Observation of correlated spin-orbit order in a strongly anisotropic quantum wire system

Quantum wires with spin-orbit coupling provide a unique opportunity to simultaneously control the coupling strength and the screened Coulomb interactions where new exotic phases of matter can be explored. Here we report on the observation of an exotic spin-orbit density wave in Pb-atomic wires on Si(557) surfaces by mapping out the evolution of the modulated spin-texture at various conditions with spin- and angle-resolved photoelectron spectroscopy. The results are independently quantified by surface transport measurements. The spin polarization, coherence length, spin dephasing rate, and the associated quasiparticle gap decrease simultaneously as the screened Coulomb interaction decreases with increasing excess coverage, providing a new mechanism for generating and manipulating a spin-orbit entanglement effect via electronic interaction. Despite clear evidence of spontaneous spin-rotation symmetry breaking and modulation of spin-momentum structure as a function of excess coverage, the average spin-polarization over the Brillouin zone vanishes, indicating that time-reversal symmetry is intact as theoretically predicted

Plasmon localization by adatoms in gold atomic wires on Si(775)

Self-organized gold chains on vicinal Si(111) surfaces represent prototype examples of quasi-one-dimensional objects that are stabilized by hybridization with Si surface states. Their plasmons contain important information about the unoccupied bandstructure close to the Fermi level. Using Si(775)-Au as an example, we report here the modifications of the plasmon dispersion by the simple atomic adatom species H and O. Using a combination of low energy electron diffraction and high-resolution electron energy loss spectroscopy, we study the interconnection between plasmonic excitation and the corresponding local surface structure. Both adsorbates do not destroy metallicity, but, similar to Si(553)-Au, atomic hydrogen enhances dimerization of the Au chains, which at small concentrations counteracts the disorder introduced by random adsorption. This effect, most likely caused by electron donation of H to the surface states, is missing in case of adsorbed oxygen, so that only the effect of disorder is observed. For both adsorbates increasing disorder as a function of adsorbate concentration finally results in plasmon localization and opening of a band gap

Plasmons in one and two dimensions

Plasmons in low-dimensional systems respresent an important tool for coupling energy into nanostructures and the localization of energy on the scale of only a few nanometers. Contrary to ordinary surface plasmons of metallic bulk materials, their dispersion goes to zero in the long wavelength limit, thus covering a broad range of energies from terahertz to near infrared, and from mesoscopic wavelengths down to just a few nanometers. Using specific and most characteristic examples, we review first the properties of plasmons in two-dimensional (2D) metallic layers from an experimental point of view. As demonstrated, tuning of their dispersion is possible by changes of charge carrier concentration in the partially filled 2D conduction bands, but for the relativistic electron gas like in graphene only in the long wavelength limit. For short wavelengths, on the other hand, the dispersion turns out to be independent of the position of the Fermi level with respect to the Dirac point. A linear dispersion, seen under the latter conditions in graphene, can also be obtained in non-relativistic electron gases by coupling between 2D and 3D electronic systems. As a well investigated example, the acoustic surface plasmons in Shockley surface states, coupled with the bulk electronic system, are discussed. Also the introduction of anisotropy, e.g. by regular arrays of steps, seems to result in linearization (and to partial localization of the plasmons normal to the steps, depending on wavelengths). In quasi-one dimensional (1D) systems, such as arrays of gold chains on regularly stepped Si surfaces, only the dispersion is 1D, whereas shape and slope of the dispersion curves depend on the 2D distribution of charge within each terrace and on coupling between wires on different terraces

Sheet plasmons in modulated graphene on Ir(111)

The sheet plasmon of graphene on Ir(111) was investigated in this paper by means of high-resolution electron energy loss spectroscopy. The perfect lateral coordination of sp2-hybridized C atoms on a large scale is manifested by brilliant moiré diffraction images. However, the modulation of the graphene films caused by hybridization at the interface limits the lifetimes of the collective excitation modes. This modulation within the films can be lowered owing to intercalation of Na. Linear dispersion was found, but surprisingly the overall slope of the dispersion is not dependent on the chemical potential within the graphene films. The dispersion measured for graphene on Ir(111) is almost identical to that measured on SiC(0001), although the carrier densities differ by two orders of magnitude. This contradicts the model that the relevant carrier density for a two-dimensional plasmon is given by (2π) -1k2 F © IOP Publishing Ltd and Deutsche Physikalische Gesellschaft.DF

Origin of metallicity in atomic Ag wires on Si(557)

