2 research outputs found
The dual nature of magnetism in a uranium heavy fermion system
The duality between localized and itinerant nature of magnetism in
electron systems has been a longstanding puzzle. Here, we report
inelastic neutron scattering measurements, which reveal both local and
itinerant aspects of magnetism in a single crystalline system of
UPtSi. In the antiferromagnetic state, we observe broad continuum
of diffuse magnetic scattering with a resonance-like gap of 7 meV,
and surprising absence of coherent spin-waves, suggestive of itinerant
magnetism. While the gap closes above the Neel temperature, strong dynamic spin
correlations persist to high temperature. Nevertheless, the size and
temperature dependence of the total magnetic spectral weight can be well
described by local moment with . Furthermore, polarized neutron
measurements reveal that the magnetic fluctuations are mostly transverse, with
little or none of the longitudinal component expected for itinerant moments.
These results suggest that a dual description of local and itinerant magnetism
is required to understand UPtSi, and by extension, other 5
systems in general.Comment: see supplementary material for more detail
Dual Nature of Magnetism in a Uranium Heavy-Fermion System
The duality between the localized and itinerant nature of magnetism in 5f-electron systems has been a long-standing puzzle. Here, we report inelastic neutron scattering measurements, which reveal both local and itinerant aspects of magnetism in a single-crystalline system of UPt2Si2. In the antiferromagnetic state, we observe a broad continuum of diffuse magnetic scattering with a resonancelike gap of ≈7 meV and the surprising absence of coherent spin waves, suggestive of itinerant magnetism. While the gap closes above the N´eel temperature, strong dynamic spin correlations persist to a high temperature. Nevertheless, the size and temperature dependence of the total magnetic spectral weight can be well described by a local moment with J ¼ 4. Furthermore, polarized neutron measurements reveal that the magnetic fluctuations are mostly transverse, with little or none of the longitudinal component expected for itinerant moments. These results suggest that a dual description of local and itinerant magnetism is required to understand UPt2Si2 and, by extension, other 5f systems, in general. © 2018 American Physical Societ