619 research outputs found
Effects of Rattling Phonons on the Quasiparticle Excitation and Dynamics in the Superconducting -Pyrochlore KOsO
Microwave penetration depth and surface resistance at 27 GHz are
measured in high quality crystals of KOsO. Firm evidence for
fully-gapped superconductivity is provided from . Below the second
transition at K, the superfluid density shows a step-like
change with a suppression of effective critical temperature .
Concurrently, the extracted quasiparticle scattering time shows a steep
enhancement, indicating a strong coupling between the anomalous rattling motion
of K ions and quasiparticles. The results imply that the rattling phonons help
to enhance superconductivity, and that K sites freeze to an ordered state with
long quasiparticle mean free path below .Comment: 5 pages, 5 figures, to be published in Phys. Rev. Let
Vortex Redistribution below the First-Order Transition Temperature in the \beta-Pyrochlore Superconductor KOs_2O_6
A miniature Hall sensor array was used to detect magnetic induction locally
in the vortex states of the -pyrochlore superconductor KOsO.
Below the first-order transition at K, which is associated
with a change in the rattling motion of K ions, the lower critical field and
the remanent magnetization both show a distinct decrease, suggesting that the
electron-phonon coupling is weakened below the transition. At high magnetic
fields, the local induction shows an unexpectedly large jump at
whose sign changes with position inside the sample. Our results demonstrate a
novel redistribution of vortices whose energy is reduced abruptly below the
first-order transition at .Comment: 5 pages, 4 figures, to be published in Phys. Rev. Let
Local spin and charge properties of beta-Ag0.33V2O5 studied by 51V NMR
Local spin and charge properties were studied on beta-Ag0.33V2O5, a
pressure-induced superconductor, at ambient pressure using 51V-NMR and
zero-field-resonance (ZFR) techniques. Three inequivalent Vi sites (i=1, 2, and
3) were identified from 51V-NMR spectra and the principal axes of the
electric-field-gradient (EFG) tensor were determined in a metallic phase and
the following charge-ordering phase. We found from the EFG analysis that the V1
sites are in a similar local environment to the V3 sites. This was also
observed in ZFR spectra as pairs of signals closely located with each other.
These results are well explained by a charge-sharing model where a 3d1 electron
is shared within a rung in both V1-V3 and V2-V2 two-leg ladders.Comment: 12pages, 16figure
Upper critical field and de Haas-van Alphen oscillations in KOsO measured in a hybrid magnet
Magnetic torque measurements have been performed on a KOsO single
crystal in magnetic fields up to 35.3 T and at temperatures down to 0.6 K. The
upper critical field is determined to be 30 T. De Haas-van Alphen
oscillations are observed. A large mass enhancement of (1+) = = 7.6 is found. It is suggested that, for the large upper critical
field to be reconciled with Pauli paramagnetic limiting, the observed mass
enhancement must be of electron-phonon origin for the most part.Comment: 4 pages, 4 figures, published versio
Crystal growth, structural studies and superconducting properties of beta-pyrochlore KOs2O6
Single crystals of KOs2O6 have been grown in a sealed quartz ampoule.
Detailed single crystal X-ray diffraction studies at room temperature show
Bragg peaks that violate Fd-3m symmetry. With a comparative structure
refinement the structure is identified as non-centrosymmetric (F-43m). Compared
to the ideal beta-pyrochlore lattice (Fd-3m), both Os tetrahedral and O
octahedral network exhibit breathing mode like volume changes accompanied by
strong anisotropic character of the K channels. The crystals show metallic
conductivity and a sharp transition to the superconducting state at Tc = 9.65
K. Superconducting properties have been investigated by magnetization
measurements performed in a temperature range from 2 to 12 K and in magnetic
fields from 0 to 60 kOe. The temperature dependence of the upper critical field
Hc2(T) has been determined and the initial slope (dHc2/dT)Tc = -33.3 kOe/K has
been obtained near Tc. The upper critical field at zero temperature was
estimated to be Hc2(0) \cong 230 kOe, which is a value close to the Pauli
paramagnetic limiting field Hp(0)\cong 250 kOe. Then, the Ginzburg-Landau (GL)
coherence length xi GL(0) \approx 3.8 nm was calculated, and the Maki parameter
alpha \approx \sqrt 2 was obtained, suggesting the possibility that KOs2O6
might behave unconventionally at low temperatures and high magnetic fields
Green's function of fully anharmonic lattice vibration
Motivated by the discovery of superconductivity in beta-pyrochlore oxides, we
study property of rattling motion coupled with conduction electrons. We derive
the general expression of the Green's function of fully anharmonic lattice
vibration within the accuracy of the second order perturbation of electron-ion
interaction by introducing self-energy, vertex-correction, and normalization
factor for each transition. Using the expression, we discuss the characteristic
properties of the spectral function in the entire range from weakly anharmonic
potential to double-well case, and calculate NMR relaxation rate due to the two
phonon Raman process
Investigation of the ferromagnetic transition in the correlated 4d perovskites SrRuRhO
The solid-solution SrRuRhO () is a
variable-electron-configuration system forming in the nearly-cubic-perovskite
basis, ranging from the ferromagnetic 4 to the enhanced paramagnetic
4. Polycrystalline single-phase samples were obtained over the whole
composition range by a high-pressure-heating technique, followed by
measurements of magnetic susceptibility, magnetization, specific heat,
thermopower, and electrical resistivity. The ferromagnetic order in long range
is gradually suppressed by the Rh substitution and vanishes at .
The electronic term of specific-heat shows unusual behavior near the critical
Rh concentration; the feature does not match even qualitatively with what was
reported for the related perovskites (Sr,Ca)RuO. Furthermore, another
anomaly in the specific heat was observed at .Comment: Accepted for publication in PR
Crystal Structure and Magnetism of the Linear-Chain Copper Oxides Sr5Pb3-xBixCuO12
The title quasi-1D copper oxides (0=< x =<0.4) were investigated by neutron
diffraction and magnetic susceptibility studies. Polyhedral CuO4 units in the
compounds were found to comprise linear-chains at inter-chain distance of
approximately 10 A. The parent chain compound (x = 0), however, shows less
anisotropic magnetic behavior above 2 K, although it is of substantially
antiferromagnetic (mu_{eff}= 1.85 mu_{B} and Theta_{W} = -46.4 K) spin-chain
system. A magnetic cusp gradually appears at about 100 K in T vs chi with the
Bi substitution. The cusp (x = 0.4) is fairly characterized by and therefore
suggests the spin gap nature at Delta/k_{B} ~ 80 K. The chain compounds hold
electrically insulating in the composition range.Comment: To be published in PR
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