Ultrashort intense-field optical vortices produced with laser-etched mirrors

We introduce a simple and practical method to create ultrashort intense optical vortices for applications involving high-intensity lasers. Our method utilizes femtosecond laser pulses to laser-etch grating lines into laser-quality gold mirrors. These grating lines holographically encode an optical vortex. We derive mathematical equations for each individual grating line to be etched, for any desired (integer) topological charge. We investigate the smoothness of the etched grooves. We show that they are smooth enough to produce optical vortices with an intensity that is only a few percent lower than in the ideal case. We demonstrate that the etched gratings can be used in a folded version of our 2f-2f setup [Mariyenko et al., Opt. Express 19, 7599 (2005)] to compensate angular dispersion. Lastly, we show that the etched gratings withstand intensities of up to 10^12 W/cm2.Comment: 14 pages, 12 figures, submitted to Optics Expres

\u3ci\u3eIn Situ\u3c/i\u3e Measurement of Three-Dimensional Ion Densities in Focused Femtosecond Pulses

We image spatial distributions of Xeq+ ions in the focus of a laser beam of ultrashort, intense pulses in all three dimensions, with a resolution of ~3μm and ~12 μm in the two transverse directions. This allows for studying ionization processes without spatially averaging ion yields. Our in situ ion imaging is also useful to analyze focal intensity profiles and to investigate the transverse modal purity of tightly focused beams of complex light. As an example, the intensity profile of a Hermite-Gaussian beam mode HG1,0 recorded with ions is found to be in good agreement with optical images

Intense-Field Ionization of Monoaromatic Hydrocarbons using Radiation Pulses of Ultrashort Duration: Monohalobenzenes and Azabenzenes

Using 50-fs, 800-nm pulses, we study the intense-field ionization and fragmentation of the monohalobenzenes C_(6)H_(5)-X (X=F, Cl, Br, I) and of the heterocyclics azabenzene C5H5N (pyridine) and the three diazabenzenes C_(4)H_(4)N_(2) (pyridazine, pyrimidine, and pyrazine). Avoiding focal intensity averaging we find indications of resonance-enhanced MPI. In the monohalobenzenes the propensity for fragmentation increases for increasing Z: fluorobenzene yields predominantly C6H5Fn+, while iodobenzene yields atomic ions with charges up to I^(8+). We ascribe this to the heavy-atom effect: the large charge of the heavy halogens' nuclei induces ultrafast intersystem crossing to dissociative triplet states

Creation of optical vortices in femtosecond pulses

We experimentally created a femtosecond optical vortex using a pair of computer-synthesized holographic gratings arranged in a 2f - 2f optical setup. We present measurements showing that the resulting donut mode is free of spatial chirp, and support this finding with an analysis of the optical wave propagation through our system based on the Kirchhoff- Fresnel diffraction integral. An interferogram confirms that our ultrashort vortex has topological charge 1, and a conservative experimental estimation of its duration is 280 fs. We used 25-fs radiation pulses (bandwidth approximately 40 nm) produced by a Ti:sapphire laser oscillator

Frequency comb vernier spectroscopy in the near infrared

We perform femtosecond frequency comb vernier spectroscopy in the near infrared with a femtosecond Er doped fiber laser, a scanning high-finesse cavity and an InGaAs camera. By utilizing the properties of a frequency comb and a scanning high-finesse cavity such spectroscopy provides broad spectral bandwidth, high spectral resolution, and high detection sensitivity on a short time scale. We achieved an absorption sensitivity of ~8E-8 cm-1Hz-1/2 corresponding to a detection limit of ~70 ppbv for acetylene, with a resolution of ~1.1 GHz in single images taken in 0.5 seconds and covering a frequency range of ~5 THz. These measurements have broad applications for sensing other greenhouse gases in this fingerprint near IR region with a simple apparatus.Comment: 14 pages, 5 figure

Frame dragging with optical vortices

General Relativistic calculations in the linear regime have been made for electromagnetic beams of radiation known as optical vortices. These exotic beams of light carry a physical quantity known as optical orbital angular momentum (OAM). It is found that when a massive spinning neutral particle is placed along the optical axis, a phenomenon known as inertial frame dragging occurs. Our results are compared with those found previously for a ring laser and an order of magnitude estimate of the laser intensity needed for a precession frequency of 1 Hz is given for these "steady" beams of light.Comment: 13 pages, 2 figure

\emph{In situ} measurement of three-dimensional ion densities in focused femtosecond pulses

We image spatial distributions of Xe$^{q+}$ ions in the focus of a laser beam of ultrashort, intense pulses in all three dimensions, with a resolution of $\sim$3 $\mu$m and $\sim$12 $\mu$m in the two transverse directions. This allows for studying ionization processes without spatially averaging ion yields. Our \emph{in situ} ion imaging is also useful to analyze focal intensity profiles and to investigate the transverse modal purity of tightly focused beams of complex light. As an example, the intensity profile of a Hermite-Gaussian beam mode HG$_{1,0}$ recorded with ions is found to be in good agreement with optical images.Comment: 4 pages, 4 figure

Reconstruction of ionization probabilities from spatially averaged data in N-dimensions

We present an analytical inversion technique which can be used to recover ionization probabilities from spatially averaged data in an N-dimensional detection scheme. The solution is given as a power series in intensity. For this reason, we call this technique a multiphoton expansion (MPE). The MPE formalism was verified with an exactly solvable inversion problem in 2D, and probabilities in the postsaturation region, where the intensity-selective scanning approach breaks down, were recovered. In 3D, ionization probabilities of Xe were successfully recovered with MPE from simulated (using the ADK tunneling theory) ion yields. Finally, we tested our approach with intensity-resolved benzene ion yields showing a resonant multiphoton ionization process. By applying MPE to this data (which was artificially averaged) the resonant structure was recovered-suggesting that the resonance in benzene may have been observable in spatially averaged data taken elsewhere.Comment: 19 pages and 3 figure