801 research outputs found
Inhomogeneous Nuclear Spin Flips
We discuss a feedback mechanism between electronic states in a double quantum
dot and the underlying nuclear spin bath. We analyze two pumping cycles for
which this feedback provides a force for the Overhauser fields of the two dots
to either equilibrate or diverge. Which of these effects is favored depends on
the g-factor and Overhauser coupling constant A of the material. The strength
of the effect increases with A/V_x, where V_x is the exchange matrix element,
and also increases as the external magnetic field B_{ext} decreases.Comment: 5 pages, 4 figures (jpg
Theory of spin, electronic and transport properties of the lateral triple quantum dot molecule in a magnetic field
We present a theory of spin, electronic and transport properties of a
few-electron lateral triangular triple quantum dot molecule in a magnetic
field. Our theory is based on a generalization of a Hubbard model and the
Linear Combination of Harmonic Orbitals combined with Configuration Interaction
method (LCHO-CI) for arbitrary magnetic fields. The few-particle spectra
obtained as a function of the magnetic field exhibit Aharonov-Bohm
oscillations. As a result, by changing the magnetic field it is possible to
engineer the degeneracies of single-particle levels, and thus control the total
spin of the many-electron system. For the triple dot with two and four
electrons we find oscillations of total spin due to the singlet-triplet
transitions occurring periodically in the magnetic field. In the three-electron
system we find a transition from a magnetically frustrated to the
spin-polarized state. We discuss the impact of these phase transitions on the
addition spectrum and the spin blockade of the lateral triple quantum dot
molecule.Comment: 30 pages (one column), 9 figure
Magnetically induced chessboard pattern in the conductance of a Kondo quantum dot
We quantitatively describe the main features of the magnetically induced
conductance modulation of a Kondo quantum dot -- or chessboard pattern -- in
terms of a constant-interaction double quantum dot model. We show that the
analogy with a double dot holds down to remarkably low magnetic fields. The
analysis is extended by full 3D spin density functional calculations.
Introducing an effective Kondo coupling parameter, the chessboard pattern is
self-consistently computed as a function of magnetic field and electron number,
which enables us to quantitatively explain our experimental data.Comment: 4 pages, 3 color figure
Fast sensing of double-dot charge arrangement and spin state with an rf sensor quantum dot
Single-shot measurement of the charge arrangement and spin state of a double
quantum dot are reported, with measurement times down to ~ 100 ns. Sensing uses
radio-frequency reflectometry of a proximal quantum dot in the Coulomb blockade
regime. The sensor quantum dot is up to 30 times more sensitive than a
comparable quantum point contact sensor, and yields three times greater signal
to noise in rf single-shot measurements. Numerical modeling is qualitatively
consistent with experiment and shows that the improved sensitivity of the
sensor quantum dot results from reduced screening and lifetime broadening.Comment: related papers at http://marcuslab.harvard.ed
Metal-insulator transition in a two-dimensional electron system: the orbital effect of in-plane magnetic field
The conductance of an open quench-disordered two-dimensional (2D) electron
system subject to an in-plane magnetic field is calculated within the framework
of conventional Fermi liquid theory applied to actually a three-dimensional
system of spinless electrons confined to a highly anisotropic (planar)
near-surface potential well. Using the calculation method suggested in this
paper, the magnetic field piercing a finite range of infinitely long system of
carriers is treated as introducing the additional highly non-local scatterer
which separates the circuit thus modelled into three parts -- the system as
such and two perfect leads. The transverse quantization spectrum of the inner
part of the electron waveguide thus constructed can be effectively tuned by
means of the magnetic field, even though the least transverse dimension of the
waveguide is small compared to the magnetic length. The initially finite
(metallic) value of the conductance, which is attributed to the existence of
extended modes of the transverse quantization, decreases rapidly as the
magnetic field grows. This decrease is due to the mode number reduction effect
produced by the magnetic field. The closing of the last current-carrying mode,
which is slightly sensitive to the disorder level, is suggested as the origin
of the magnetic-field-driven metal-to-insulator transition widely observed in
2D systems.Comment: 19 pages, 7 eps figures, the extension of cond-mat/040613
Rashba-control for the spin excitation of a fully spin polarized vertical quantum dot
Far infrared radiation absorption of a quantum dot with few electrons in an
orthogonal magnetic field could monitor the crossover to the fully spin
polarized state. A Rashba spin-orbit coupling can tune the energy and the spin
density of the first excited state which has a spin texture carrying one extra
unit of angular momentum. The spin orbit coupling can squeeze a flipped spin
density at the center of the dot and can increase the gap in the spectrum.Comment: 4 pages, 5 figure
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Anion Stabilization in Electrostatic Environments
Excess charge stabilization of molecules in metallic environments is of particular importance for fields such as molecular electronics and surface chemistry. We study the energetics of benzene and its anion between two metallic plates. We observe that orientational effects are important at small inter-plate separation. This leads to benzene oriented perpendicular to the gates being more stable than the parallel case due to induced dipole effects. We find that the benzene anion, known for being unstable in the gas-phase, is stabilized by the plates at zero bias and an inter-plate distance of 21 Å. We also observe the effect of benzene under a voltage bias generated by the plates; under a negative bias, the anion becomes destabilized. We use the electron localization function to analyze the changes in electron density due to the bias. These findings suggest that image effects such as those present in nanoscale devices, are able to stabilize excess charge and should be important to consider when modeling molecular transport junctions and charge-transfer effects.Chemistry and Chemical Biolog
Effect of confinement potential shape on exchange interaction in coupled quantum dots
Exchange interaction has been studied for electrons in coupled quantum dots
(QD's) by a configuration interaction method using confinement potentials with
different profiles. The confinement potential has been parametrized by a
two-centre power-exponential function, which allows us to investigate various
types of QD's described by either soft or hard potentials of different range.
For the soft (Gaussian) confinement potential the exchange energy decreases
with increasing interdot distance due to the decreasing interdot tunnelling.
For the hard (rectangular-like) confinement potential we have found a
non-monotonic behaviour of the exchange interaction as a function of distance
between the confinement potential centres. In this case, the exchange
interaction energy exhibits a pronounced maximum for the confinement potential
profile which corresponds to the nanostructure composed of the small inner QD
with a deep potential well embedded in the large outer QD with a shallow
potential well. This effect results from the strong localization of electrons
in the inner QD, which leads to the large singlet-triplet splitting.
Implications of this finding for quantum logic operations have been discussed.Comment: 16 pages, including 11 figure
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Fast Sensing of Double-Dot Charge Arrangement and Spin State with a Radio-Frequency Sensor Quantum Dot
Single-shot measurement of the charge arrangement and spin state of a double quantum dot are reported with measurement times down to 100 ns. Sensing uses radio-frequency reflectometry of a proximal quantum dot in the Coulomb blockade regime. The sensor quantum dot is up to 30 times more sensitive than a comparable quantum point-contact sensor and yields three times greater signal to noise in rf single-shot measurements. Numerical modeling is qualitatively consistent with experiment and shows that the improved sensitivity of the sensor quantum dot results from reduced lifetime broadening and screening.PhysicsOther Research Uni
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