999 research outputs found
Fabrication and transport critical currents of multifilamentary MgB2/Fe wires and tapes
Multifilamentary MgB2/Fe wires and tapes with high transport critical current
densities have been fabricated using a straightforward powder-in-tube (PIT)
process. After annealing, we measured transport jc values up to 1.1 * 105 A/cm2
at 4.2 K and in a field of 2 T in a MgB2/Fe square wire with 7 filaments
fabricated by two-axial rolling, and up to 5 * 104 A/cm2 at 4.2 K in 1 T in a
MgB2/Fe tape with 7 filaments. For higher currents these multifilamentary wires
and tapes quenched due to insufficient thermal stability of filaments. Both the
processing routes and deformation methods were found to be important factors
for fabricating multifilamentary MgB2 wires and tapes with high transport jc
values.Comment: 13 pages, 7 figure
High power rechargeable magnesium/iodine battery chemistry
© The Author(s) 2017. Rechargeable magnesium batteries have attracted considerable attention because of their potential high energy density and low cost. However, their development has been severely hindered because of the lack of appropriate cathode materials. Here we report a rechargeable magnesium/iodine battery, in which the soluble iodine reacts with Mg2+ to form a soluble intermediate and then an insoluble final product magnesium iodide. The liquid-solid two-phase reaction pathway circumvents solid-state Mg2+ diffusion and ensures a large interfacial reaction area, leading to fast reaction kinetics and high reaction reversibility. As a result, the rechargeable magnesium/iodine battery shows a better rate capability (180 mAh g-1 at 0.5 C and 140 mAh g-1 at 1 C) and a higher energy density (âŒ400 Wh kg-1) than all other reported rechargeable magnesium batteries using intercalation cathodes. This study demonstrates that the liquid-solid two-phase reaction mechanism is promising in addressing the kinetic limitation of rechargeable magnesium batteries
Investigating properties of heavy and superheavy atomic systems with configurations
We have investigated energies and spectroscopic properties such as lifetimes,
factors, and hyperfine structure constants of the neutral atoms P through
Mc belonging to Group-15, singly ionized atoms S through Lv of Group-16
and doubly ionized atoms Cl through Ts of Group-17 of the
periodic table. These elements have configurations with , which
are highly open-shell and expected to exhibit strong electron correlation
effects. We have used four-component Dirac-Coulomb Hamiltonian along with Gaunt
term and a relativistic effective core potential through the relativistic
multi-reference configuration interaction method to perform the calculations
with sufficient accuracy and compare the results with the available literature
data. These comparisons suggest that our predicted values, for which
experimental data are not available, are reliable enough to be useful for
future applications.Comment: 19 pages,12 table
Anatomic Insights into Disrupted Small-World Networks in Pediatric Posttraumatic Stress Disorder.
