Spontaneous-emission rates in finite photonic crystals of plane scatterers

The concept of a plane scatterer that was developed earlier for scalar waves is generalized so that polarization of light is included. Starting from a Lippmann-Schwinger formalism for vector waves, we show that the Green function has to be regularized before T-matrices can be defined in a consistent way. After the regularization, optical modes and Green functions are determined exactly for finite structures built up of an arbitrary number of parallel planes, at arbitrary positions, and where each plane can have different optical properties. The model is applied to the special case of finite crystals consisting of regularly spaced identical planes, where analytical methods can be taken further and only light numerical tasks remain. The formalism is used to calculate position- and orientation-dependent spontaneous-emission rates inside and near the finite photonic crystals. The results show that emission rates and reflection properties can differ strongly for scalar and for vector waves. The finite size of the crystal influences the emission rates. For parallel dipoles close to a plane, emission into guided modes gives rise to a peak in the frequency-dependent emission rate.Comment: 18 pages, 6 figures, to be published in Phys. Rev.

Continued-fraction representation of the Kraus map for non-Markovian reservoir damping

Quantum dissipation is studied for a discrete system that linearly interacts with a reservoir of harmonic oscillators at thermal equilibrium. Initial correlations between system and reservoir are assumed to be absent. The dissipative dynamics as determined by the unitary evolution of system and reservoir is described by a Kraus map consisting of an infinite number of matrices. For all Laplace-transformed Kraus matrices exact solutions are constructed in terms of continued fractions that depend on the pair correlation functions of the reservoir. By performing factorizations in the Kraus map a perturbation theory is set up that conserves in arbitrary perturbative order both positivity and probability of the density matrix. The latter is determined by an integral equation for a bitemporal matrix and a finite hierarchy for Kraus matrices. In lowest perturbative order this hierarchy reduces to one equation for one Kraus matrix. Its solution is given by a continued fraction of a much simpler structure as compared to the non-perturbative case. In lowest perturbative order our non-Markovian evolution equations are applied to the damped Jaynes-Cummings model. From the solution for the atomic density matrix it is found that the atom may remain in the state of maximum entropy for a significant time span that depends on the initial energy of the radiation field

Modified atomic decay rate near absorptive scatterers at finite temperature

The change in the decay rate of an excited atom that is brought about by extinction and thermal-radiation effects in a nearby dielectric medium is determined from a quantummechanical model. The medium is a collection of randomly distributed thermally-excited spherical scatterers with absorptive properties. The modification of the decay rate is described by a set of correction functions for which analytical expressions are obtained as sums over contributions from the multipole moments of the scatterers. The results for the modified decay rate as a function of the distance between the excited atom and the dielectric medium show the influence of absorption, scattering and thermal-radiation processes. Some of these processes are found to be mutually counteractive. The changes in the decay rate are compared to those following from an effective-medium theory in which the discrete scatterers are replaced by a continuum

Eigenmode analysis of the damped Jaynes-Cummings model

The generating functions for density matrix elements of the Jaynes-Cummings model with cavity damping are analysed in terms of their eigenmodes, which are characterised by a specific temporal behaviour. These eigenmodes are shown to be proportional to particular generalised hypergeometric functions. The relative weights of these eigenmodes in the generating functions are determined by the initial conditions of the model. These weights are found by deriving orthogonality relations involving adjoint modes. In an example it is shown how the time-dependent density matrix elements and the related factorial moments can be extracted from the eigenmode decompositions of the generating functions

Field quantization in inhomogeneous absorptive dielectrics

The quantization of the electromagnetic field in a three-dimensional inhomogeneous dielectric medium with losses is carried out in the framework of a damped-polariton model with an arbitrary spatial dependence of its parameters. The equations of motion for the canonical variables are solved explicitly by means of Laplace transformations for both positive and negative time. The dielectric susceptibility and the quantum noise-current density are identified in terms of the dynamical variables and parameters of the model. The operators that diagonalize the Hamiltonian are found as linear combinations of the canonical variables, with coefficients depending on the electric susceptibility and the dielectric Green function. The complete time dependence of the electromagnetic field and of the dielectric polarization is determined. Our results provide a microscopic justification of the phenomenological quantization scheme for the electromagnetic field in inhomogeneous dielectrics.Comment: 19 page

Field quantization in inhomogeneous anisotropic dielectrics with spatio-temporal dispersion

A quantum damped-polariton model is constructed for an inhomogeneous anisotropic linear dielectric with arbitrary dispersion in space and time. The model Hamiltonian is completely diagonalized by determining the creation and annihilation operators for the fundamental polariton modes as specific linear combinations of the basic dynamical variables. Explicit expressions are derived for the time-dependent operators describing the electromagnetic field, the dielectric polarization and the noise term in the latter. It is shown how to identify bath variables that generate the dissipative dynamics of the medium.Comment: 24 page

Atomic decay near a quantized medium of absorbing scatterers

The decay of an excited atom in the presence of a medium that both scatters and absorbs radiation is studied with the help of a quantum-electrodynamical model. The medium is represented by a half space filled with a randomly distributed set of non-overlapping spheres, which consist of a linear absorptive dielectric material. The absorption effects are described by means of a quantized damped-polariton theory. It is found that the effective susceptibility of the bulk does not fully account for the medium-induced change in the atomic decay rate. In fact, surface effects contribute to the modification of the decay properties as well. The interplay of scattering and absorption in the total decay rate is discussed.Comment: 20 pages, 1 figur

Electromagnetic field quantization in an anisotropic magnetodielectric medium with spatial-temporal dispersion

By modeling a linear, anisotropic and inhomogeneous magnetodielectric medium with two independent set of harmonic oscillators, electromagnetic field is quantized in such a medium. The electric and magnetic polarizations of the medium are expressed as linear combinations of the ladder operators describing the magnetodielectric medium. The Maxwell and the constitutive equations of the medium are obtained as the Heisenberg equations of the total system. The electric and magnetic susceptibilities of the medium are obtained in terms of the tensors coupling the medium with the electromagnetic field. The explicit forms of the electromagnetic field operators are obtained in terms of the ladder operators of the medium.Comment: 18 pages, no figure

Canonical quantization of macroscopic electromagnetism

Application of the standard canonical quantization rules of quantum field theory to macroscopic electromagnetism has encountered obstacles due to material dispersion and absorption. This has led to a phenomenological approach to macroscopic quantum electrodynamics where no canonical formulation is attempted. In this paper macroscopic electromagnetism is canonically quantized. The results apply to any linear, inhomogeneous, magnetodielectric medium with dielectric functions that obey the Kramers-Kronig relations. The prescriptions of the phenomenological approach are derived from the canonical theory.Comment: 21 pages, additional reference

Sum rules for correlation functions of ionic mixtures in arbitrary dimension d≥2d\geq 2

The correlations in classical multi-component ionic mixtures with spatial dimension $d\geq 2$ are studied by using a restricted grand-canonical ensemble and the associated hierarchy equations for the correlation functions. Sum rules for the first few moments of the two-particle correlation function are derived and their dependence on $d$ is established. By varying $d$ continuously near $d=2$ it is shown how the sum rules for the two-dimensional mixture are related to those for mixtures at higher $d$.Comment: 19 page