46 research outputs found
Zn and Ni doping effects on the low-energy spin excitations in LaSrCuO
Impurity effects of Zn and Ni on the low-energy spin excitations were
systematically studied in optimally doped La1.85Sr0.15Cu1-yAyO4 (A=Zn, Ni) by
neutron scattering. Impurity-free La1.85Sr0.15CuO4 shows a spin gap of 4meV
below Tc in the antiferromagnetic(AF) incommensurate spin excitation. In
Zn:y=0.004, the spin excitation shows a spin gap of 3meV below Tc. In
Zn:y=0.008 and Zn:y=0.011, however, the magnetic signals at 3meV decrease below
Tc and increase again at lower temperature, indicating an in-gap state. In
Zn:y=0.017, the low-energy spin state remains unchanged with decreasing
temperature, and elastic magnetic peaks appear below 20K then exponentially
increase. As for Ni:y=0.009 and Ni:y=0.018, the low-energy excitations below
3meV and 2meV disappear below Tc. The temperature dependence at 3meV, however,
shows no upturn in constrast with Zn:y=0.008 and Zn:y=0.011, indicating the
absence of in-gap state. In Ni:y=0.029, the magnetic signals were observed also
at 0meV. Thus the spin gap closes with increasing Ni. Furthermore, as omega
increases, the magnetic peak width broadens and the peak position, i.e.
incommensurability, shifts toward the magnetic zone center (pi pi). We
interpret the impurity effects as follows: Zn locally makes a
non-superconducting island exhibiting the in-gap state in the superconducting
sea with the spin gap. Zn reduces the superconducting volume fraction, thus
suppressing Tc. On the other hand, Ni primarily affects the superconducting
sea, and the spin excitations become more dispersive and broaden with
increasing energy, which is recognized as a consequence of the reduction of
energy scale of spin excitations. We believe that the reduction of energy scale
is relevant to the suppression of Tc.Comment: 13pages, 14figures; submitted to Phys. Rev.
Oxygen Phonon Branches in Detwinned YBa2Cu3O7
We report results of inelastic neutron scattering measurements of phonon
dispersions on a detwinned sample of YBaCu3O7 and compare them with model
calculations. Plane oxygen bond stretching phonon branches disperse steeply
downwards from the zone center in both the a and the b direction indicating a
strong electron-phonon coupling. Half way to the zone boundary, the phonon
peaks become ill-defined but we see no need to invoke unit cell doubling or
charge stripe formation: lattice dynamical shell model calculations predict
such behavior as a result of branch anticrossings. There were no observable
superconductivity-related temperature effects on selected plane oxygen bond
stretching modes measured on a twinned sample.Comment: 5 pages, 3 figures, To appear in Journal of Low Temperature Physics
(Proceedings of MOS2002; Revised version (1) with many changes throughout the
tex
Renormalization of Commensurate Magnetic Peak in Ni-doped LaSrCuO
We have studied the magnetic excitations in impurity doped
LaSrCuAO (A=Ni or Zn) by neutron
scattering. The dispersion for Zn: is similar to that for the impurity
free sample: incommensurate peaks with the incommensurability
(rlu) do not change their positions up to 21 meV. On the
other hand, for Ni:, two incommensurate peaks observed at low energies
suddenly change into a broad commensurate peak at meV.
Compared to the impurity free sample with a similar Sr-concentration ,
[B. Vignolle {\it et al.} Nature Physics {\bf 3} (2007) 163],
for Ni: is decreased by nearly the same factor for
the reduction in . This is very similar to the shift of the resonance
energy () in Ni-doped YBaCuO.[Y. Sidis {\it
et al.}: Phys. Rev. Lett. {\bf 84} (2000) 5900]. These common impurity effects
on the shift of and suggest the same
magnetic origin for the resonance peak in YBaCuO and
that for a crossing point of upward and downward dispersions in the
LaSrCuO. We propose that the sudden change in the
dispersion is better described by a crossover from incommensurate spin
fluctuations to a gapped spin wave rather than a hourglass-like dispersion.Comment: 11 pages, 5 figure
Change of the Ground State upon Hole Doping Unveiled by Ni Impurity in High- Cuprates
The electronic ground state in high- cuprates where the
superconducting state is suppressed by Ni substitution has been investigated in
LaSrCuNiO from the specific heat and muon spin
relaxation measurements. It has been found that the ground state changes from a
magnetically ordered state with the strong hole-trapping by Ni to a metallic
state with the Kondo effect of Ni with increasing hole-concentration. Moreover,
the analysis of the results has revealed that a phase separation into the
magnetically ordered phase and the metallic phase occurs around the boundary of
two phases.Comment: 11pages, 4 figure
Spin Pseudo Gap in La2-xSrxCuO4 Studied by Neutron Scattering
Spin excitations of La2-xSrxCuO have been studied using inelastic neutron
scattering techniques in the energy range of 2 meV =< w =< 12 meV and the
temperature range of 8 K =< T =< 150 K. We observed a signature of a spin
pseudo gap in the excitation spectrum above Tc for the slightly overdoped
sample with x = 0.18. On heating, the spin pseudo gap gradually collapses
between T = 80 K and 150 K. For the x = 0.15 and 0.20, although the visibility
of gap-like structure at T ~ Tc is lower compared to the x = 0.18 sample, the
broad bump of kai"(w) appears at w ~ 5 meV,close to the spin-gap energy at base
temperature, suggests the existence of the spin pseudo gap in the normal state.Comment: revtex, 7 pages, 8 eps figures, PRB (2003) in pres
Incommensurate spin correlations induced by magnetic Fe ions substituted into overdoped Bi1.75Pb0.35Sr1.90CuO6+z
Spin correlations in the overdoped region of Bi1.75Pb0.35Sr1.90CuO6+z have
been explored with Fe-doped single crystals characterized by neutron
scattering, muon-spin-rotation (muSR) spectroscopy, and magnetic susceptibility
measurements. Static incommensurate spin correlations induced by the Fe spins
are revealed by elastic neutron scattering. The resultant incommensurability
delta is unexpectedly large (~0.2 r.l.u.), as compared with delta ~ 1/8 in
overdoped superconductor La2-xSrxCuO4. Intriguingly, the large delta in this
overdoped region is close to the hole concentration p. This result is
reminiscent of the delta ~ p trend observed in underdoped La2-xSrxCuO4;
however, it is inconsistent with the saturation of delta in the latter compound
in the overdoped regime. While our findings in Fe-doped
Bi1.75Pb0.35Sr1.90CuO6+z support the commonality of incommensurate spin
correlations in high-Tc cuprate superconductors, they also suggest that the
magnetic response might be dominated by a distinct mechanism in the overdoped
region.Comment: 4 pages, 5 figures. Revision in introduction, discussion, and
conclusion
Magnetization under High Pressure in MnSi
The magnetization M(H) has been measured in the weakly helimagnetic itinerant
compound MnSi under high pressure up to 10.2 kbar and high magnetic field up to
9 Tesla. We interpret the simultaneous decrease under pressure of the saturated
magnetization, , and the Curie temperature, in the frame of the
self-consistent renormalization theory (SCR) of spin fluctuations. From the
analysis of the so-called Arrot-plot ( versus ) and
the respective volume dependence of and , we estimate the evolution
of the characteristic spin fluctuation temperatures, and when the
system approaches its critical pressure, =15 kbar, corresponding to the
disappearance of the long range magnetic order at T=0.Comment: 12 pages, 5 figures. Submitted to Phys. Rev.