We investigated the metallicity of Ag-root 3 ordered atomic wires close to one monolayer (ML) coverage, which are formed on Si(557) via self assembly. For this purpose we combined high resolution electron energy loss spectroscopy with tunneling microscopy. By extending the excess Ag coverage up to 0.6 ML on samples annealed at high temperatures where partial desorption occurs, we demonstrate that one-dimensional metallicity in the Ag-root 3 x root 3 R30 degrees ordered atomic wires on the (111) mini-terraces originates only from Ag atoms in excess of (local) monolayer coverage, which are adsorbed and localized at the highly stepped parts of the Si(557) surface. Thus these Ag atoms act as extrinsic dopants on the atomic scale, causing coverage dependent subband filling and increasing localization as a function of doping concentration. The second layer lattice gas as well as Ag islands on the (111) terraces turn out not to be relevant as dopants. We simulated the peculiar saturation behavior within a modified lattice gas model and give evidence that the preparation dependent saturation of doping is due to changes of average terrace size and step morphology induced by high temperature treatment.Niedersächsisches Ministerium für Wissenschaftund KulturDFG/FOR/170

Graphene plasmons and retardation: strong light-matter coupling

We study the retardation regime of doped graphene plasmons, given by the nominal crossing of the unretarded plasmon and light-cone. In addition to modifications in the plasmon dispersion relation, retardation implies strong coupling between propagating light and matter, even for homogeneous graphene, which opens up the possibility of efficient plasmonics in simple graphene devices. We exemplify this enhancement in a double-layer configuration that exhibits {\em perfect} (if lossless) light transmissions across a classically forbidden region, providing a simpler analog of the corresponding phenomenon in perforated metal sheets. We also show that (broad) Fabry-P\'erot resonances present without graphene turn into sharply peaked, quasi-discrete modes in the presence of graphene where graphene's response function is given by the typical Fano lineshape.Comment: 6 pages, 4 figure

Scattering at magnetic and nonmagnetic impurities on surfaces with strong spin-orbit coupling

Adsorption-induced reduction of surface-state conductivity in epitaxial Bi(111) films, a prototype system with large Rashba-induced surface-state splitting, by adsorbed atoms of Bi, Fe, and Co has been investigated by macroscopic surface magnetotransport measurements at a temperature of 10 K. A detailed analysis of magnetotransport, dc transport, and Hall data reveals that the scattering efficiencies for Co and Fe are larger by a factor of 2 than that for Bi. While for the latter charge transfer and change of band filling near the Fermi level are negligible, we find an increase of hole concentration upon Co and Fe adsorption. These atoms act as acceptors and immobilize on average about 0.5 electrons per adsorbed atom. Besides the dominant classical magnetoconductance signal the films show signatures of weak antilocalization, reflecting the strong spin-orbit coupling in Bi(111) surface states. This behavior can be changed to weak localization by the adsorption of high concentrations (0.1 monolayers) of magnetic impurities (Fe,Co), similarly to results found on the topological insulator Bi2Se3. Our results demonstrate that details of chemical bond formation for impurities are crucial for local spin moments and electronic scattering properties. © 2012 American Physical Society.DFGDAA

Tuning the conductivity along atomic chains by selective chemisorption

Adsorption of Au on vicinal Si(111) surfaces results in growth of long-range ordered metallic quantum wires. In this paper, we utilized site-specific and selective adsorption of oxygen to modify chemically the transport via different channels in the systems Si(553)-Au and Si(557)-Au. They were analyzed by electron diffraction and four-tip STM-based transport experiments. Modeling of the adsorption process by density functional theory shows that the adatoms and rest atoms on Si(557)-Au provide energetically favored adsorption sites, which predominantly alter the transport along the wire direction. Since this structural motif is missing on Si(553)-Au, the transport channels remain almost unaffected by oxidation. © 2017 American Physical Society.DFG/FOR/170

Plasmons in layered structures including graphene

We investigate the optical properties of layered structures with graphene at the interface for arbitrary linear polarization at finite temperature including full retardation by working in the Weyl gauge. As a special case, we obtain the full response and the related dielectric function of a layered structure with two interfaces. We apply our results to discuss the longitudinal plasmon spectrum of several single and double layer devices such as systems with finite and zero electronic densities. We further show that a nonhomogeneous dielectric background can shift the relative weight of the in-phase and out-of-phase mode and discuss how the plasmonic mode of the upper layer can be tuned into an acoustic mode with specific sound velocity.Comment: 18 pages, 6 figure