67 research outputs found

    Physical and Electrical Performance of Vapor–Solid Grown ZnO Straight Nanowires

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    Physical and electrical properties of wurtzitic ZnO straight nanowires grown via a vapor–solid mechanism were investigated. Raman spectrum shows four first-order phonon frequencies and a second-order Raman frequency of the ZnO nanowires. Electrical and photoconductive performance of individual ZnO straight nanowire devices was studied. The results indicate that the nanowires reported here are n-type semi-conductors and UV light sensitive, and a desirable candidate for fabricating UV light nanosensors and other applications

    Synthesis and White-Light Emission of ZnO/HfO2: Eu Nanocables

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    ZnO/HfO2:Eu nanocables were prepared by radio frequency sputtering with electrospun ZnO nanofibers as cores. The well-crystallized ZnO/HfO2:Eu nanocables showed a uniform intact core–shell structure, which consisted of a hexagonal ZnO core and a monoclinic HfO2 shell. The photoluminescence properties of the samples were characterized. A white-light band emission consisted of blue, green, and red emissions was observed in the nanocables. The blue and green emissions can be attributed to the zinc vacancy and oxygen vacancy defects in ZnO/HfO2:Eu nanocables, and the yellow–red emissions are derived from the inner 4f-shell transitions of corresponding Eu3+ ions in HfO2:Eu shells. Enhanced white-light emission was observed in the nanocables. The enhancement of the emission is ascribed to the structural changes after coaxial synthesis

    Genomic Organization and Expression Demonstrate Spatial and Temporal Hox Gene Colinearity in the Lophotrochozoan Capitella sp. I

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    Hox genes define regional identities along the anterior–posterior axis in many animals. In a number of species, Hox genes are clustered in the genome, and the relative order of genes corresponds with position of expression in the body. Previous Hox gene studies in lophotrochozoans have reported expression for only a subset of the Hox gene complement and/or lack detailed genomic organization information, limiting interpretations of spatial and temporal colinearity in this diverse animal clade. We studied expression and genomic organization of the single Hox gene complement in the segmented polychaete annelid Capitella sp. I. Total genome searches identified 11 Hox genes in Capitella, representing 11 distinct paralog groups thought to represent the ancestral lophotrochozoan complement. At least 8 of the 11 Capitella Hox genes are genomically linked in a single cluster, have the same transcriptional orientation, and lack interspersed non-Hox genes. Studying their expression by situ hybridization, we find that the 11 Capitella Hox genes generally exhibit spatial and temporal colinearity. With the exception of CapI-Post1, Capitella Hox genes are all expressed in broad ectodermal domains during larval development, consistent with providing positional information along the anterior–posterior axis. The anterior genes CapI-lab, CapI-pb, and CapI-Hox3 initiate expression prior to the appearance of segments, while more posterior genes appear at or soon after segments appear. Many of the Capitella Hox genes have either an anterior or posterior expression boundary coinciding with the thoracic–abdomen transition, a major body tagma boundary. Following metamorphosis, several expression patterns change, including appearance of distinct posterior boundaries and restriction to the central nervous system. Capitella Hox genes have maintained a clustered organization, are expressed in the canonical anterior–posterior order found in other metazoans, and exhibit spatial and temporal colinearity, reflecting Hox gene characteristics that likely existed in the protostome–deuterostome ancestor

    Ultrafast terahertz probes of transient conducting and insulating phases in an electron–hole gas

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    Many-body systems in nature exhibit complexity and self-organization arising from seemingly simple laws. The long-range Coulomb interaction between electrical charges generates a plethora of bound states in matter, ranging from the hydrogen atom to complex biochemical structures. Semiconductors form an ideal laboratory for studying many-body interactions of quasi-particles among themselves and with lattice vibrations and light. Oppositely charged electron and hole quasi-particles can coexist in an ionized but correlated plasma, or form bound hydrogen-like pairs called excitons which strongly affect physical properties. The pathways between such states however remain elusive in near-visible optical experiments that detect a subset of excitons with vanishing center-of-mass momenta. In contrast, transitions between internal exciton levels which occur in the far-infrared at terahertz (10 s) frequencies are in dependent of this restriction suggesting their use as a novel pro be of pair dynamics. Here, we employ an ultrafast terahertz probe to directly investigate the dynamical interplay of optically-generated excitons and unbound electron-hole pairs in GaAs quantum wells. Our observations witness an unexpected quasi-instantaneous excitonic enhancement, reveal formation of insulating excitons on a hundred picosecond timescale and manifest conditions under which excitonic populations prevail

    The Use of Laser Raman Spectroscopy in the Study of the Formation of Oxide Glasses

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    FEMTOSECOND TIME-RESOLVED 4-WAVE-MIXING FROM BIEXCITONS IN GAAS QUANTUM-WELLS - DOMINANCE OF THE INTERACTION-INDUCED SIGNAL

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    Time-resolved (TR) four-wave mixing (FWM) experiments are performed on a high-quality GaAs quantum-well sample where biexcitons make the dominant contribution under certain experimental conditions. TR-FWM peaks well after both beams passed through, regardless of relative contributions of biexcitons to FWM. Our experiments show that the diffraction of the interaction-induced field dominates FWM from biexcitons, as well as from excitons

    FEMTOSECOND-PULSE DISTORTION IN QUANTUM-WELLS

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    We show that a low-intensity femtosecond pulse is severely distorted while propagating through a relatively thin (<7000 ($) over circle A) GaAs multiple-quantum-well sample and that this pulse distortion depends critically on the dephasing time T-2 and the total thickness l. An interferometric measurement reveals the existence of well-defined nodes at which the envelope function changes its sign. This pulse distortion significantly affects femtosecond experiments such as pump-probe or four-wave-mixing experiments

    CARRIER-CARRIER SCATTERING IN A DEGENERATE ELECTRON-SYSTEM - STRONG INHIBITION OF SCATTERING NEAR THE FERMI EDGE

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    We report the first direct measurement of carrier-carrier scattering rates in a degenerate electron system. Our results on modulation-doped quantum wells, using femtosecond four-wave-mixing (FWM) techniques, demonstrate a strong inhibition of scattering near the Fermi edge, and exhibit other behavior predicted by Landau Fermi liquid theory. Time-resolved (100 fs) FWM measurements clearly show photon echoes, demonstrating the inhomogeneous character of this intrinsic system, as well as prompt signals arising from many-body effects
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