154 research outputs found
Anomalous temperature behavior of resistivity in lightly doped manganites around a metal-insulator phase transition
An unusual temperature and concentration behavior of resistivity in
has been observed at slight doping
(). Namely, introduction of copper results in a splitting of
the resistivity maximum around a metal-insulator transition temperature
into two differently evolving peaks. Unlike the original -free
maximum which steadily increases with doping, the second (satellite) peak
remains virtually unchanged for , increases for and finally
disappears at with . The observed phenomenon
is thought to arise from competition between substitution induced strengthening
of potential barriers (which hamper the charge hopping between neighboring
sites) and weakening of carrier's kinetic energy. The data are well fitted
assuming a nonthermal tunneling conductivity theory with randomly distributed
hopping sites.Comment: 10 REVTEX pages, 2 PostScript figures (epsf.sty); to be published in
JETP Letter
Modification of the ground state in Sm-Sr manganites by oxygen isotope substitution
The effect of O O isotope substitution on electrical
resistivity and magnetic susceptibility of SmSrMnO manganites
is analyzed. It is shown that the oxygen isotope substitution drastically
affects the phase diagram at the crossover region between the ferromagnetic
metal state and that of antiferromagnetic insulator (0.4 0.6), and
induces the metal-insulator transition at for = 0.475 and 0.5. The nature
of antiferromagnetic insulator phase is discussed.Comment: 4 pages, 3 eps figures, RevTeX, submitted to Phys. Rev. Let
Theory of Insulator Metal Transition and Colossal Magnetoresistance in Doped Manganites
The persistent proximity of insulating and metallic phases, a puzzling
characterestic of manganites, is argued to arise from the self organization of
the twofold degenerate e_g orbitals of Mn into localized Jahn-Teller(JT)
polaronic levels and broad band states due to the large electron - JT phonon
coupling present in them. We describe a new two band model with strong
correlations and a dynamical mean-field theory calculation of equilibrium and
transport properties. These explain the insulator metal transition and colossal
magnetoresistance quantitatively, as well as other consequences of two state
coexistence
Quenched disorder induced magnetization jumps in (Sm,Sr)MnO
Magnetic field induced step-like changes in magnetization and resistivity of
SmSr manganites were studied. A strong dependence of these features on the
cooling rate was observed. Magnetostriction, however, does not show the
presence of large strain in our samples. From all these features we can rule
out the conventional explanation of magnetization jumps as a consequence of
martensitic transition. We propose instead that quenched by fast cooling
disorder leads to the formation of an inhomogeneous metastable state and to
subsequent magnetization jumps.Comment: 4 pages, 4 figures, to be published in PRB Brief
Surface morphology of DyxOy films grown on Si
The crystalline structure and surface morphology of DyxOy dielectric films grown on Si substrates were studied by grazing incidence diffraction and absorption with use of synchrotron radiation and by atomic force microscopy. The crystalline structure and the roughness of DyxOy films were found to be strongly dependent on the deposition rate. The dielectric-silicon interface depends on the type of gas used in the annealing process. Moreover. results from the near edge X-ray absorption studies, have revealed that none of the examined films has a stoichiometry close to the Dy2O3. The level of stoichiometry is determined by the technological conditions. Nevertheless, MOS structures with Dy(x)Q(y) films (EOT similar to 23 angstrom) have shown a rather good DyxOy-Si interface properties, which can be further improve by thermal annealing, and introducing of several additives, therefore DyxOy films can be considered as suitable candidates for gate dielectric in MOS devices. (c) 2006 Elsevier B.V. All rights reserved
Oxygen isotope effect and phase separation in the optical conductivity of (LaPr)CaMnO thin films
The optical conductivities of films of
(LaPr)CaMnO with different oxygen isotopes
(O and O) have been determined in the spectral range from 0.3 to
4.3 eV using a combination of transmission in the mid-infrared and ellipsometry
from the near-infrared to ultra-violet regions. We have found that the isotope
exchange strongly affects the optical response in the ferromagnetic phase in a
broad frequency range, in contrast to the almost isotope-independent optical
conductivity above . The substitution by O strongly suppresses the
Drude response and a mid-infrared peak while enhancing the conductivity peak at
1.5 eV. A qualitative explanation can be given in terms of the phase separation
