Linking confined electron spins through coherent light-matter interaction.

Electron spins confined to self-assembled quantum dots are considered as nodes for a coherent optical network capable of supporting distributed quantum states. Through a series of experiments, the work contributing to this dissertation examines some of the key criteria for constructing such a network. First, the ability to optically extract a coherent spin state from the quantum dot without perturbing the nuclear environment is explored: nuclear feedback is an issue that has frustrated previous studies into electron spin coherence in these systems. With the novel techniques we develop, we identify and characterise the previously undetermined intrinsic mechanisms that govern the coherence of the central spin. We show how the coherence of the electron spin is intimately related to the growth of these strained nanostructures. Second, a model network is constructed in which two spins confined to separate quantum dots are projected into a highly entangled state. This is the first time electron spins in distant quantum dots have been entangled, and in doing so we demonstrate controllable entanglement generation at the highest rates recorded for optically accessible qubit definitions. We investigate the realisation of a hybrid quantum network by demonstrating the first interconnect between wholly different single quantum systems: a semiconductor quantum dot and a trapped ytterbium ion. In forming an optical link between these two complementary qubit definitions, we show that we can circumvent their intrinsic optical differences through coherent photon generation at the quantum dot. A network built from these diverse constituents could combine the ultrafast operations self-assembled quantum dots enable with the long coherence times states in trapped ions experience. Finally, in a step towards truly scalable entanglement generation between quantum dot spins, we design minimally invasive structures that will funnel large proportions of the optical dipole field from the optically dense material that surrounds the quantum dot. The techniques developed in this work and the knowledge gained from their operation should enable the demonstration the creation of high-order nonlocal states between quantum dot spins, single photons and trapped ions, as well as the development of new optically active systems that will benefit from enhanced spin coherence

Non-classical mechanical states guided in a phononic waveguide

The ability to create, manipulate and detect non-classical states of light has been key for many recent achievements in quantum physics and for developing quantum technologies. Achieving the same level of control over phonons, the quanta of vibrations, could have a similar impact, in particular on the fields of quantum sensing and quantum information processing. Here we present a crucial step towards this level of control and realize a single-mode waveguide for individual phonons in a suspended silicon micro-structure. We use a cavity-waveguide architecture, where the cavity is used as a source and detector for the mechanical excitations, while the waveguide has a free standing end in order to reflect the phonons. This enables us to observe multiple round-trips of the phonons between the source and the reflector. The long mechanical lifetime of almost 100 $\mu s$ demonstrates the possibility of nearly lossless transmission of single phonons over, in principle, tens of centimeters. Our experiment demonstrates full on-chip control over traveling single phonons strongly confined in the directions transverse to the propagation axis, potentially enabling a time-encoded multimode quantum memory at telecom wavelength and advanced quantum acoustics experiments

Ultra-low-noise Microwave to Optics Conversion in Gallium Phosphide

Mechanical resonators can act as excellent intermediaries to interface single photons in the microwave and optical domains due to their high quality factors. Nevertheless, the optical pump required to overcome the large energy difference between the frequencies can add significant noise to the transduced signal. Here we exploit the remarkable properties of thin-film gallium phosphide to demonstrate on-chip microwave-to-optical conversion, realised by piezoelectric actuation of a Gigahertz-frequency optomechanical resonator. The large optomechanical coupling and the suppression of two-photon absorption in the material allows us to operate the device at optomechanical cooperativities greatly exceeding one, and, when using a pulsed upconversion pump, induce less than one thermal noise phonon. We include a high-impedance on-chip matching resonator to mediate the mechanical load with the 50-Ohm source. Our results establish gallium phosphide as a versatile platform for ultra-low-noise conversion of photons between microwave and optical frequencies

Microwave-to-optics conversion using a mechanical oscillator in its quantum groundstate

Conversion between signals in the microwave and optical domains is of great interest both for classical telecommunication, as well as for connecting future superconducting quantum computers into a global quantum network. For quantum applications, the conversion has to be both efficient, as well as operate in a regime of minimal added classical noise. While efficient conversion has been demonstrated using mechanical transducers, they have so far all operated with a substantial thermal noise background. Here, we overcome this limitation and demonstrate coherent conversion between GHz microwave signals and the optical telecom band with a thermal background of less than one phonon. We use an integrated, on-chip electro-opto-mechanical device that couples surface acoustic waves driven by a resonant microwave signal to an optomechanical crystal featuring a 2.7 GHz mechanical mode. We initialize the mechanical mode in its quantum groundstate, which allows us to perform the transduction process with minimal added thermal noise, while maintaining an optomechanical cooperativity >1, so that microwave photons mapped into the mechanical resonator are effectively upconverted to the optical domain. We further verify the preservation of the coherence of the microwave signal throughout the transduction process

Dataset for An integrated microwave-to-optics interface for scalable quantum computing

Source data for figures

On-chip distribution of quantum information using traveling phonons

Distributing quantum entanglement on a chip is a crucial step toward realizing scalable quantum processors. Using traveling phonons-quantized guided mechanical wave packets-as a medium to transmit quantum states is now gaining substantial attention due to their small size and low propagation speed compared to other carriers, such as electrons or photons. Moreover, phonons are highly promising candidates to connect heterogeneous quantum systems on a chip, such as microwave and optical photons for long-distance transmission of quantum states via optical fibers. Here, we experimentally demonstrate the feasibility of distributing quantum information using phonons by realizing quantum entanglement between two traveling phonons and creating a time-bin-encoded traveling phononic qubit. The mechanical quantum state is generated in an optomechanical cavity and then launched into a phononic waveguide in which it propagates for around 200 micrometers. We further show how the phononic, together with a photonic qubit, can be used to violate a Bell-type inequality.QN/Groeblacher LabQN/Quantum Nanoscienc

Ultra-low-noise microwave to optics conversion in gallium phosphide

Mechanical resonators can act as excellent intermediaries to interface single photons in the microwave and optical domains due to their high quality factors. Nevertheless, the optical pump required to overcome the large energy difference between the frequencies can add significant noise to the transduced signal. Here we exploit the remarkable properties of thin-film gallium phosphide to demonstrate bi-directional on-chip conversion between microwave and optical frequencies, realized by piezoelectric actuation of a Gigahertz-frequency optomechanical resonator. The large optomechanical coupling and the suppression of two-photon absorption in the material allows us to operate the device at optomechanical cooperativities greatly exceeding one. Alternatively, when using a pulsed upconversion pump, we demonstrate that we induce less than one thermal noise phonon. We include a high-impedance on-chip matching resonator to mediate the mechanical load with the 50-Ω source. Our results establish gallium phosphide as a versatile platform for ultra-low-noise conversion of photons between microwave and optical frequencies.QN/Groeblacher La