The influence of depolarization field on dielectric and pyroelectric properties of ferroelectric films

Calculations of the spontaneous polarization (Ps), dielectric susceptibility (c) and pyroelectric coefficient (P) of the ferroelectric films have been performed in the thermodynamic phenomenological theory framework. The Euler-Lagrange equation determining polarization dependence on the film parameters and the external electric field was solved analytically under the boundary conditions with different extrapolation lengths at two surfaces, respectively. The depolarization field contribution was taken into account in the model of short-circuited mono-domain ferroelectric film, treated as perfect insulator. The detailed analysis of the aforementioned quantities, space distribution and their average values in two cases with and without depolarization field was carried out. It was shown that the depolarization field shifts critical temperature to smaller values and the critical thickness to bigger value in comparison to those obtained without accounting the depolarization field. Meanwhile average values of Ps, c and P dependences on the film parameters and temperature are similar to the corresponding dependences obtained without accounting the depolarization field. The depolarization field was shown to flatten Ps, c and P space distributions, which have the peculiarities otherwise (e.g. small maxima in c and P coordinate profiles near the film surfaces). It was shown that depolarization field influence in short-circuited film could be neglected when the film thickness or the extrapolation lengths in the boundary conditions are larger than the correlation length value

The enhancement of ferromagnetism in uniaxially stressed diluted magnetic semiconductors

We predict a new mechanism of enhancement of ferromagnetic phase transition temperature $T_c$ in uniaxially stressed diluted magnetic semiconductors (DMS) of p-type. Our prediction is based on comparative studies of both Heisenberg (inherent to undistorted DMS with cubic lattice) and Ising (which can be applied to strongly enough stressed DMS) models in a random field approximation permitting to take into account the spatial inhomogeneity of spin-spin interaction. Our calculations of phase diagrams show that area of parameters for existence of DMS-ferromagnetism in Ising model is much larger than that in Heisenberg model.Comment: Accepted for publication in Phys. Rev.

Suppression of carrier induced ferromagnetism by composition and spin fluctuations in diluted magnetic semiconductors

We suggest an approach to account for spatial (composition) and thermal fluctuations in "disordered" magnetic models (e.g. Heisenberg, Ising) with given spatial dependence of magnetic spin-spin interaction. Our approach is based on introduction of fluctuating molecular field (rather than mean field) acting between the spins. The distribution function of the above field is derived self-consistently. In general case this function is not Gaussian, latter asymptotics occurs only at sufficiently large spins (magnetic ions) concentrations $n_i$. Our approach permits to derive the equation for a critical temperature $T_c$ of ferromagnetic phase transition with respect to the above fluctuations. We apply our theory to the analysis of influence of composition fluctuations on $T_c$ in diluted magnetic semiconductors (DMS) with RKKY indirect spin-spin interaction.Comment: 6 pages, 2 figure

Energy scales and magnetoresistance at a quantum critical point

The magnetoresistance (MR) of CeCoIn_5 is notably different from that in many conventional metals. We show that a pronounced crossover from negative to positive MR at elevated temperatures and fixed magnetic fields is determined by the scaling behavior of quasiparticle effective mass. At a quantum critical point (QCP) this dependence generates kinks (crossover points from fast to slow growth) in thermodynamic characteristics (like specific heat, magnetization etc) at some temperatures when a strongly correlated electron system transits from the magnetic field induced Landau Fermi liquid (LFL) regime to the non-Fermi liquid (NFL) one taking place at rising temperatures. We show that the above kink-like peculiarity separates two distinct energy scales in QCP vicinity - low temperature LFL scale and high temperature one related to NFL regime. Our comprehensive theoretical analysis of experimental data permits to reveal for the first time new MR and kinks scaling behavior as well as to identify the physical reasons for above energy scales.Comment: 7 pages, 6 figure

Direct evidence of soft mode behavior near the Burns' temperature in PbMg1/3_{1 / 3}Nb2/3_{2 / 3}O3_{3} (PMN) relaxor ferroectric

Inelastic neutron scattering measurements of the relaxor ferroelectric PbMg$_{1 / 3}$Nb$_{2 / 3}$O$_{3}$ (PMN) in the temperature range 490~K$<$T$<$880~K directly observe the soft mode (SM) associated with the Curie-Weiss behavior of the dielectric constant $\varepsilon$(T). The results are treated within the framework of the coupled SM and transverse optic (TO1) mode and the temperature dependence of the SM frequency at q=0.075 a* is determined. The parameters of the SM are consistent with the earlier estimates and the frequency exhibits a minimum near the Burns temperature ($\approx$ 650K)Comment: 6 figure