Precise determination of h/m_Rb using Bloch oscillations and atomic interferometry: a mean to deduce the fine structure constant

We use Bloch oscillations to transfer coherently many photon momenta to atoms. Then we can measure accurately the ratio h/m_Rb and deduce the fine structure constant alpha. The velocity variation due to the Bloch oscillations is measured thanks to Raman transitions. In a first experiment, two Raman $\pi$ pulses are used to select and measure a very narrow velocity class. This method yields to a value of the fine structure constant alpha^{-1}= 137.035 998 84 (91) with a relative uncertainty of about 6.6 ppb. More recently we use an atomic interferometer consisting in two pairs of pi/2 pulses. We present here the first results obtained with this method

Light management in highly-textured perovskite solar cells: From full-device ellipsometry characterization to optical modelling for quantum efficiency optimization

While perovskite solar cells (PSCs) are now reaching high power conversion efficiencies (PCEs), further performance improvement requires a fine management and an optimization of the light pathway and harvesting in the cells. These go through an accurate understanding, characterization and modelling of the optical processes occurring in these complex, often textured, multi-layered systems. In the present work, we have considered a typical methylammonium lead iodide (MAPI) solar cell built on a fluorine-doped tin oxide (FTO) electrode of high roughness (43 nm RMS). By variable-angle spectroscopic ellipsometry (VASE) of the full PSC device, we have been able to determine the optical constants of all the device layers. We have designed a one-dimensional (1D) optical model of the stacked layers where the rough texture is described as layers of effective-medium index. We have supported the model using data extracted from scanning electron microscopy, diffuse spectroscopy and photovoltaic efficiency measurements. We show that the 1D model, while insufficient to describe scattering by the FTO plate alone, gives an accurate description of the full device optical properties. By comparison with the experimental external quantum efficiency (EQE), we estimate the internal quantum efficiency (IQE) and the effect of the losses related to electron transfer. Based on this work, we finally discuss the optical losses mechanisms and the possible strategies that can be implemented to improve light management within PSC devices and further increase their performances.Comment: 14 pages, 5 figure

An achiral magnetic photonic antenna as a tunable nanosource of superchiral light

Sensitivity to molecular chirality is crucial for many fields, from biology and chemistry to the pharmaceutical industry. By generating superchiral light, nanophotonics has brought innovative solutions to reduce the detection volume and increase sensitivity at the cost of a non-selectivity of light chirality or a strong contribution to the background. Here, we theoretically propose an achiral plasmonic resonator, based on a rectangular nanoslit in a thin gold layer behaving as a magnetic dipole, to generate a tunable nanosource of purely superchiral light. This nanosource is free of any background, and the sign of its chirality is externally tunable in wavelength and polarization. These properties result from the coupling between the incident wave and the magnetic dipolar character of our nano-antenna. Thus, our results propose a platform with deep subwavelength detection volumes for chiral molecules in particular, in the visible, and a roadmap for optimizing the signal-to-noise ratios in circular dichroism measurements to reach single-molecule sensitivity

Bloch oscillations of ultracold atoms: a tool for a metrological determination of h/mRbh/m_{Rb}

We use Bloch oscillations in a horizontal moving standing wave to transfer a large number of photon recoils to atoms with a high efficiency (99.5% per cycle). By measuring the photon recoil of $^{87}Rb$, using velocity selective Raman transitions to select a subrecoil velocity class and to measure the final accelerated velocity class, we have determined $h/m_{Rb}$ with a relative precision of 0.4 ppm. To exploit the high momentum transfer efficiency of our method, we are developing a vertical standing wave set-up. This will allow us to measure $h/m_{Rb}$ better than $10^{-8}$ and hence the fine structure constant $\alpha$ with an uncertainty close to the most accurate value coming from the ($g-2$) determination

Combination of Bloch oscillations with a Ramsey-Bord\'e interferometer : new determination of the fine structure constant

We report a new experimental scheme which combines atom interferometry with Bloch oscillations to provide a new measurement of the ratio $h/m_{\mathrm{Rb}}$. By using Bloch oscillations, we impart to the atoms up to 1600 recoil momenta and thus we improve the accuracy on the recoil velocity measurement. The deduced value of $h/m_{\mathrm{Rb}}$ leads to a new determination of the fine structure constant $\alpha^{-1}=137.035 999 45 (62)$ with a relative uncertainty of $4.6\times 10^{-9}$. The comparison of this result with the value deduced from the measurement of the electron anomaly provides the most stringent test of QED

The Lamb shift in muonic hydrogen and the proton radius

By means of pulsed laser spectroscopy applied to muonic hydrogen (μ− p) we have measured the 2S F = 1 1/2 − 2PF = 2 3/2 transition frequency to be 49881.88(76) GHz. By comparing this measurement with its theoretical prediction based on bound-state QED we have determined a proton radius value of rp = 0.84184 (67) fm. This new value is an order of magnitude preciser than previous results but disagrees by 5 standard deviations from the CODATA and the electronproton scattering values. An overview of the present effort attempting to solve the observed discrepancy is given. Using the measured isotope shift of the 1S-2S transition in regular hydrogen and deuterium also the rms charge radius of the deuteron rd = 2.12809 (31) fm has been determined. Moreover we present here the motivations for the measurements of the μ 4He + and μ 3He + 2S-2P splittings. The alpha and triton charge radii are extracted from these measurements with relative accuracies of few 10 − 4. Measurements could help to solve the observed discrepancy, lead to the best test of hydrogen-like energy levels and provide crucial tests for few-nucleon ab-initio theories and potentials