present in these materials. Moreover, the optical response is similar to the
one extracted from measurements in polished samples and other thin films, which
signals to the importance of internal strain.Comment: 11 pages, 11 figures, to appear in PR
Novel electronic states close to Mott transition in low-dimensional and frustrated systems
Recent studies demonstrated that there may appear different novel states in
correlated systems close to localized-itinerant crossover. Especially
favourable conditions for that are met in low-dimensional and in frustrated
systems. In this paper I discuss on concrete examples some of such novel
states. In particular, for some spinels and triangular systems there appears a
"partial Mott transition", in which first some finite clusters (dimers, trimes,
tetramers, heptamers) go over to the itinerant regime, and the real bulk Mott
transition occurs only later. Also some other specific possibilities in this
crossover regime are shortly discussed, such as spin-Peierls-Peierls transition
in TiOCl, spontaneous charge disproportionation in some cases, etc.Comment: To be published in Journal of Physics - Condensed Matter, conference
serie
Phase diagram and isotope effect in (PrEu)_0.7Ca_0.3CoO_3 cobaltites exhibiting spin-state transitions
We present the study of magnetization, thermal expansion, specific heat,
resistivity, and a.c. susceptibility of
(PrEu)CaCoO cobaltites. The measurements were
performed on ceramic samples with and . Based on these
results, we construct the phase diagram, including magnetic and spin-state
transitions. The transition from the low- to intermediate-spin state is
observed for the samples with , whereas for a lower Eu-doping level,
there are no spin-state transitions, but a crossover between the ferromagnetic
and paramagnetic states occurs. The effect of oxygen isotope substitution along
with Eu doping on the magnetic/spin state is discussed. The oxygen-isotope
substitution (O by O) is found to shift both the magnetic and
spin-state phase boundaries to lower Eu concentrations. The isotope effect on
the spin-state transition temperature () is rather strong, but it is
much weaker for the transition to a ferromagnetic state (). The
ferromagnetic ordering in the low-Eu doped samples is shown to be promoted by
the Co ions, which favor the formation of the intermediate-spin state of
neighboring Co ions.Comment: 13 pages, including 11 figures, to be published in Phys. Rev.
Phytosanitary features of pea morphotypes under the conditions of the Tyumen region
The selection material and finished varieties of peas for sowing different morphotypes of the grain direction were assessed for the formation of a phytosanitary state and productivity, and the effectiveness of protection methods. During the growing season, leaf and stem diseases were observed with varying degrees of development and timing of manifestation (p. Ascochyta, p. Uromyces, p. Erysiphe communis G) with development depending on the year and genus of the pathogen from 0.2-40%. The development of the river. Ascochyta - 10-20%, r. Erysiphe - 11-49%, p. Uromyces - 0.2-20%. Some resistance was determined in 22% of varieties p. Erysiphe communis G., 11% p. Ascochyta and 14% p. Uromyces. The yield for the period of study of pea varieties of the sowing grain direction varied from 3.2 to 4.6 t/ha, stable yields in the morphogroup chameleon with an increase of 0.64 t/ha or 17% to the standard. Protection of peas requires mandatory pre-sowing treatment with a chemical disinfectant, a biological preparation with the inclusion of an agrochemical in the mixture, which contributes to the development of the root system, activation of growth vigor, and a 70-90% reduction in pathogenic fungi on seeds and roots. Fungicidal protection in the budding phase - the formation of beans contributed to the preservation of the crop by 0.3-0.4 t/ha
Isotope effects in underdoped cuprate superconductors: a quantum phenomenon
We show that the unusual doping dependence of the isotope effects on
transition temperature and zero temperature in - plane penetration depth
naturally follows from the doping driven 3D-2D crossover, the 2D quantum
superconductor to insulator transition (QSI) in the underdoped limit and the
change of the relative doping concentration upon isotope substitution. Close to
the QSI transition both, the isotope coefficient of transition temperature and
penetration depth approach the coefficient of the relative dopant
concentration, and its divergence sets the scale. These predictions are fully
consistent with the experimental data and imply that close to the underdoped
limit the unusual isotope effect on transition temperature and penetration
depth uncovers critical phenomena associated with the quantum superconductor to
insulator transition in two dimensions.Comment: 6 pages, 3 figure
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