Studies of Charge Exchange in a High‐Pressure Pulsed Electron Impact Source

This is the publisher's version, also available electronically from http://scitation.aip.org/content/aip/journal/jcp/56/3/10.1063/1.1677327.A high pressure pulsed ion source has been used in a time‐of‐flight mass spectrometer in order to study the charge exchangereactions in Ar–H2 and Ar–D2 systems using the ion source in the Čermák mode of operation. As the source was used in a pulsed mode, it was possible to identify the various secondary ions arising from the charge exchangereactions in these systems. Very good agreement has been shown to exist between the experimental results and simple theoretical deductions. Calculations have been made to determine the cross sections for the charge exchangereactions between the various species from the experimental data

Thin static charged dust Majumdar-Papapetrou shells with high symmetry in D >= 4

We present a systematical study of static D >= 4 space-times of high symmetry with the matter source being a thin charged dust hypersurface shell. The shell manifold is assumed to have the following structure S_(beta) X R^(D-2-beta), beta (in the interval ) is dimension of a sphere S_(beta). In case of (beta) = 0, we assume that there are two parallel hyper-plane shells instead of only one. The space-time has Majumdar-Papapetrou form and it inherits the symmetries of the shell manifold - it is invariant under both rotations of the S_(beta) and translations along R^(D-2-beta). We find a general solution to the Einstein-Maxwell equations with a given shell. Then, we examine some flat interior solutions with special attention paid to D = 4. A connection to D = 4 non-relativistic theory is pointed out. We also comment on a straightforward generalisation to the case of Kastor-Traschen space-time, i.e. adding a non-negative cosmological constant to the charged dust matter source.Comment: Accepted in Int. J. Theor. Phy

Magnonic Weyl states in Cu2OSeO3

The multiferroic ferrimagnet Cu$_2$OSeO$_3$ with a chiral crystal structure attracted a lot of recent attention due to the emergence of magnetic skyrmion order in this material. Here, the topological properties of its magnon excitations are systematically investigated by linear spin-wave theory and inelastic neutron scattering. When considering Heisenberg exchange interactions only, two degenerate Weyl magnon nodes with topological charges $\pm$2 are observed at high-symmetry points. Each Weyl point splits into two as the symmetry of the system is further reduced by including into consideration the nearest-neighbor Dzyaloshinsky-Moriya interaction, crucial for obtaining an accurate fit to the experimental spin-wave spectrum. The predicted topological properties are verified by surface state and Chern number analysis. Additionally, we predict that a measurable thermal Hall conductivity can be associated with the emergence of the Weyl points, the position of which can be tuned by changing the crystal symmetry of the material

Pressure-induced huge increase of Curie temperature of the van der Waals ferromagnet VI3

Evolution of magnetism in single crystals of the van der Waals compound VI3 in external pressure up to 7.3 GPa studied by measuring magnetization and ac magnetic susceptibility is reported. Four magnetic phase transitions, at T1 = 54.5 K, T2 = 53 K, TC = 49.5 K, and TFM = 26 K, respectively have been observed at ambient pressure. The first two have been attributed to the onset of ferromagnetism in specific crystal-surface layers. The bulk ferromagnetism is characterized by the magnetic ordering transition at Curie temperature TC and the transition between two different ferromagnetic phases TFM, accompanied by a structure transition from monoclinic to triclinic symmetry upon cooling. The pressure effects on magnetic parameters were studied with three independent techniques. TC was found to be almost unaffected by pressures up to 0.6 GPa whereas TFM increases rapidly with increasing pressure and reaches TC at a triple point at ~ 0.85 GPa. At higher pressures, only one magnetic phase transition is observed moving to higher temperatures with increasing pressure to reach 99 K at 7.3 GPa. In contrast, the low-temperature bulk magnetization is dramatically reduced by applying pressure (by more than 50% at 2.5 GPa) suggesting a possible pressure-induced reduction of vanadium magnetic moment. We discussed these results in light of recent theoretical studies to analyze exchange interactions and provide how to increase the Curie temperature of VI3.Comment: 20 pages, 16 figure

