220 research outputs found
Anomalous pressure effect on the remanent lattice striction of a (La,Pr)SrMnO bilayered manganite single crystal
We have studied the pressure effect on magnetostriction, both in the
-plane and along the c-axis, of a (La,Pr)SrMnO
bilayered manganite single crystal over the temperature region where the
field-induced ferromagnetic metal (FMM) transition takes place. For comparison,
we have also examined the pressure dependence of magnetization curves at the
corresponding temperatures. The applied pressure reduces the critical field of
the FMM transition and it enhances the remanent magnetostriction. An anomalous
pressure effect on the remanent lattice relaxation is observed and is similar
to the pressure effect on the remanent magnetization along the c-axis. These
findings are understood from the view point that the double-exchange
interaction driven FMM state is strengthened by application of pressure.Comment: 7 pages,7 figure
Steplike Lattice Deformation of Single Crystalline (LaPr)SrMnO Bilayered Manganite
We report a steplike lattice transformation of single crystalline
(LaPr)SrMnObilayered manganite
accompanied by both magnetization and magnetoresistive jumps, and examine the
ultrasharp nature of the field-induced first-order transition from a
paramagnetic insulator to a ferromagnetic metal phase accompanied by a huge
decrease in resistance. Our findings support that the abrupt magnetostriction
is closely related to an orbital frustration existing in the inhomogeneous
paramagnetic insulating phase rather than a martensitic scenario between
competing two phases.Comment: 5 pages,4figures, v4: figures are changed, in press in Phys.Rev.Let
Ferromagnetism in defect-ridden oxides and related materials
The existence of high-temperature ferromagnetism in thin films and
nanoparticles of oxides containing small quantities of magnetic dopants remains
controversial. Some regard these materials as dilute magnetic semiconductors,
while others think they are ferromagnetic only because the magnetic dopants
form secondary ferromagnetic impurity phases such as cobalt metal or magnetite.
There are also reports in d0 systems and other defective oxides that contain no
magnetic ions. Here, we investigate TiO2 (rutile) containing 1 - 5% of iron
cations and find that the room-temperature ferromagnetism of films prepared by
pulsed-laser deposition is not due to magnetic ordering of the iron. The films
are neither dilute magnetic semiconductors nor hosts to an iron-based
ferromagnetic impurity phase. A new model is developed for defect-related
ferromagnetism which involves a spin-split defect band populated by charge
transfer from a proximate charge reservoir in the present case a mixture Fe2+
and Fe3+ ions in the oxide lattice. The phase diagram for the model shows how
inhomogeneous Stoner ferromagnetism depends on the total number of electrons
Ntot, the Stoner exchange integral I and the defect bandwidth W; the band
occupancy is governed by the d-d Coulomb interaction U. There are regions of
ferromagnetic metal, half-metal and insulator as well as nonmagnetic metal and
insulator. A characteristic feature of the high-temperature Stoner magnetism is
an an anhysteretic magnetization curve which is practically temperature
independent below room temperature. This is related to a wandering
ferromagnetic axis which is determined by local dipole fields. The
magnetization is limited by the defect concentration, not by the 3d doping.
Only 1-2 % of the volume of the films is magnetically ordered.Comment: 22 pages, 6 figure
Magneto-optical investigation of the field-induced spin-glass insulator to ferromagnetic metallic transition of the bilayer manganite (LaPr)SrMnO
We measured the magneto-optical response of
(LaPr)SrMnO in order to investigate the
microscopic aspects of the magnetic field driven spin-glass insulator to
ferromagnetic metal transition. Application of a magnetic field recovers the
ferromagnetic state with an overall redshift of the electronic structure,
growth of the bound carrier localization associated with ferromagnetic domains,
development of a pseudogap, and softening of the Mn-O stretching and bending
modes that indicate a structural change. We discuss field- and
temperature-induced trends within the framework of the Tomioka-Tokura global
electronic phase diagram picture and suggest that controlled disorder near a
phase boundary can be used to tune the magnetodielectric response. Remnants of
the spin-glass insulator to ferromagnetic metallic transition can also drive
300 K color changes in (LaPr)SrMnO.Comment: 9 pages, 8 figure
Effect of pressure on steplike magnetostriction of single crystalline (LaPr)SrMnO bilayered manganite
e report the effect of pressure on the steplike magnetostriction of single
crystalline bilayered manganite (LaPr)1.2Sr1.8Mn2O8, for our understandings of
the ultrasharp nature of the field-induced first-order transition from a
paramagnetic insulator to a ferromagnetic metal phase. The application of
pressure suppresses a steplike transformation and causes a broad change in the
magnetostriction. The injection of an electric current to the crystal also
