Direct versus Delayed pathways in Strong-Field Non-Sequential Double Ionization

We report full-dimensionality quantum and classical calculations for double ionization of laser-driven helium at 390 nm. Good qualitative agreement is observed. We show that the classical double ionization trajectories can be divided into two distinct pathways: direct and delayed. The direct pathway, with an almost simultaneous ejection of both electrons, emerges from small laser intensities. With increasing intensity its relative importance, compared to the delayed ionization pathway, increases until it becomes the predominant pathway for total electron escape energy below around 5.25 $U_{p}$. However the delayed pathway is the predominant one for double ionization above a certain cut-off energy at all laser intensities

From soft harmonic phonons to fast relaxational dynamics in CH3_{3}NH3_{3}PbBr3_{3}

The lead-halide perovskites, including CH$_{3}$NH$_{3}$PbBr$_{3}$, are components in cost effective, highly efficient photovoltaics, where the interactions of the molecular cations with the inorganic framework are suggested to influence the electronic and ferroelectric properties. CH$_{3}$NH$_{3}$PbBr$_{3}$ undergoes a series of structural transitions associated with orientational order of the CH$_{3}$NH$_{3}$ (MA) molecular cation and tilting of the PbBr$_{3}$ host framework. We apply high-resolution neutron scattering to study the soft harmonic phonons associated with these transitions, and find a strong coupling between the PbBr$_{3}$ framework and the quasistatic CH$_{3}$NH$_{3}$ dynamics at low energy transfers. At higher energy transfers, we observe a PbBr$_{6}$ octahedra soft mode driving a transition at 150 K from bound molecular excitations at low temperatures to relatively fast relaxational excitations that extend up to $\sim$ 50-100 meV. We suggest that these temporally overdamped dynamics enables possible indirect band gap processes in these materials that are related to the enhanced photovoltaic properties.Comment: (main text - 5 pages, 4 figures; supplementary information - 3 pages, 3 figures

Absence of strong magnetic fluctuations in the iron phosphide superconductors LaFePO and Sr2ScO3FeP

We report neutron inelastic scattering measurements on polycrystalline LaFePO and Sr2ScO3FeP, two members of the iron phosphide families of superconductors. No evidence is found for any magnetic fluctuations in the spectrum of either material in the energy and wavevector ranges probed. Special attention is paid to the wavevector at which spin-density-wave-like fluctuations are seen in other iron-based superconductors. We estimate that the magnetic signal, if present, is at least a factor of four (Sr2ScO3FeP) or seven (LaFePO) smaller than in the related iron arsenide and chalcogenide superconductors. These results suggest that magnetic fluctuations are not as influential on the electronic properties of the iron phosphide systems as they are in other iron-based superconductors.Comment: 7 pages, 5 figure

A combined R-matrix eigenstate basis set and finite-differences propagation method for the time-dependent Schr\"{od}dinger equation: the one-electron case

In this work we present the theoretical framework for the solution of the time-dependent Schr\"{o}dinger equation (TDSE) of atomic and molecular systems under strong electromagnetic fields with the configuration space of the electron's coordinates separated over two regions, that is regions $I$ and $II$. In region $I$ the solution of the TDSE is obtained by an R-matrix basis set representation of the time-dependent wavefunction. In region $II$ a grid representation of the wavefunction is considered and propagation in space and time is obtained through the finite-differences method. It appears this is the first time a combination of basis set and grid methods has been put forward for tackling multi-region time-dependent problems. In both regions, a high-order explicit scheme is employed for the time propagation. While, in a purely hydrogenic system no approximation is involved due to this separation, in multi-electron systems the validity and the usefulness of the present method relies on the basic assumption of R-matrix theory, namely that beyond a certain distance (encompassing region $I$) a single ejected electron is distinguishable from the other electrons of the multi-electron system and evolves there (region II) effectively as a one-electron system. The method is developed in detail for single active electron systems and applied to the exemplar case of the hydrogen atom in an intense laser field.Comment: 13 pages, 6 figures, submitte

Social and Cultural Barriers to Diabetes Prevention in Oklahoma American Indian Women

INTRODUCTION: The prevalence of diabetes is disproportionately higher among minority populations, especially American Indians. Prevention or delay of diabetes in this population would improve quality of life and reduce health care costs. Identifying cultural definitions of health and diabetes is critically important to developing effective diabetes prevention programs. METHODS: In-home qualitative interviews were conducted with 79 American Indian women from 3 tribal clinics in northeast Oklahoma to identify a cultural definition of health and diabetes. Grounded theory was used to analyze verbatim transcripts. RESULTS: The women interviewed defined health in terms of physical functionality and absence of disease, with family members and friends serving as treatment promoters. Conversely, the women considered their overall health to be a personal issue addressed individually without burdening others. The women presented a fatalistic view of diabetes, regarding the disease as an inevitable event that destroys health and ultimately results in death. CONCLUSION: Further understanding of the perceptions of health in at-risk populations will aid in developing diabetes prevention programs

Semiclassical charged black holes with a quantized massive scalar field

Semiclassical perturbations to the Reissner-Nordstrom metric caused by the presence of a quantized massive scalar field with arbitrary curvature coupling are found to first order in \epsilon = \hbar/M^2. The DeWitt-Schwinger approximation is used to determine the vacuum stress-energy tensor of the massive scalar field. When the semiclassical perturbation are taken into account, we find extreme black holes will have a charge-to-mass ratio that exceeds unity, as measured at infinity. The effects of the perturbations on the black hole temperature (surface gravity) are studied in detail, with particular emphasis on near extreme ``bare'' states that might become precisely zero temperature ``dressed'' semiclassical black hole states. We find that for minimally or conformally coupled scalar fields there are no zero temperature solutions among the perturbed black holes.Comment: 19 pages; 1 figure; ReVTe

Testing the stability of fundamental constants with the 199Hg+ single-ion optical clock

Over a two-year duration, we have compared the frequency of the 199Hg+ 5d106s 2S 1/2 (F=0) 5d9 6s2 2D 5/2 (F=2) electric-quadrupole transition at 282 nm with the frequency of the ground-state hyperfine splitting in neutral 133Cs. These measurements show that any fractional time variation of the ratio nu(Cs)/nu(Hg) between the two frequencies is smaller than +/- 7 10^-15 / yr (1 sigma uncertainty). According to recent atomic structure calculations, this sets an upper limit to a possible fractional time variation of g(Cs) m_e / m_p alpha^6.0 at the same level.Comment: 4 pages with 3 figures. RevTeX 4, Submitted to Phys. Rev. Let