1,156 research outputs found
Calculating Nonlocal Optical Properties of Structures with Arbitrary Shape
In a recent Letter [Phys. Rev. Lett. 103, 097403 (2009)], we outlined a
computational method to calculate the optical properties of structures with a
spatially nonlocal dielectric function. In this Article, we detail the full
method, and verify it against analytical results for cylindrical nanowires.
Then, as examples of our method, we calculate the optical properties of Au
nanostructures in one, two, and three dimensions. We first calculate the
transmission, reflection, and absorption spectra of thin films. Because of
their simplicity, these systems demonstrate clearly the longitudinal (or
volume) plasmons characteristic of nonlocal effects, which result in anomalous
absorption and plasmon blueshifting. We then study the optical properties of
spherical nanoparticles, which also exhibit such nonlocal effects. Finally, we
compare the maximum and average electric field enhancements around nanowires of
various shapes to local theory predictions. We demonstrate that when nonlocal
effects are included, significant decreases in such properties can occur.Comment: 30 pages, 12 figures, 1 tabl
Microscopic theory of surface-enhanced Raman scattering in noble-metal nanoparticles
We present a microscopic model for surface-enhanced Raman scattering (SERS)
from molecules adsorbed on small noble-metal nanoparticles. In the absence of
direct overlap of molecular orbitals and electronic states in the metal, the
main enhancement source is the strong electric field of the surface plasmon
resonance in a nanoparticle acting on a molecule near the surface. In small
particles, the electromagnetic enhancement is strongly modified by quantum-size
effects. We show that, in nanometer-sized particles, SERS magnitude is
determined by a competition between several quantum-size effects such as the
Landau damping of surface plasmon resonance and reduced screening near the
nanoparticle surface. Using time-dependent local density approximation, we
calculate spatial distribution of local fields near the surface and enhancement
factor for different nanoparticles sizes.Comment: 8 pages, 6 figures. Considerably extended final versio
Detection of the Second r-process Peak Element Tellurium in Metal-Poor Stars
Using near-ultraviolet spectra obtained with the Space Telescope Imaging
Spectrograph onboard the Hubble Space Telescope, we detect neutral tellurium in
three metal-poor stars enriched by products of r-process nucleosynthesis, BD+17
3248, HD 108317, and HD 128279. Tellurium (Te, Z=52) is found at the second
r-process peak (A=130) associated with the N=82 neutron shell closure, and it
has not been detected previously in Galactic halo stars. The derived tellurium
abundances match the scaled solar system r-process distribution within the
uncertainties, confirming the predicted second peak r-process residuals. These
results suggest that tellurium is predominantly produced in the main component
of the r-process, along with the rare earth elements.Comment: Accepted for publication in the Astrophysical Journal Letters (5
pages, 2 figures
New Detections of Arsenic, Selenium, and Other Heavy Elements in Two Metal-Poor Stars
We use the Space Telescope Imaging Spectrograph on board the Hubble Space
Telescope to obtain new high-quality spectra covering the 1900 to 2360 Angstrom
wavelength range for two metal-poor stars, HD 108317 and HD 128279. We derive
abundances of Cu II, Zn II, As I, Se I, Mo II, and Cd II, which have not been
detected previously in either star. Abundances derived for Ge I, Te I, Os II,
and Pt I confirm those derived from lines at longer wavelengths. We also derive
upper limits from the non-detection of W II, Hg II, Pb II, and Bi I. The mean
[As/Fe] ratio derived from these two stars and five others in the literature is
unchanged over the metallicity range -2.8 = +0.28
+/- 0.14 (std. dev. = 0.36 dex). The mean [Se/Fe] ratio derived from these two
stars and six others in the literature is also constant, = +0.16 +/-
0.09 (std. dev. = 0.26 dex). The As and Se abundances are enhanced relative to
a simple extrapolation of the iron-peak abundances to higher masses, suggesting
that this mass region (75 < A < 82) may be the point at which a different
nucleosynthetic mechanism begins to dominate the quasi-equilibrium alpha-rich
freezeout of the iron peak. = +0.56 +/- 0.23 in HD 108317 and HD
128279, and we infer that lines of Cu I may not be formed in local
thermodynamic equilibrium in these stars. The [Zn/Fe], [Mo/Fe], [Cd/Fe], and
[Os/Fe] ratios are also derived from neutral and ionized species, and each
ratio pair agrees within the mutual uncertainties, which range from 0.15 to
0.52 dex.Comment: Accepted for publication in the Astrophysical Journal. 13 pages, 10
figure
rp-Process weak-interaction mediated rates of waiting-point nuclei
Electron capture and positron decay rates are calculated for
neutron-deficient Kr and Sr waiting point nuclei in stellar matter. The
calculation is performed within the framework of pn-QRPA model for rp-process
conditions. Fine tuning of particle-particle, particle-hole interaction
parameters and a proper choice of the deformation parameter resulted in an
accurate reproduction of the measured half-lives. The same model parameters
were used to calculate stellar rates. Inclusion of measured Gamow-Teller
strength distributions finally led to a reliable calculation of weak rates that
reproduced the measured half-lives well under limiting conditions. For the
rp-process conditions, electron capture and positron decay rates on Kr
and Sr are of comparable magnitude whereas electron capture rates on
Sr and Kr are 1--2 orders of magnitude bigger than the
corresponding positron decay rates. The pn-QRPA calculated electron capture
rates on Kr are bigger than previously calculated. The present
calculation strongly suggests that, under rp-process conditions, electron
capture rates form an integral part of weak-interaction mediated rates and
should not be neglected in nuclear reaction network calculations as done
previously.Comment: 13 pages, 4 figures, 4 tables; Astrophysics and Space Science (2012
Surface plasmons at single nanoholes in Au-films
The generation of surface plasmon polaritons (SPP's) at isolated nanoholes in
100 nm thick Au films is studied using near-field scanning optical microscopy
(NSOM). Finite-difference time-domain calculations, some explicitly including a
model of the NSOM tip, are used to interpret the results. We find the holes act
as point-like sources of SPP's and demonstrate that interference between SPP's
and a directly transmitted wave allows for determination of the wavelength,
phase, and decay length of the SPP. The near-field intensity patterns can be
manipulated by varying the angle and polarization of the incident beam.Comment: 12 pages, 3 figure
First demonstration of real-time 100 Gbit/s 3-Level duobinary transmission for optical interconnects
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