weakens the steplike variation in both the magnetostriction and
magnetoresistance. The stabilization of ferromagnetic interaction or the
delocalization of charge carriers is promoted with the applied pressure or
applied current, resulting in the suppressed steplike behavior. Our findings
suggest that the step phenomenon is closely related to the existence of
localized carriers such as the short-range charge-orbital ordered clusters.Comment: 5 pages,4 figure
Shielding efficiency and E(J) characteristics measured on large melt cast Bi-2212 hollow cylinders in axial magnetic fields
We show that tubes of melt cast Bi-2212 used as current leads for LTS magnets
can also act as efficient magnetic shields. The magnetic screening properties
under an axial DC magnetic field are characterized at several temperatures
below the liquid nitrogen temperature (77 K). Two main shielding properties are
studied and compared with those of Bi-2223, a material that has been considered
in the past for bulk magnetic shields. The first property is related to the
maximum magnetic flux density that can be screened, Blim; it is defined as the
applied magnetic flux density below which the field attenuation measured at the
centre of the shield exceeds 1000. For a cylinder of Bi-2212 with a wall
thickness of 5 mm and a large ratio of length over radius, Blim is evaluated to
1 T at T = 10 K. This value largely exceeds the Blim value measured at the same
temperature on similar tubes of Bi-2223. The second shielding property that is
characterized is the dependence of Blim with respect to variations of the sweep
rate of the applied field, dBapp/dt. This dependence is interpreted in terms of
the power law E = Ec(J/Jc)^n and allows us to determine the exponent n of this
E(J) characteristics for Bi-2212. The characterization of the magnetic field
relaxation involves very small values of the electric field. This gives us the
opportunity to experimentally determine the E(J) law in an unexplored region of
small electric fields. Combining these results with transport and AC shielding
measurements, we construct a piecewise E(J) law that spans over 8 orders of
magnitude of the electric field.Comment: 16 pages, 7 figure
Soft X-ray resonant scattering study of single-crystal LaSrMnO
Soft X-ray resonant scattering studies at the Mn - and
the La - edges of single-crystal LaSrMnO are
reported. At low temperatures, below K, energy scans
with a fixed momentum transfer at the \emph{A}-type antiferromagnetic (0 0 1)
reflection around the Mn -edges with incident linear
and polarizations show strong resonant enhancements. The
splitting of the energy spectra around the Mn -edges may
indicate the presence of a mixed valence state, e.g., Mn/Mn. The
relative intensities of the resonance and the clear shoulder-feature as well as
the strong incident and polarization dependences strongly
indicate its complex electronic origin. Unexpected enhancement of the charge
Bragg (0 0 2) reflection at the La -edges with
polarization has been observed up to 300 K, with an anomaly appearing around
the orbital-ordering transition temperature, K,
suggesting a strong coupling (competition) between them.Comment: Accepted by European Physical Journal
Anisotropic phonon conduction and lattice distortions in CMR-type bilayer manganite (LaPr)SrMnO (z=0,0.2,0.4 and 0.6) single crystals
We have undertaken a systematic study of thermal conductivity as a function
of temperature and magnetic field of single crystals of the compound
(LaPr)SrMnO for (Pr) =0.2,0.4. and
0.6. The lattice distortion due to Pr-substitution and anisotropic thermal
conductivity in bilayer manganites are discussed on the basis of different
relaxation models of local lattice distortions in metal and insulating states
proposed by Maderda et al. The giant magnetothermal effect is scaled as a
function of magnetization and discussed on the basis of a systematic variation
of the occupation of the -electron orbital states due to Pr-substitution.Comment: 7 pages, 6 figures, in press in Phys.Rev.
Microscopic theory of quadrupolar ordering in TmTe
We have calculated the crystal electric field of TmTe (T>T_Q) and have
obtained that the ground state of a Tm 4f hole is the doublet in
agreement with Mossbauer experiments. We study the quadrupole interactions
arising from quantum transitions of 4f holes of Tm. An effective attraction is
found at the L point of the Brillouin zone, . Assuming that the
quadrupolar condensation involves a single arm of we show that
there are two variants for quadrupole ordering which are described by the space
groups C2/c and C2/m. The Landau free energy is derived in mean-field theory.
The phase transition is of second order. The corresponding quadrupole order
parameters are combinations of and components. The obtained
domain structure is in agreement with observations from neutron diffraction
studies for TmTe. Calculated lattice distortions are found to be different for
the two variants of quadrupole ordering. We suggest to measure lattice
displacements in order to discriminate between those two structures.Comment: 10 pages, 2 figures, 5 tables; accepted by PR
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