comment: 14 pages 4 figure
Restoring interlayer Josephson coupling in La1.885Ba0.115CuO4 by charge transfer melting of stripe order
We show that disruption of charge-density-wave (stripe) order by charge transfer excitation, enhances the superconducting phase rigidity in La1.885Ba0.115CuO4. Time-resolved resonant soft x-ray diffraction demonstrates that charge order melting is prompt following near-infrared photoexcitation whereas the crystal structure remains intact for moderate fluences. THz time-domain spectroscopy reveals that, for the first 2 ps following photoexcitation, a new Josephson plasma resonance edge, at higher frequency with respect to the equilibrium edge, is induced indicating enhanced superconducting interlayer coupling. The fluence dependence of the charge-order melting and the enhanced superconducting interlayer coupling are correlated with a saturation limit of âŒ0.5mJ/cm2. Using a combination of x-ray and optical spectroscopies we establish a hierarchy of timescales between enhanced superconductivity, melting of charge order, and rearrangement of the crystal structure
Femtosecond dynamics of the collinear-to-spiral antiferromagnetic phase transition in CuO
We report on the ultrafast dynamics of magnetic order in a single crystal of
CuO at a temperature of 207 K in response to strong optical excitation using
femtosecond resonant x-ray diffraction. In the experiment, a femtosecond laser
pulse induces a sudden, nonequilibrium increase in magnetic disorder. After a
short delay ranging from 400 fs to 2 ps, we observe changes in the relative
intensity of the magnetic ordering diffraction peaks that indicate a shift from
a collinear commensurate phase to a spiral incommensurate phase. These results
indicate that the ultimate speed for this antiferromagnetic re-orientation
transition in CuO is limited by the long-wavelength magnetic excitation
connecting the two phases.Comment: Accepted by Physical Review Letters (Dec. 2, 2011
Ultrafast Structural Phase Transition Driven by Photoinduced Melting of Charge and Orbital Order
We use femtosecond x-ray diffraction to probe directly the structural dynamics of a charge ordered and orbitally ordered thin film of La0.42Ca0.58MnO3 initiated by an ultrafast optical pulse. At low excitation fluences we observe the displacive excitation of a coherent optical A(g) phonon. Under high excitation conditions we observe a complete phase transition within 1 ps via the disappearance of a superlattice reflection. The initial step of the phase transition occurs on a time scale significantly faster than the 200 fs time resolution of our experiment
Nonthermal Melting of a Charge Density Wave in TiSe2
We use time-resolved optical reflectivity and x-ray diffraction with femtosecond resolution to study the dynamics of the structural order parameter of the charge density wave phase in TiSe2. We find that the energy density required to melt the charge density wave nonthermally is substantially lower than that required for thermal suppression and is comparable to the charge density wave condensation energy. This observation, together with the fact that the structural dynamics take place on an extremely fast time scale, supports the exciton condensation mechanism for the charge density wave in TiSe2