Rotational quenching rate coefficients for H_2 in collisions with H_2 from 2 to 10,000 K

Rate coefficients for rotational transitions in H_2 induced by H_2 impact are presented. Extensive quantum mechanical coupled-channel calculations based on a recently published (H_2)_2 potential energy surface were performed. The potential energy surface used here is presumed to be more reliable than surfaces used in previous work. Rotational transition cross sections with initial levels J <= 8 were computed for collision energies ranging between 0.0001 and 2.5 eV, and the corresponding rate coefficients were calculated for the temperature range 2 < T <10,000 K. In general, agreement with earlier calculations, which were limited to 100-6000 K, is good though discrepancies are found at the lowest and highest temperatures. Low-density-limit cooling functions due to para- and ortho-H_2 collisions are obtained from the collisional rate coefficients. Implications of the new results for non-thermal H_2 rotational distributions in molecular regions are also investigated

Rotational Quenching Rate Coefficients for H\u3csub\u3e2\u3c/sub\u3e in Collisions with H\u3csub\u3e2\u3c/sub\u3e from 2 to 10,000 K

Rate coefficients for rotational transitions in H2 induced by H2 impact are presented. Extensive quantum mechanical coupled-channel calculations based on a recently published (H2)2 potential energy surface were performed. The potential energy surface used here has been demonstrated to be more reliable than surfaces used in previous work. Rotational transition cross sections with initial levels of J≤8 were computed for collision energies ranging between 10-4 and 2.5 eV, and the corresponding rate coefficients were calculated for the temperature range 2≤T≤10,000 K. In general, agreement with earlier calculations, which were limited to 100-6000 K, is good, although discrepancies are found at the lowest and highest temperatures. Low-density-limit cooling functions due to para- and ortho-H2 collisions are obtained from the collisional rate coefficients. Implications of the new results for nonthermal H2 rotational distributions in molecular regions are also investigated

Study of strong photon-magnon coupling in a YIG-film split-ring resonant system

By using the stripline Microwave Vector Network Analyzer Ferromagnetic Resonance and Pulsed Inductive Microwave Magnetometry spectroscopy techniques, we study a strong coupling regime of magnons to microwave photons in the planar geometry of a lithographically formed split-ring resonator (SRR) loaded by a single-crystal epitaxial yttrium-iron garnet (YIG) film. Strong anti-crossing of the photon modes of SRR and of the magnon modes of the YIG film is observed in the applied-magnetic-field resolved measurements. The coupling strength extracted from the experimental data reaches 9 percent at 3 GHz. Theoretically, we propose an equivalent circuit model of an SRR loaded by a magnetic film. This model follows from the results of our numerical simulations of the microwave field structure of the SRR and of the magnetization dynamics in the YIG film driven by the microwave currents in the SRR. The equivalent circuit model is in good agreement with the experiment. It provides a simple physical explanation of the process of mode anti-crossing. Our findings are important for future applications in microwave quantum photonic devices as well as in magnetically tunable metamaterials exploiting the strong coupling of magnons to microwave photons

Close-coupling calculations of low-energy inelastic and elastic processes in 4^4He collisions with H2_2: A comparative study of two potential energy surfaces

The two most recently published potential energy surfaces (PESs) for the HeH$_2$ complex, the so-called MR (Muchnick and Russek) and BMP (Boothroyd, Martin, and Peterson) surfaces, are quantitatively evaluated and compared through the investigation of atom-diatom collision processes. The BMP surface is expected to be an improvement, approaching chemical accuracy, over all conformations of the PES compared to that of the MR surface. We found significant differences in inelastic rovibrational cross sections computed on the two surfaces for processes dominated by large changes in target rotational angular momentum. In particular, the H$_2$($\nu=1, j=0$) total quenching cross section computed using the BMP potential was found to be a factor of $~$1000 larger than that obtained with the MR surface.Comment: 26 pages, 11 figure

