Condensation and Slow Dynamics of Polar Nanoregions in Lead Relaxors

It is now well established that the unique properties of relaxor ferroelectrics are due to the presence of polar nanoregions (PNR's). We present recent results from Neutron and Raman scattering of single crystals of PZN, PZN-xPT, and PMN. Both sets of measurements provide information on the condensation of the PNR's and on their slow dynamics, directly through the central peak and, indirectly, through their coupling to transverse phonons. A comparative analysis of these results allows identification of three stages in the evolution of the PNR's with decreasing temperature: a purely dynamic stage, a quasi-static stage with reorientational motion and a frozen stage. A model is proposed, based on a prior study of KTN, which explains the special behavior of the transverse phonons (TO and TA) in terms of their mutual coupling through the rotations of the PNR's.Comment: AIP 6x9 style files, 10 pages, 4 figures, Conference-Fundamental Physics of Ferroelectrics 200

Breather decay into a vortex/anti-vortex pair in a Josephson Ladder

We present experimental evidence for a new behavior which involves discrete breathers and vortices in a Josephson Ladder. Breathers can be visualized as the creation and subsequent annihilation of vortex/anti-vortex pairs. An externally applied magnetic field breaks the vortex/anti-vortex symmetry and causes the breather to split apart. The motion of the vortex or anti-vortex creates multi-site breathers, which are always to one side or the other of the original breather depending on the sign of the applied field. This asymmetry in applied field is experimentally observed.Comment: 10 pages, 5 figure

Elastic properties of Gd5Si2Ge2 studied with an ultrasonic pulse-echo technique

We present the results of a study of the elastic properties of Gd5Si2Ge2, an alloy with giant magnetocaloric, magnetostrictive, and colossal magnetoresistive properties. Sound wave velocities measured in a number of different geometries allowed us to determine the whole elastic tensor for the monoclinic phase of this material. The anisotropy of the crystal is explored using the polar plots of the variations in the main crystallographic planes of the sound speed, the Young’s modulus, the shear modulus, and the linear compressibility. The effect of hydrostatic pressure on the Gd5Si2Ge2 properties is clarified. The acoustical axes are determined. The bulk modulus is estimated as 68.5 GPa; the Debye temperature is 250 K

A Neutron Elastic Diffuse Scattering Study of PMN

We have performed elastic diffuse neutron scattering studies on the relaxor Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_3$ (PMN). The measured intensity distribution near a (100) Bragg peak in the (hk0) scattering plane assumes the shape of a butterfly with extended intensity in the (110) and (1$\bar{1}$0) directions. The temperature dependence of the diffuse scattering shows that both the size of the polar nanoregions (PNR) and the integrated diffuse intensity increase with cooling even for temperatures below the Curie temperature $T_C \sim 213$ K.Comment: Submitted to PR

Giant resonant light forces in microspherical photonics

Resonant light pressure effects can open new degrees of freedom in optical manipulation with microparticles, but they have been traditionally considered as relatively subtle effects. Using a simplified two-dimensional model of surface electromagnetic waves evanescently coupled to whispering gallery modes (WGMs) in transparent circular cavities, we show that under resonant conditions the peaks of the optical forces can approach theoretical limits imposed by the momentum conservation law on totally absorbing particles. Experimentally, we proved the existence of strong peaks of the optical forces by studying the optical propulsion of dielectric microspheres along tapered microfibers. We observed giant optical propelling velocities ∼0.45 mm s−1 for some of the 15-20 µm polystyrene microspheres in water for guided powers limited at ∼43 mW. Such velocities exceed previous observations by more than an order of magnitude, thereby providing evidence for the strongly enhanced resonant optical forces. We analyzed the statistical properties of the velocity distribution function measured for slightly disordered (∼1% size variations) ensembles of microspheres with mean diameters varying from 3 to 20 µm. These results demonstrate a principal possibility of optical sorting of microspheres with the positions of WGM resonances overlapped at the wavelength of the laser source. They can be used as building blocks of the lossless coupled resonator optical waveguides and various integrated optoelectronics devices

Dynamics of NEMS resonators across dissipation limits

The oscillatory dynamics of nanoelectromechanical systems (NEMS) is at the heart of many emerging applications in nanotechnology. For common NEMS, such as beams and strings, the oscillatory dynamics is formulated using a dissipationless wave equation derived from elasticity. Under a harmonic ansatz, the wave equation gives an undamped free vibration equation; solving this equation with the proper boundary conditions provides the undamped eigenfunctions with the familiar standing wave patterns. Any harmonically driven solution is expressible in terms of these undamped eigenfunctions. Here, we show that this formalism becomes inconvenient as dissipation increases. To this end, we experimentally map out the position- and frequency-dependent oscillatory motion of a NEMS string resonator driven linearly by a non-symmetric force at one end at different dissipation limits. At low dissipation (high Q factor), we observe sharp resonances with standing wave patterns that closely match the eigenfunctions of an undamped string. With a slight increase in dissipation, the standing wave patterns become lost, and waves begin to propagate along the nanostructure. At large dissipation (low Q factor), these propagating waves become strongly attenuated and display little, if any, resemblance to the undamped string eigenfunctions. A more efficient and intuitive description of the oscillatory dynamics of a NEMS resonator can be obtained by superposition of waves propagating along the nanostructure