107 research outputs found

    Plasmonic and Thermooptical Properties of Spherical Metallic Nanoparticles for Their Thermoplasmonic and Photonic Applications

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    Investigations and use of nanoparticles (NPs) as photothermal (PT) agents in laser and optical nanotechnology are fast growing areas of research and applications. The potential benefits of NPs applications include possibility for thermal imaging and treatment of materials containing of NPs, applications of NPs for light-to-thermal energy conversion, in catalysis, laser nanomedicine, and chemistry. Efficiency of applications of metallic NPs for laser and optical nanotechnology depends on plasmonic and thermophysical properties of NPs, characteristics of radiation, and surroundingmedium. Herewe present the results of comparative analysis of NP properties (plasmonic, thermooptical, and others) allowing selecting their parameters for thermoplasmonic and photonic applications. Plasmonic and thermooptical properties of several metallic (aurum, silver, platinum, cobalt, zinc, nickel, titanium, cuprum, aluminum, molybdenum, vanadium, and palladium) NPs are theoretically investigated and analysis of them is carried out. Investigation of the influence of NPs parameters (type of metal, radii, optical indexes, density, and heat capacity of NP material), characteristics of radiation (wavelength and pulse duration), and ambient parameters on plasmonic and thermophysical properties of NPs has been carried out. It was established that maximum value of thermooptical parameter (maximum NP temperature) can be achieved with the use of absorption efficiency factor of NP smaller than its maximum valu

    Light-absorption selection of nanoparticles and nanofluids containing nanoparticles for their effective heating by solar radiation

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    Light-absorption selection of single nanoparticle for solar radiation requires the simultaneous fulfillment of all of the following novel conditions—maximal close (overlap) of the dependence of nanoparticle efficiency absorption factor on wavelength with the dependence solar irradiance, predominant role of nanoparticle absorption over its scattering, the use of maximal values of nanoparticle efficiency absorption factor and its size. These results highlight the possibility for effective application of single homogeneous Ti and core–shell Ti–TiO2, Ni–NiO nanoparticles with radii of about 75 nm as perfect absorbers for solar radiation in the complete optical spectrum 250–2500 nm

    Microscopic Calculation of Total Ordinary Muon Capture Rates for Medium - Weight and Heavy Nuclei

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    Total Ordinary Muon Capture (OMC) rates are calculated on the basis of the Quasiparticle Random Phase Approximation for several spherical nuclei from 90^Zr to 208^Pb. It is shown that total OMC rates calculated with the free value of the axial-vector coupling constant g_A agree well with the experimental data for medium-size nuclei and exceed considerably the experimental rates for heavy nuclei. The sensitivity of theoretical OMC rates to the nuclear residual interactions is discussed.Comment: 27 pages and 3 figure

    Dislocation Kinks in Copper: Widths, Barriers, Effective Masses, and Quantum Tunneling

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    We calculate the widths, migration barriers, effective masses, and quantum tunneling rates of kinks and jogs in extended screw dislocations in copper, using an effective medium theory interatomic potential. The energy barriers and effective masses for moving a unit jog one lattice constant are close to typical atomic energies and masses: tunneling will be rare. The energy barriers and effective masses for the motion of kinks are unexpectedly small due to the spreading of the kinks over a large number of atoms. The effective masses of the kinks are so small that quantum fluctuations will be important. We discuss implications for quantum creep, kink--based tunneling centers, and Kondo resonances

    Breit Hamiltonian and QED Effects for Spinless Particles

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    We describe a simplified derivation for the relativistic corrections of order α4\alpha^4 for a bound system consisting of two spinless particles. We devote special attention to pionium, the bound system of two oppositely charged pions. The leading quantum electrodynamic (QED) correction to the energy levels is of the order of α3\alpha^3 and due to electronic vacuum polarization. We analyze further corrections due to the self-energy of the pions, and due to recoil effects, and we give a complete result for the scalar-QED leading logarithmic corrections which are due to virtual loops involving only the scalar constituent particles (the pions); these corrections are of order α5lnα\alpha^5 \ln \alpha for S states.Comment: 12 pages, LaTeX; references added (J. Phys. B, in press

    Nonlinear thermo-optical properties of two-layered spherical system of gold nanoparticle core and water vapor shell during initial stage of shell expansion

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    Nonlinear thermo-optical properties of two-layered spherical system of gold nanoparticle core and water vapor shell, created under laser heating of nanoparticle in water, were theoretically investigated. Vapor shell expansion leads to decreasing up to one to two orders of magnitude in comparison with initial values of scattering and extinction of the radiation with wavelengths 532 and 633 nm by system while shell radius is increased up to value of about two radii of nanoparticle. Subsequent increasing of shell radius more than two radii of nanoparticle leads to rise of scattering and extinction properties of system over initial values. The significant decrease of radiation scattering and extinction by system of nanoparticle-vapor shell can be used for experimental detection of the energy threshold of vapor shell formation and investigation of the first stages of its expansion

    The Boltzmann equation for colourless plasmons in hot QCD plasma. Semiclassical approximation

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    Within the framework of the semiclassical approximation, we derive the Boltzmann equation describing the dynamics of colorless plasmons in a hot QCD plasma. The probability of the plasmon-plasmon scattering at the leading order in the coupling constant is obtained. This probability is gauge-independent at least in the class of the covariant and temporal gauges. It is noted that the structure of the scattering kernel possesses important qualitative difference from the corresponding one in the Abelian plasma, in spite of the fact that we focused our study on the colorless soft excitations. It is shown that four-plasmon decay is suppressed by the power of gg relative to the process of nonlinear scattering of plasmons by thermal particles at the soft momentum scale. It is stated that the former process becomes important in going to the ultrasoft region of the momentum scale.Comment: 41, LaTeX, minor changes, identical to published versio
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