Photonic Berry curvature in double liquid crystal microcavities with broken inversion symmetry

We investigate a photonic device consisting of two coupled optical cavities possessing Rashba-Dresselhaus spin-orbit coupling, TE-TM splitting, and linear polarisation splitting that opens a tuneable energy gap at the diabolic points of the photon dispersion; giving rise to an actively addressable local Berry curvature. The proposed architecture stems from recent advancements in the design of artificial photonic gauge fields in liquid crystal cavities [K. Rechci\'{n}ska et al., Science 366, 727 (2019)]. Our study opens new perspectives for topological photonics, room-temperature spinoptronics, and studies on the quantum geometrical structure of photonic bands in extreme settings

Magneto-optical induced supermode switching in quantum fluids of light

The insensitivity of photons towards external magnetic fields forms one of the hardest barriers against efficient magneto-optical control, aiming at modulating the polarization state of light. However, there is even scarcer evidence of magneto-optical effects that can spatially modulate light. Here, we demonstrate the latter by exploiting strongly coupled states of semimagnetic matter and light in planar semiconductor microcavities. We nonresonantly excite two spatially adjacent exciton-polariton condensates which, through inherent ballistic near field coupling mechanism, spontaneously synchronise into a dissipative quantum fluidic supermode of definite parity. Applying a magnetic field along the optical axis, we continuously adjust the light-matter composition of the condensate exciton-polaritons, inducing a supermode switch into a higher order mode of opposite parity. Our findings set the ground towards magnetic spatial modulation of nonlinear light.Comment: 9 pages, 6 figure

Reduced Self-Aggregation and Improved Stability of Silica-Coated Fe3O4/Ag SERS-Active Nanotags Functionalized With 2-Mercaptoethanesulfonate

Nanocomposites combining magnetic and plasmonic properties are very attractive within the field of surface-enhanced Raman scattering (SERS) spectroscopy. Applications presented so far take advantage of not only the cooperation of both components but also synergy (enhanced properties), leading to multi-approach analysis. While many methods were proposed to synthesize such plasmonic-magnetic nanoparticles, the issue of their collective magnetic behavior, inducing irreversible self-aggregation, has not been addressed yet. Thus, here we present a simple and fast method to overcome this problem, employing 2-mercaptoethanesulfonate (MES) ions as both a SERS tag and primer molecules in the silica-coating process of the previously fabricated Fe3O4/Ag nanocomposite. The use of MES favored the formation of silica-coated nanomaterial comprised of well-dispersed small clusters of Fe3O4/Ag nanoparticles. Furthermore, adsorbed MES molecules provided a reliable SERS response, which was successfully detected after magnetic assembly of the Fe3O4/Ag@MES@SiO2 on the surface of the banknote. Improved chemical stability after coating with a silica layer was also found when the nanocomposite was exposed to suspension of yeast cells. This work reports on the application of 2-mercaptoethanesulfonate not only providing a photostable SERS signal due to a non-aromatic Raman reporter but also acting as a silica-coating primer and a factor responsible for a substantial reduction of the self-aggregation of the plasmonic-magnetic nanocomposite. Additionally, here obtained Fe3O4/Ag@MES@SiO2 SERS nanotags showed the potential as security labels for the authentication purposes, retaining its original SERS performance after deposition on the banknote

Natural exceptional points in the excitation spectrum of a light-matter system

We observe natural exceptional points in the excitation spectrum of an exciton-polariton system by optically tuning the light-matter interactions. The observed exceptional points do not require any spatial or polarization degrees of freedom and result solely from the transition from weak to strong light-matter coupling. We demonstrate that they do not coincide with the threshold for photon lasing, confirming previous theoretical predictions [Phys. Rev. Lett. 122, 185301 (2019), Optica 7, 1015 (2020) ]. Using a technique where a strong coherent laser pump induces up-converted excitations, we encircle the exceptional point in the parameter space of coupling strength and particle momentum. Our method of local optical control of light-matter coupling paves the way to investigation of fundamental phenomena including dissipative phase transitions and non-Hermitian topological states

Photonic Berry curvature in double liquid crystal microcavities with broken inversion symmetry

We investigate a photonic device consisting of two coupled optical cavities possessing Rashba-Dresselhaus spin-orbit coupling, TE-TM splitting, and linear polarization splitting that opens a tunable energy gap at the diabolic points of the photon dispersion; giving rise to an actively addressable local Berry curvature. The proposed architecture stems from recent advancements in the design of artificial photonic gauge fields in liquid crystal cavities [K. Rechcińska, Science 366, 727 (2019)SCIEAS0036-807510.1126/science.aay4182]. Our study opens perspectives for topological photonics, room-temperature spinoptronics, and studies on the quantum geometrical structure of photonic bands in extreme settings.</p

Control of dimer chain topology by Rashba-Dresselhaus spin-orbit coupling

We study theoretically a dimer chain in the presence of Rashba-Dresselhaus spin-orbit coupling (RDSOC) with equal strength. We show that the RDSOC can be described as a synthetic gauge field that controls not only the magnitude but also the sign of tunneling coefficients between sites. This allows to emulate not only a Su-Schrieffer-Heeger chain which is commonly implemented in various platforms, but also, all energy spectra of the transverse field Ising model with both ferromagnetic and antiferromagnetic coupling. We simulate a realistic implementation of these effective Hamiltonians based on liquid crystal microcavities. In that case, the RDSOC can be switched on and off by an applied voltage, which controls the band topology, the existence and characteristics of topological edge states, or the nature of the ground state. This setting is promising for topological photonics applications and from a quantum simulation perspective

Structural and Magnetic Properties of Co‒Mn Codoped ZnO Nanoparticles Obtained by Microwave Solvothermal Synthesis

Zinc oxide nanoparticles codoped with Co2+ and Mn2+ ions (Zn(1&#8722;x&#8722;y)MnxCoyO NPs) were obtained for the first time by microwave solvothermal synthesis. The nominal content of Co2+ and Mn2+ in Zn(1&#8722;x&#8722;y)MnxCoyO NPs was x = y = 0, 1, 5, 10 and 15 mol % (the amount of both ions was equal). The precursors were obtained by dissolving zinc acetate dihydrate, manganese (II) acetate tetrahydrate and cobalt (II) acetate tetrahydrate in ethylene glycol. The morphology, phase purity, lattice parameters, dopants content, skeleton density, specific surface area, average particle size, average crystallite size, crystallite size distribution and magnetic properties of NPs were determined. The real content of dopants was up to 25.0% for Mn2+ and 80.5% for Co2+ of the nominal content. The colour of the samples changed from white to dark olive green in line with the increasing doping level. Uniform spherical NPs with wurtzite structure were obtained. The average size of NPs decreased from 29 nm to 21 nm in line with the increase in the dopant content. Brillouin type paramagnetism and an antiferromagnetic interaction between the magnetic ions was found for all samples, except for that with 15 mol % doping level, where a small ferromagnetic contribution was found. A review of the preparation methods of Co2+ and Mn2+ codoped ZnO is presented