58 research outputs found
Semiclassical analysis of the lowest-order multipole deformations of simple metal clusters
We use a perturbative semiclassical trace formula to calculate the three
lowest-order multipole (quadrupole \eps_2, octupole \eps_3, and
hexadecapole \eps_4) deformations of simple metal clusters with atoms in their ground states. The self-consistent mean field of the
valence electrons is modeled by an axially deformed cavity and the oscillating
part of the total energy is calculated semiclassically using the shortest
periodic orbits. The average energy is obtained from a liquid-drop model
adjusted to the empirical bulk and surface properties of the sodium metal. We
obtain good qualitative agreement with the results of quantum-mechanical
calculations using Strutinsky's shell-correction method.Comment: LaTeX file (v2) 6 figures, to be published in Phys. Lett.
A Comprehensive Approach to Investigating Fluorine-Bearing Gas Mixtures
An integrated method is proposed for examining the compositions of fluorine-bearing gaseous mixtures, which allows for determining the concentration of HF, F2, N2, O2, CO2, CF4, and C2F6 in these mixtures. The concentration of hydrogen fluoride is determined by its sorption on sodium fluoride followed by the determination of the fluoride ion by the potentiometric method. The lower threshold of determination of hydrogen fluoride is found to be 0.09 vol.%. The concentrations of N2, O2, CO2, CF4, and C2F6 are determined by the gas chromatographic method using a thermal conductivity detector. The proposed gas-chromatography method offers a quantitative measurement of the concentration of N2, O2, CO2, CF4, and C2F6 at the lower limits of detection of 0.008, 0.012, 0.011, 0.009, and 0.019 vol.%, respectively. Based on the developed method, the compositions of a standard fluorine-nitrogen (10 vol.%) and anodic gas samples, synthesized in a laboratory electrolyzer at the National Research Tomsk Polytechnic University and in an industrial electrochemical reactor at JSC Siberian Chemical Plant (Russia), are studied
Possible doublet mechanism for a regular component of parity violation in neutron scattering
A nucleus with octupole deformation of the mean field reveals rotational
doublets with the same angular momentum and opposite parity. Mediated by the
Coriolis-type interaction, the doublet structure leads to a strong regular
component in the parity violation caused by weak interaction. This can explain
sign correlations observed in polarized neutron scattering by Th.Comment: 10 pages, revtex, no figure
Cluster Interpretation of Properties of Alternating Parity Bands in Heavy Nuclei
The properties of the states of the alternating parity bands in actinides,
Ba, Ce and Nd isotopes are analyzed within a cluster model. The model is based
on the assumption that cluster type shapes are produced by the collective
motion of the nuclear system in the mass asymmetry coordinate. The calculated
spin dependences of the parity splitting and of the electric multipole
transition moments are in agreement with the experimental data.Comment: 29 pages, 10 figure
Collinear cluster tripartition as sequential binary fission in the U(n,f) reaction
The mechanism leading to the formation of the observed products of the
collinear cluster tripartition is carried out within the framework of the model
based on the dinuclear system concept. The yield of fission products is
calculated using the statistical model based on the driving potentials for the
fissionable system. The minima of potential energy of the decaying system
correspond to the charge numbers of the products which are produced with large
probabilities in the sequential fission (partial case of the collinear cluster
tripartition) of the compound nucleus. The realization of this mechanism
supposes the asymmetric fission channel as the first stage of sequential
mechanism. It is shown that only the use of the driving potential calculated by
the binding energies with the shell correction allows us to explain the yield
of the true ternary fission products. The theoretical model is applied to
research collinear cluster tripartition in the reaction U(n,f). Calculations showed that in the first stage of this fission reaction,
the isotopes Ge and Nd are formed with relatively large
probabilities and in the second stage of sequential fission of the isotope Nd
mainly Ni and Ge are formed. This is in agreement with the yield of the isotope
Ni which is observed as the product of the collinear cluster
tripartition in the experiment.Comment: 20 pages, 9 figure
Adiabatic description of nonspherical quantum dot models
Within the effective mass approximation an adiabatic description of
spheroidal and dumbbell quantum dot models in the regime of strong dimensional
quantization is presented using the expansion of the wave function in
appropriate sets of single-parameter basis functions. The comparison is given
and the peculiarities are considered for spectral and optical characteristics
of the models with axially symmetric confining potentials depending on their
geometric size making use of the total sets of exact and adiabatic quantum
numbers in appropriate analytic approximations
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