Long-range magnetic order in CePdAl3_3 enabled by orthorhombic deformation

We investigate the effect of structural deformation on the magnetic properties of orthorhombic CePdAl$_3$ in relation to its tetragonal polymorph. Utilizing x-ray and neutron diffraction we establish that the crystal structure has the $Cmcm$ space group symmetry and exhibits pseudo-tetragonal twinning. According to density-functional calculations the tetragonal-orthorhombic deformation mechanism has its grounds in relatively small free enthalpy difference between the polymorphs, allowing either phase to be quenched and fully accounts for the twinned microstructure of the orthorhombic phase. Neutron diffraction measurements show that orthorhombic CePdAl$_3$ establishes long-range magnetic order below $T_\mathrm{N}$=5.29 (5) K characterized by a collinear, antiferromagnetic arrangement of magnetic moments. Magnetic anisotropies of orthorhombic CePdAl$_3$ arise from strong spin-orbit coupling as evidenced by the crystal-field splitting of the $4f$ multiplet, fully characterised with neutron spectroscopy. We discuss the potential mechanism of frustration posed by antiferromagnetic interactions between nearest neighbours in the tetragonal phase, which hinders the formation of long-range magnetic order in tetragonal CePdAl$_3$. We propose that orthorhombic deformation releases the frustration and allows for long-range magnetic order.Comment: Finalized paper from the splitting of arxiv.org/abs/2106.08194v

Guided assembly of nanoparticles on electrostatically charged nanocrystalline diamond thin films

We apply atomic force microscope for local electrostatic charging of oxygen-terminated nanocrystalline diamond (NCD) thin films deposited on silicon, to induce electrostatically driven self-assembly of colloidal alumina nanoparticles into micro-patterns. Considering possible capacitive, sp2 phase and spatial uniformity factors to charging, we employ films with sub-100 nm thickness and about 60% relative sp2 phase content, probe the spatial material uniformity by Raman and electron microscopy, and repeat experiments at various positions. We demonstrate that electrostatic potential contrast on the NCD films varies between 0.1 and 1.2 V and that the contrast of more than ±1 V (as detected by Kelvin force microscopy) is able to induce self-assembly of the nanoparticles via coulombic and polarization forces. This opens prospects for applications of diamond and its unique set of properties in self-assembly of nano-devices and nano-systems

A transdisciplinary co‐conceptualisation of marine identity

Challenge 10 of the United Nations Decade of Ocean Science for Sustainable Development (2021–2030) calls for the restoration of society's relationship with the ocean. Research suggests that the relationship people have with marine environments can influence their depth of engagement in marine citizenship action, and the important role for ‘marine identity’ in driving that action. Although identity is well‐researched, marine identity is a concept novel to academia and a baseline understanding is required, both to grasp the scope of the concept, and to support research into its role in transforming the human‐ocean relationship. Here, a transdisciplinary study, endorsed as a UN Ocean Decade Activity and by the EU Mission Ocean & Waters, brought together a multinational community of marine researchers and practitioners to co‐produce a baseline conceptualisation of marine identity, drawing on photovoice and deliberative methodology. This paper presents the findings of the co‐production process and offers a first introduction in the literature of the multiple variations and formations of marine identity. We find marine identity to be a complex and multidimensional concept, suffused with individual experiences and understandings of the marine environment, based on social and cultural understandings of the ocean, contemporarily and historically. We present real‐world examples of marine identity to illustrate key themes that were developed through co‐production. Policy implications: We propose marine identity as a catalyst for understanding existing multifaceted and caring relationships with the ocean, as well as the restoration of society's relationship with the ocean. Marine identity research should, therefore, be prioritised in research seeking to contribute to the UN Ocean Decade Challenge 10, as this will support integration of non‐material values of the ocean into marine planning processes and policy making, enabling effective responses to Challenge 10's emphasis on integrating traditional/cultural ways of knowing and valuing the marine environment, through diverse marine identities. We welcome research efforts that will further develop the marine identity concept and empirically investigate the relationships between marine identity, marine citizenship, and people's relationships with the ocean. Read the free Plain Language Summary for this article on the Journal blog