ROVIBRATIONAL QUENCHING RATE COEFFICIENTS OF HD IN COLLISIONS WITH He

ABSTRACT Along with H 2 , HD has been found to play an important role in the cooling of the primordial gas for the formation of the first stars and galaxies. It has also been observed in a variety of cool molecular astrophysical environments. The rate of cooling by HD molecules requires knowledge of collisional rate coefficients with the primary impactors, H, He, and H 2 . To improve knowledge of the collisional properties of HD, we present rate coefficients for the He-HD collision system over a range of collision energies from 10 −5 to 5 × 10 3 cm −1 . Fully quantum mechanical scattering calculations were performed for initial HD rovibrational states of j = 0 and 1 for v = 0-17 which utilized accurate diatom rovibrational wave functions. Rate coefficients of all Δv = 0, −1, and −2 transitions are reported. Significant discrepancies with previous calculations, which adopted a small basis and harmonic HD wave functions for excited vibrational levels, were found for the highest previously considered vibrational state of v = 3. Applications of the He-HD rate coefficients in various astrophysical environments are briefly discussed

Limits on decaying dark energy density models from the CMB temperature-redshift relation

The nature of the dark energy is still a mystery and several models have been proposed to explain it. Here we consider a phenomenological model for dark energy decay into photons and particles as proposed by Lima (J. Lima, Phys. Rev. D 54, 2571 (1996)). He studied the thermodynamic aspects of decaying dark energy models in particular in the case of a continuous photon creation and/or disruption. Following his approach, we derive a temperature redshift relation for the CMB which depends on the effective equation of state $w_{eff}$ and on the "adiabatic index" $\gamma$. Comparing our relation with the data on the CMB temperature as a function of the redshift obtained from Sunyaev-Zel'dovich observations and at higher redshift from quasar absorption line spectra, we find $w_{eff}=-0.97 \pm 0.034$, adopting for the adiabatic index $\gamma=4/3$, in good agreement with current estimates and still compatible with $w_{eff}=-1$, implying that the dark energy content being constant in time.Comment: 8 pages, 1 figur

HD/H2 Molecular Clouds in the Early Universe: The Problem of Primordial Deuterium

We have detected new HD absorption systems at high redshifts, z_abs=2.626 and z_abs=1.777, identified in the spectra of the quasars J0812+3208 and Q1331+170, respectively. Each of these systems consists of two subsystems. The HD column densities have been determined: log(N(HD),A)=15.70+/-0.07 for z_A=2.626443(2) and log(N(HD),B)=12.98+/-0.22 for z_B=2.626276(2) in the spectrum of J0812+3208 and log(N(HD),C)=14.83+/-0.15 for z_C=1.77637(2) and log(N(HD),D)=14.61+/-0.20 for z_D=1.77670(3) in the spectrum of Q1331+170. The measured HD/H2 ratio for three of these subsystems has been found to be considerably higher than its values typical of clouds in our Galaxy. We discuss the problem of determining the primordial deuterium abundance, which is most sensitive to the baryon density of the Universe \Omega_{b}. Using a well-known model for the chemistry of a molecular cloud, we have estimated the isotopic ratio D/H=HD/2H_2=(2.97+/-0.55)x10^{-5} and the corresponding baryon density \Omega_{b}h^2=0.0205^{+0.0025}_{-0.0020}. This value is in good agreement with \Omega_{b}h^2=0.0226^{+0.0006}_{-0.0006} obtained by analyzing the cosmic microwave background radiation anisotropy. However, in high-redshift clouds, under conditions of low metallicity and low dust content, hydrogen may be incompletely molecularized even in the case of self-shielding. In this situation, the HD/2H_2 ratio may not correspond to the actual D/H isotopic ratio. We have estimated the cloud molecularization dynamics and the influence of cosmological evolutionary effects on it

Composite excitation of Josephson phase and spin waves in Josephson junctions with ferromagnetic insulator

Coupling of Josephson-phase and spin-waves is theoretically studied in a superconductor/ferromagnetic insulator/superconductor (S/FI/S) junction. Electromagnetic (EM) field inside the junction and the Josephson current coupled with spin-waves in FI are calculated by combining Maxwell and Landau-Lifshitz-Gilbert equations. In the S/FI/S junction, it is found that the current-voltage (I-V) characteristic shows two resonant peaks. Voltages at the resonant peaks are obtained as a function of the normal modes of EM field, which indicates a composite excitation of the EM field and spin-waves in the S/FI/S junction. We also examine another type of junction, in which a nonmagnetic insulator (I) is located at one of interfaces between S and FI. In such a S/I/FI/S junction, three resonant peaks appear in the I-V curve, since the Josephson-phase couples to the EM field in the I layer.Comment: 16 pages, 5 figure