Phonon anharmonicities and ultrafast dynamics in epitaxial Sb2Te3

In this study we report on the investigation of epitaxially grown Sb2Te3 by employing Fourier-Transform transmission Spectroscopy (FTS) with laser-induced Coherent Synchrotron Radiation (CSR) in the Terahertz (THz) spectral range. Static spectra in the range between 20 and 120 cm−1 highlight a peculiar softening of an in-plane IR-active phonon mode upon temperature decrease, as opposed to all Raman active modes which instead show a hardening upon temperature decrease in the same energy range. The phonon mode softening is found to be accompanied by an increase of free carrier concentration. A strong coupling of the two systems (free carriers and phonons) is observed and further evidenced by exciting the same phonon mode at 62 cm−1 within an ultrafast pump-probe scheme employing a femtosecond laser as pump and a CSR single cycle THz pulse as probe. Separation of the free carrier contribution and the phonon resonance in the investigated THz range reveals that, both damping of the phonon mode and relaxation of hot carriers in the time domain happen on the same time scale of 5 ps. This relaxation is about a factor of 10 slower than expected from the Lorentz time-bandwidth limit. The results are discussed in the framework of phonon scattering at thermal and laser induced transient free carriers

Frustration and Melting of Colloidal Molecular Crystals

Using numerical simulations we show that a variety of novel colloidal crystalline states and multi-step melting phenomena occur on square and triangular two-dimensional periodic substrates. At half-integer fillings different kinds of frustration effects can be realized. A two-step melting transition can occur in which individual colloidal molecules initially rotate, destroying the overall orientational order, followed by the onset of interwell colloidal hopping, in good agreement with recent experiments.Comment: 6 pages, 3 postscript figures. Procedings of International Conference on Strongly Coupled Coulomb Systems, Santa Fe, 200

Geometric frustration and magnetization plateaus in quantum spin and Bose-Hubbard models on tubes

We study XXZ Heisenberg models on frustrated triangular lattices wrapped around a cylinder. In addition to having interesting magnetic phases, these models are equivalent to Bose-Hubbard models that describe the physical problem of adsorption of noble gases on the surface of carbon nanotubes. We find analytical results for the possible magnetization plateau values as a function of the wrapping vectors of the cylinder, which in general introduce extra geometric frustration besides the one due to the underlying triangular lattice. We show that for particular wrapping vectors $(N,0)$, which correspond to the zig-zag nanotubes, there is a macroscopically degenerate ground state in the classical Ising limit. The Hilbert space for the degenerate states can be enumerated by a mapping first into a path in a square lattice wrapped around a cylinder (a Bratteli diagram), and then to free fermions interacting with a single ${\bf Z}_N$ degree of freedom. From this model we obtain the spectrum in the anisotropic Heisenberg limit, showing that it is gapless. The continuum limit is a $c=1$ conformal field theory with compactification radius $R=N$ set by the physical tube radius. We show that the compactification radius quantization is exact in the projective $J_\perp/J_z \ll 1$ limit, and that higher order corrections reduce the value of $R$. The particular case of a $(N=2,0)$ tube, which corresponds to a 2-leg ladder with cross links, is studied separately and shown to be gapped because the fermion mapped problem contains superconducting pairing terms.Comment: 10 pages, 11 figure

One-dimensional Kondo lattice at partial band filling

An effective Hamiltonian for the localized spins in the one-dimensional Kondo lattice model is derived via a unitary transformation involving a bosonization of delocalized conduction electrons. The effective Hamiltonian is shown to reproduce all the features of the model as identified in various numerical simulations, and provides much new information on the ferro- to paramagnetic phase transition and the paramagnetic phase.Comment: 11 pages Revtex, 1 Postscript figure. To appear in Phys. Rev. Let

Phonon anharmonicities and ultrafast dynamics in epitaxial Sb2Te3

In this study we report on the investigation of epitaxially grown Sb2Te3 by employing Fourier-Transform transmission Spectroscopy (FTS) with laser-induced Coherent Synchrotron Radiation (CSR) in the Terahertz (THz) spectral range. Static spectra in the range between 20 and 120 cm−1 highlight a peculiar softening of an in-plane IR-active phonon mode upon temperature decrease, as opposed to all Raman active modes which instead show a hardening upon temperature decrease in the same energy range. The phonon mode softening is found to be accompanied by an increase of free carrier concentration. A strong coupling of the two systems (free carriers and phonons) is observed and further evidenced by exciting the same phonon mode at 62 cm−1 within an ultrafast pump-probe scheme employing a femtosecond laser as pump and a CSR single cycle THz pulse as probe. Separation of the free carrier contribution and the phonon resonance in the investigated THz range reveals that, both damping of the phonon mode and relaxation of hot carriers in the time domain happen on the same time scale of 5 ps. This relaxation is about a factor of 10 slower than expected from the Lorentz time-bandwidth limit. The results are discussed in the framework of phonon scattering at thermal and laser induced transient free carriers

