Ab initio calculation of the binding energy of impurities in semiconductors: Application to Si nanowires

We discuss the binding energy E_b of impurities in semiconductors within density functional theory (DFT) and the GW approximation, focusing on donors in nanowires as an example. We show that DFT succeeds in the calculation of E_b from the Kohn-Sham (KS) hamiltonian of the ionized impurity, but fails in the calculation of E_b from the KS hamiltonian of the neutral impurity, as it misses most of the interaction of the bound electron with the surface polarization charges of the donor. We trace this deficiency back to the lack of screened exchange in the present functionals

Study of Phase Reconstruction Techniques applied to Smith-Purcell Radiation Measurements

Measurements of coherent radiation at accelerators typically give the absolute value of the beam profile Fourier transform but not its phase. Phase reconstruction techniques such as Hilbert transform or Kramers Kronig reconstruction are used to recover such phase. We report a study of the performances of these methods and how to optimize the reconstructed profiles.Comment: Presented at IPAC'14 - THPME08

Effect of Compton Scattering on the Electron Beam Dynamics at the ATF Damping Ring

Compton scattering provides one of the most promising scheme to obtain polarized positrons for the next generation of $e^-$ -- $e^+$ colliders. Moreover it is an attractive method to produce monochromatic high energy polarized gammas for nuclear applications and X-rays for compact light sources. In this framework a four-mirror Fabry-P\'erot cavity has been installed at the Accelerator Test Facility (ATF - KEK, Tsukuba, Japan) and is used to produce an intense flux of polarized gamma rays by Compton scattering \cite{ipac-mightylaser}. For electrons at the ATF energy (1.28 GeV) Compton scattering may result in a shorter lifetime due to the limited bucket acceptance. We have implemented the effect of Compton scattering on a 2D tracking code with a Monte-Carlo method. This code has been used to study the longitudinal dynamics of the electron beam at the ATF damping ring, in particular the evolution of the energy spread and the bunch length under Compton scattering. The results obtained are presented and discussed. Possible methods to observe the effect of Compton scattering on the ATF beam are proposed

Beam Profile Measurements and Simulations of the PETRA Laser-Wire

The Laser-wire will be an essential diagnostic tool at the International Linear Collider. It uses a finely focussed laser beam to measure the transverse profile of electron bunches by detecting the Compton-scattered photons (or degraded electrons) downstream of where the laser beam intersects the electron beam. Such a system has been installed at the PETRA storage ring at DESY, which uses a piezo-driven mirror to scan the laser-light across the electron beam. Lat- est results of experimental data taking are presented and compared to detailed simulations using the Geant4 based program BDSIM.Comment: 3 pagesm 4 figures. Submitted as a conference paper for the Particle Accelerator Conference 2005 (PAC05

Simulations and Studies of Electron Beam Dynamics under Compton Back-scattering for the Compact X-ray Source ThomX

MOPWO004 - ISBN 978-3-95450-122-9International audienceIn this article are presented beam dynamics investiga- tions of a relativistic electron bunch in the compact storage ring ThomX (50 MeV), which is under construction at LAL to produce hard X-ray using Compton Back-Scattering (CBS). The effect of CBS has been implemented in a 6D tracking code. In addition to CBS, the influence of lattice non linearities and various collective effects on the flux of scattered Compton photons is investigated

Some theoretical results on semiconductor spherical quantum dots

We use an improved version of the standard effective mass approximation model to describe quantum effects in nanometric semiconductor Quantum Dots (QDs). This allows analytic computation of relevant quantities to a very large extent. We obtain, as a function of the QD radius, in precise domains of validity, the QD excitonic ground state energy and its Stark and Lamb shifts. Finally, the Purcell effect in QDs is shown to lead to potential QD-LASER emitting in the range of visible light

Size-Dependence of the Wavefunction of Self-Assembled Quantum Dots

The radiative and non-radiative decay rates of InAs quantum dots are measured by controlling the local density of optical states near an interface. From time-resolved measurements we extract the oscillator strength and the quantum efficiency and their dependence on emission energy. From our results and a theoretical model we determine the striking dependence of the overlap of the electron and hole wavefunctions on the quantum dot size. We conclude that the optical quality is best for large quantum dots, which is important in order to optimally tailor quantum dot emitters for, e.g., quantum electrodynamics experiments.Comment: 5 pages, 3 figure

Quasiparticle energies for large molecules: a tight-binding GW approach

We present a tight-binding based GW approach for the calculation of quasiparticle energy levels in confined systems such as molecules. Key quantities in the GW formalism like the microscopic dielectric function or the screened Coulomb interaction are expressed in a minimal basis of spherically averaged atomic orbitals. All necessary integrals are either precalculated or approximated without resorting to empirical data. The method is validated against first principles results for benzene and anthracene, where good agreement is found for levels close to the frontier orbitals. Further, the size dependence of the quasiparticle gap is studied for conformers of the polyacenes ($C_{4n+2}H_{2n+4}$) up to n = 30.Comment: 10 pages, 5 eps figures submitted to Phys. Rev.

Effect of Compton Scattering on the Electron Beam Dynamics at the ATF Damping Ring

Compton scattering provides one of the most promising scheme to obtain polarized positrons for the next generation of $e^-$ -- $e^+$ colliders. Moreover it is an attractive method to produce monochromatic high energy polarized gammas for nuclear applications and X-rays for compact light sources. In this framework a four-mirror Fabry-P\'erot cavity has been installed at the Accelerator Test Facility (ATF - KEK, Tsukuba, Japan) and is used to produce an intense flux of polarized gamma rays by Compton scattering \cite{ipac-mightylaser}. For electrons at the ATF energy (1.28 GeV) Compton scattering may result in a shorter lifetime due to the limited bucket acceptance. We have implemented the effect of Compton scattering on a 2D tracking code with a Monte-Carlo method. This code has been used to study the longitudinal dynamics of the electron beam at the ATF damping ring, in particular the evolution of the energy spread and the bunch length under Compton scattering. The results obtained are presented and discussed. Possible methods to observe the effect of Compton scattering on the ATF beam are proposed

Voltammetric Oxidation of Drugs of Abuse II. Codeine and Metabolites

The oxidation of codeine on glassy carbon electrodes has been studied in detail using differential pulse voltammetry. The results obtained using a glassy carbon electrode clearly show a much more complex oxidation mechanism than that previously reported when platinum and gold electrodes were used. To clarify the codeine oxidative profile, several metabolites and analogues of this alkaloid, codeine N-oxide, norcodeine, dihydrocodeine, acetylcodeine and 6-chlorodesoxycodeine, were synthesized and studied. It was deduced that the anodic waves observed in codeine oxidation are related to the presence of methoxy, hydroxy and tertiary amine groups. Due to the similarity of potentials at which these oxidative processes take place, at some pHs an overlap of peaks occurs and only one anodic wave is observed