Purpose To use diffusion-tensor (DT) imaging and graph theory approaches to explore the brain structural connectome in pediatric posttraumatic stress disorder (PTSD). Materials and Methods This study was approved by the relevant research ethics committee, and all participantsâ parents or guardians provided informed consent. Twenty-four pediatric patients with PTSD and 23 control subjects exposed to trauma but without PTSD were recruited after the 2008 Sichuan earthquake. The structural connectome was constructed by using DT imaging tractography and thresholding the mean fractional anisotropy of 90 brain regions to yield 90 Ă 90 partial correlation matrixes. Graph theory analysis was used to examine the group-specific topologic properties, and nonparametric permutation tests were used for group comparisons of topologic metrics. Results Both groups exhibited small-world topology. However, patients with PTSD showed an increase in the characteristic path length (P = .0248) and decreases in local efficiency (P = .0498) and global efficiency (P = .0274). Furthermore, patients with PTSD showed reduced nodal centralities, mainly in the default mode, salience, central executive, and visual regions (P < .05, corrected for false-discovery rate). The Clinician-Administered PTSD Scale score was negatively correlated with the nodal efficiency of the left superior parietal gyrus (r = â0.446, P = .043). Conclusion The structural connectome showed a shift toward âregularization,â providing a structural basis for functional alterations of pediatric PTSD. These abnormalities suggest that PTSD can be understood by examining the dysfunction of large-scale spatially distributed neural networks
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Ultrasound-triggered disruption and self-healing of reversibly cross-linked hydrogels for drug delivery and enhanced chemotherapy
Foldable photoelectronics and muscle-like transducers require highly stretchable and transparent electrical conductors. Some conducting oxides are transparent, but not stretchable. Carbon nanotube films, graphene sheets and metal-nanowire meshes can be both stretchable and transparent, but their electrical resistances increase steeply with strain <100%. Here we present highly stretchable and transparent Au nanomesh electrodes on elastomers made by grain boundary lithography. The change in sheet resistance of Au nanomeshes is modest with a one-time strain of ~160% (from ~21âΩ per square to ~67âΩ per square), or after 1,000 cycles at a strain of 50%. The good stretchability lies in two aspects: the stretched nanomesh undergoes instability and deflects out-of-plane, while the substrate stabilizes the rupture of Au wires, forming distributed slits. Larger ratio of mesh-size to wire-width also leads to better stretchability. The highly stretchable and transparent Au nanomesh electrodes are promising for applications in foldable photoelectronics and muscle-like transducers.Engineering and Applied Science
On the sample size dependence of the critical current density in MgB superconductors
Sample size dependent critical current density has been observed in magnesium
diboride superconductors. At high fields, larger samples provide higher
critical current densities, while at low fields, larger samples give rise to
lower critical current densities. The explanation for this surprising result is
proposed in this study based on the electric field generated in the
superconductors. The dependence of the current density on the sample size has
been derived as a power law ( is the factor
characterizing curve ). This dependence provides one with
a new method to derive the factor and can also be used to determine the
dependence of the activation energy on the current density.Comment: Revtex, 4 pages, 5 figure
Experimental and Simulation Study on the Emissions of a Multi-Point Lean Direct Injection Combustor
Spurred by the worldâs attention to pollution emissions from commercial aero-engines, the International Civil Aviation Organization (ICAO) has made more stringent emission regulations for civil aircraft engines, especially the NOx emission.This paper develops a Five-Point lean direct injection (LDI) combustor with three swirler schemes to reduce the emissions of commercial aircraft engines. The flowfield of the combustor is studied numerically. Moreover, the combustion efficiency and gaseous emissions in different inlet conditions and fuel ratios of the main stage (α) are studied experimentally. The corresponding results reveal that, under a fuel-air ratio (FAR) between 0.0130 and 0.0283 and an α value between 30% and 60%, the combustion efficiency is 99.18%, 98.83%, and 99.03% when the pilot stage works alone, and 99.69%, 99.23%, and 99.75% when the pilot and main stage work simultaneously. Furthermore, the experimental results suggest that the NOx emission decreases as α increases, demonstrating that the convergent swirler has a tremendous advantage in reducing NOx emissions over Venturi
Direct observation of active material concentration gradients and crystallinity breakdown in LiFePO4 electrodes during charge/discharge cycling of lithium batteries
The phase changes that occur during discharge of an electrode comprised of LiFePO4, carbon, and PTFE binder have been studied in lithium half cells by using X-ray diffraction measurements in reflection geometry. Differences in the state of charge between the front and the back of LiFePO4 electrodes have been visualized. By modifying the X-ray incident angle the depth of penetration of the X-ray beam into the electrode was altered, allowing for the examination of any concentration gradients that were present within the electrode. At high rates of discharge the electrode side facing the current collector underwent limited lithium insertion while the electrode as a whole underwent greater than 50% of discharge. This behavior is consistent with depletion at high rate of the lithium content of the electrolyte contained in the electrode pores. Increases in the diffraction peak widths indicated a breakdown of crystallinity within the active material during cycling even during the relatively short duration of these experiments, which can also be linked to cycling at high rate
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