155 research outputs found
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New Low Mass Isotopes of Emanation (Element 86)
Among the spallation products obtained from the 350-Mev proton bombardment of Th{sup 232} they have identified two gaseous alpha-emitters which apparently do not decay into any presently known alpha-decay chains. The half-lives observed for the decay of the alpha-activities are 23 minutes and 2.1 hours. These half-lives may be principally determined by an unknown amount of orbital electron capture. At least one alpha-emitting daughter (about 4 hours half-life) has been observed to grow from a gaseous parent, but it has not been determined whether it arises from alpha-decay or electron-capture. Since these gaseous atoms emit alpha-particles it is assumed that they are isotopes of element 86 (emanation or radon) rather than a lighter rare gas. if they were heavy isotopes such as Em{sup 221} or Em{sup 223}, both unknown, they would decay into known alpha-decay series, the neptunium and actinium series, respectively, and so would grow known short lived alpha-emitters which would have been detected. It thus appears reasonable that they must be lighter than the known emanation isotopes
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An Ion Exchange Study of Possible Hydridized 5f Bonding in theActinides
A study has been made of the elution behavior of curium(III), americium(III), plutonium(III), actinium(III), plutonium(IV), neptunium(IV), uraniuM(IV), thorium(IV), neptunium(V), plutonium (VI), uranium (VI), lanthanum(III), cerium(III), europium(III), ytterbium(III), ytterium(III), strontium(II), barium(II), radium(II), cesium(I) with 3.2 M, 6.2 M, 9.3 M, and 12.2 M HCl solutions from Dowex-50 cation exchange resin columns. These elutions show that in high concentrations of hydrochloric acid the actinides form complex ions with chloride ion to a much greater extent than the lanthanides. The strengths of the tripositive actinide complex ions apparently go in the order plutonium > americium> curium, although their ionic radii also decrease in this same order. To explain these results, a partial covalent character may be ascribed to the bonding in the transuranium complex ions. It is shown that a reasonable structure for such covalent bonding involves hybridization of the 5f orbitals in the actinide elements
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Spallation-Fission Competition in Heaviest Elements; HeliumIon-Induced Reactions in Uranium Isotopes
A radiochemical study of fission and spallation products produced by bombardment of U{sup 233}, U{sup 235}, and U{sup 238} with 18-46 Mev helium ions has been made. As in the case of similar studies using isotopes of plutonium as targets, most of the reaction cross section is taken up by fission. Also, the pronounced increase of the total cross section for ({alpha},xn) reactions with increasing mass number of the target that was observed for plutonium targets is observed for uranium targets
Spallation reactions. A successful interplay between modeling and applications
The spallation reactions are a type of nuclear reaction which occur in space
by interaction of the cosmic rays with interstellar bodies. The first
spallation reactions induced with an accelerator took place in 1947 at the
Berkeley cyclotron (University of California) with 200 MeV deuterons and 400
MeV alpha beams. They highlighted the multiple emission of neutrons and charged
particles and the production of a large number of residual nuclei far different
from the target nuclei. The same year R. Serber describes the reaction in two
steps: a first and fast one with high-energy particle emission leading to an
excited remnant nucleus, and a second one, much slower, the de-excitation of
the remnant. In 2010 IAEA organized a worskhop to present the results of the
most widely used spallation codes within a benchmark of spallation models. If
one of the goals was to understand the deficiencies, if any, in each code, one
remarkable outcome points out the overall high-quality level of some models and
so the great improvements achieved since Serber. Particle transport codes can
then rely on such spallation models to treat the reactions between a light
particle and an atomic nucleus with energies spanning from few tens of MeV up
to some GeV. An overview of the spallation reactions modeling is presented in
order to point out the incomparable contribution of models based on basic
physics to numerous applications where such reactions occur. Validations or
benchmarks, which are necessary steps in the improvement process, are also
addressed, as well as the potential future domains of development. Spallation
reactions modeling is a representative case of continuous studies aiming at
understanding a reaction mechanism and which end up in a powerful tool.Comment: 59 pages, 54 figures, Revie
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PIONEERING THE NUCLEAR AGE
This paper reviews the historical aspects of nuclear physics. The scientific aspects of the early transuranium elements are discussed and arms control measures are reviewed. 11 refs., 14 figs. (LSP
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SCIENCE ADVICE TO THE PRESIDENT; DURING AND IMMEDIATELY AFTER WORLD WAR II:
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Journal of Glenn T. Seaborg: 1961-1971 (Appendix: Press Conferences)
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