300 research outputs found
Photoconductive detection of hydrogen in ZnO and rutile TiO2
Hydrogen donors in ZnO and rutile TiO2 are probed by means of
photoconductivity and IR absorption. It is shown that the O–H bonds giving
rise to the local vibrational modes (LVMs) of interstitial hydrogen at 3611
and 3290 cm−1 in the case of ZnO and TiO2, respectively, also occur in the
photoconductivity spectra as Fano resonances. The effects of isotope
substitution, concentration, sample thickness, influence of other donors
present in both oxides are considered. Based on the shape and frequency of
these resonances, it is concluded that the apparent ionization energy of
interstitial hydrogen in rutile TiO2 is less than 300 meV. By a direct
comparison, we also demonstrate that photoconductive detection of LVMs of
defects in thin semiconductor films is superior to the standard IR absorption
On the method of photoconductive detection of defects in semiconductors by vibrational mode-related Fano resonances
The method of photoconductive detection of defect-related vibrational modes in semiconductors by Fano resonances is validated by a combined photoconductivity and infrared absorption study of the interstitial hydrogen donor in ZnO. Depth-resolved isotopic substitution experiments with varying concentrations of H and D show that the effect of vibrational mode-related absorption has to be taken into account in order to allow for an unambiguous interpretation of the experimental data. A quantitative model is presented which describes the influence of sample thickness, defect concentration, and the presence of other donors on the sign, magnitude, and shape of the Fano resonances. Implications for the photoconductive detection of defect-related vibrational modes are discusse
Symplectic geometries on supermanifolds
Extension of symplectic geometry on manifolds to the supersymmetric case is
considered. In the even case it leads to the even symplectic geometry (or,
equivalently, to the geometry on supermanifolds endowed with a non-degenerate
Poisson bracket) or to the geometry on an even Fedosov supermanifolds. It is
proven that in the odd case there are two different scalar symplectic
structures (namely, an odd closed differential 2-form and the antibracket)
which can be used for construction of symplectic geometries on supermanifolds.Comment: LaTex, 1o pages, LaTex, changed conten
UV continuum emission and diagnostics of hydrogen-containing non-equilibrium plasmas
For the first time the emission of the radiative dissociation continuum of
the hydrogen molecule ( electronic
transition) is proposed to be used as a source of information for the
spectroscopic diagnostics of non-equilibrium plasmas. The detailed analysis of
excitation-deactivation kinetics, rate constants of various collisional and
radiative transitions and fitting procedures made it possible to develop two
new methods of diagnostics of: (1) the ground state
vibrational temperature from the relative intensity
distribution, and (2) the rate of electron impact dissociation
(d[\mbox{H_{2}}]/dt)_{\text{diss}} from the absolute intensity of the
continuum. A known method of determination of from relative
intensities of Fulcher- bands was seriously corrected and simplified
due to the revision of transition probabilities and cross sections of
electron impact excitation. General considerations are illustrated
with examples of experiments in pure hydrogen capillary-arc and H+Ar
microwave discharges.Comment: REVTeX, 25 pages + 12 figures + 9 tables. Phys. Rev. E, eprint
replaced because of resubmission to journal after referee's 2nd repor
Competition and coexistence of antiferromagnetism and superconductivity in RBa_2Cu_3O_{6+x} (R = Lu, Y) single crystals
We use c-axis resistivity and magnetoresistance measurements to study the
interplay between antiferromagnetic (AF) and superconducting (SC) ordering in
underdoped RBa_2Cu_3O_{6+x} (R = Lu, Y) single crystals. Both orders are found
to emerge from an anisotropic 3D metallic state, upon which antiferromagnetism
opposes superconductivity by driving the doped holes towards localization.
Despite the competition, the superconductivity sets in before the AF order is
completely destroyed and coexists with latter in a certain range of hole
doping. We find also that strong magnetic fields affect the AF-SC interplay by
both suppressing the superconductivity and stabilizing the Neel order.Comment: 7 pages, 6 figure
Normal-state resistivity anisotropy in underdoped RBa_2Cu_3O_{6+x} crystals
We have revealed new features in the out-of-plane resistivity rho_c of
heavily underdoped RBa_2Cu_3O_{6+x} (R=Tm,Lu) single crystals, which give
evidence for two distinct mechanisms contributing the c-axis transport. We have
observed a crossover towards "metal-like" (d rho_c/d T > 0) behavior at the
temperature T_m which quickly increases with decreasing doping. The
"metal-like" conductivity contribution dominates at T < T_m and provides a
saturation of the resistivity anisotropy, rho_c / rho_{ab}. The
antiferromagnetic ordering is found to block this "metal-like" part of the
c-axis conductivity and complete decoupling of CuO_2 planes, which may be the
reason of superconductivity disappearance.Comment: RevTex, 4 pages including 4 eps figures. To be published in
Phys.Rev.Let
Higher order relations in Fedosov supermanifolds
Higher order relations existing in normal coordinates between affine
extensions of the curvature tensor and basic objects for any Fedosov
supermanifolds are derived. Representation of these relations in general
coordinates is discussed.Comment: 11 LaTex pages, no figure
Magnetoresistance Anomalies in Antiferromagnetic YBa_2Cu_3O_{6+x}: Fingerprints of Charged Stripes
We report novel features in the in-plane magnetoresistance (MR) of heavily
underdoped YBa_2Cu_3O_{6+x}, which unveil a developed ``charged stripe''
structure in this system. One of the striking features is an anisotropy of the
MR with a "d-wave" symmetry upon rotating the magnetic field H within the ab
plane, which is caused by the rotation of the stripes with the external field.
With decreasing temperature, a hysteresis shows up below ~20 K in the MR curve
as a function of H and finally below 10 K the magnetic-field application
produces a persistent change in the resistivity. This "memory effect" is caused
by the freezing of the directionally-ordered stripes.Comment: 4 pages, 6 figures, final version, to appear in 4 October 1999 issue
of PR
Magnetoresistance in Heavily Underdoped YBa_2Cu_3O_{6+x}: Antiferromagnetic Correlations and Normal-State Transport
We report on a contrasting behavior of the in-plane and out-of-plane
magnetoresistance (MR) in heavily underdoped antiferromagnetic (AF)
YBa_2Cu_3O_{6+x} (x<0.37). The out-of-plane MR (I//c) is positive over most of
the temperature range and shows a sharp increase, by about two orders of
magnitude, upon cooling through the Neel temperature T_N. A contribution
associated with the AF correlations is found to dominate the out-of-plane MR
behavior for H//c from far above T_N, pointing to the key role of spin
fluctuations in the out-of-plane transport. In contrast, the transverse
in-plane MR (I//a(b);H//c) appears to be small and smooth through T_N, implying
that the development of the AF order has little effect on the in-plane
resistivity.Comment: 4 pages, 5 figures, accepted for publication in Phys.Rev.Let
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