Inter-Edge interaction in the Quantum Hall Effect

We consider effects of the interaction between electrons drifting along the opposite sides of a narrow sample under the conditions of the quantum Hall effect. A spatial variation of this interaction leads to backward scattering of collective excitations propagating along the edges. Experiments on propagation of the edge modes in samples with constrictions may give information about the strength of the inter-edge electron interaction in the quantum Hall regime.Comment: 12 Pages, Latex, Accepted for publication in PRL

Persistent currents in mesoscopic rings: A numerical and renormalization group study

The persistent current in a lattice model of a one-dimensional interacting electron system is systematically studied using a complex version of the density matrix renormalization group algorithm and the functional renormalization group method. We mainly focus on the situation where a single impurity is included in the ring penetrated by a magnetic flux. Due to the interplay of the electron-electron interaction and the impurity the persistent current in a system of N lattice sites vanishes faster then 1/N. Only for very large systems and large impurities our results are consistent with the bosonization prediction obtained for an effective field theory. The results from the density matrix renormalization group and the functional renormalization group agree well for interactions as large as the band width, even though as an approximation in the latter method the flow of the two-particle vertex is neglected. This confirms that the functional renormalization group method is a very powerful tool to investigate correlated electron systems. The method will become very useful for the theoretical description of the electronic properties of small conducting ring molecules.Comment: 9 pages, 8 figures include

1/f Noise and Extreme Value Statistics

We study the finite-size scaling of the roughness of signals in systems displaying Gaussian 1/f power spectra. It is found that one of the extreme value distributions (Gumbel distribution) emerges as the scaling function when the boundary conditions are periodic. We provide a realistic example of periodic 1/f noise, and demonstrate by simulations that the Gumbel distribution is a good approximation for the case of nonperiodic boundary conditions as well. Experiments on voltage fluctuations in GaAs films are analyzed and excellent agreement is found with the theory.Comment: 4 pages, 4 postscript figures, RevTe

Sources of Sex Information Used by Young British Women Who Have Sex with Women (WSW) and Women Who Have Sex Exclusively with Men (WSEM): Evidence from the National Survey of Sexual Attitudes and Lifestyles

There is little consideration about the provision of information about sex to women who have sex with women (WSW). This study drew on data from the third National Survey of Sexual Attitudes and Lifestyle, a nationally representative survey of people in Great Britain. Logistic regression was undertaken to examine firstly the relationships between WSW and women who have sex exclusively with men (WSEM) and their main source of information about sex, and secondly between WSW/WSEM and unmet need for information about sex. Each source was included as the binary outcome indicating yes this was the main source, or no this was not the main source of information about sex. The results found that WSW had significantly lower odds of reporting lessons at schools as their main source of information, and significantly higher odds of reporting sources defined as ‘other’ (predominantly first girlfriend/boyfriend or sexual partner) as their main source of information. Reported levels of unmet need for information was also higher amongst young WSW compared with WSEM. This study provides new insights into the sex educational needs of young women and highlights the need for sex education in schools in Great Britain to include information on a full-range of sexual practices, including same-sex sexual relationships

Vibrational spectra of C60C8H8 and C70C8H8 in the rotor-stator and polymer phases

C60-C8H8 and C70-C8H8 are prototypes of rotor-stator cocrystals. We present infrared and Raman spectra of these materials and show how the rotor-stator nature is reflected in their vibrational properties. We measured the vibrational spectra of the polymer phases poly(C60C8H8) and poly(C70C8H8) resulting from a solid state reaction occurring on heating. Based on the spectra we propose a connection pattern for the fullerene in poly(C60C8H8), where the symmetry of the C60 is D2h. On illuminating the C60-C8H8 cocrystal with green or blue light a photochemical reaction was observed leading to a similar product to that of the thermal polymerization.Comment: 26 pages, 8 figures, to appear in Journal of Physical Chemistry B 2nd version: minor changes in wording, accepted version by journa