10 research outputs found
Creating nuclear spin entanglement using an optical degree of freedom
Funding: Marie Curie Early Stage Training network QIPEST (Grant No. MESTCT-2005-020505), the EPSRC through QIP IRC (Grant Nos. GR/S82176/01 and GR/S15808/01), the National Research Foundation and Ministry of Education, Singapore, the DAAD (German Academic Exchange Service), Linacre College, Oxford, and the Royal Society.Molecular nanostructures are promising building blocks for future quantum technologies, provided methods of harnessing their multiple degrees of freedom can be identified and implemented. Due to low decoherence rates, nuclear spins are considered ideal candidates for storing quantum information, while optical excitations can give rise to fast and controllable interactions for information processing. A recent paper [M. Schaffry et al., Phys. Rev. Lett. 104, 200501 (2010)] proposed a method for entangling two nuclear spins through their mutual coupling to a transient optically excited electron spin. Building on the same idea, we present here an extended and much more detailed theoretical framework, showing that this method is in fact applicable to a much wider class of molecular structures than previously discussed in the original proposal.Publisher PDFPeer reviewe
Spin Amplification for Magnetic Sensors Employing Crystal Defects
Recently there have been several theoretical and experimental studies of the
prospects for magnetic field sensors based on crystal defects, especially
nitrogen vacancy (NV) centres in diamond. Such systems could potentially be
incorporated into an AFM-like apparatus in order to map the magnetic properties
of a surface at the single spin level. In this Letter we propose an augmented
sensor consisting of an NV centre for readout and an `amplifier' spin system
that directly senses the local magnetic field. Our calculations show that this
hybrid structure has the potential to detect magnetic moments with a
sensitivity and spatial resolution far beyond that of a simple NV centre, and
indeed this may be the physical limit for sensors of this class
Quantum metrology with molecular ensembles
This work was supported by the EPSRC through QIP IRC (Grants No. GR/S82176/01 and No. GR/S15808/01), the National Research Foundation and Ministry of Education, Singapore, the DAAD, and the Royal Society.The field of quantum metrology promisesmeasurement devices that are fundamentally superior to conventional technologies. Specifically, when quantum entanglement is harnessed, the precision achieved is supposed to scale more favorably with the resources employed, such as system size and time required. Here, we consider measurement of magnetic-field strength using an ensemble of spin-active molecules. We identify a third essential resource: the change in ensemble polarization (entropy increase) during the metrology experiment. We find that performance depends crucially on the form of decoherence present; for a plausible dephasing model, we describe a quantum strategy, which can indeed beat the standard strategy.Publisher PDFPeer reviewe
Ensemble based quantum metrology
The field of quantum metrology promises measurement devices that are
fundamentally superior to conventional technologies. Specifically, when quantum
entanglement is harnessed the precision achieved is supposed to scale more
favourably with the resources employed, such as system size and the time
required. Here we consider measurement of magnetic field strength using an
ensemble of spins, and we identify a third essential resource: the initial
system polarisation, i.e. the low entropy of the original state. We find that
performance depends crucially on the form of decoherence present; for a
plausible dephasing model, we describe a quantum strategy which can indeed beat
the standard quantum limit
Creating nuclear spin entanglement using an optical degree of freedom
Molecular nanostructures are promising building blocks for future quantum
technologies, provided methods of harnessing their multiple degrees of freedom
can be identified and implemented. Due to low decoherence rates nuclear spins
are considered ideal candidates for storing quantum information while optical
excitations can give rise to fast and controllable interactions for information
processing. A recent paper (Physical Review Letters \textbf{104} 200501)
proposed a method for entangling two nuclear spins through their mutual
coupling to a transient optically excited electron spin. Building on the same
idea, we here present an extended and much more detailed theoretical framework,
showing that this method is in fact applicable to a much wider class of
molecular structures than previously discussed in the original proposal
Creation and manipulation of quantum states in nanostructures
Nanostructures are promising building blocks for quantum technologies due to their reproducible nature and ability to self-assemble into complex structures. However, the need to control these nanostructures represents a key challenge. Hence, this thesis investigates the manipulation and creation of quantum states in certain nanostructures. The results of this thesis can be applied to quantum information processing and to extremely sensitive magnetic-field measurements.In the first research chapter, we propose and examine methods for entangling two (remote) nuclear spins through their mutual coupling to a transient optically excited electron spin. From our calculations we identify the specific molecular properties that permit high entangling power gates for different protocols.In the next research chapter, we investigate another method to create entanglement; this time between two remote electronic spins. This method uses a very sensitive magnetic-field sensor based on a crystal defect that allows the detection of single magnetic moments. The act of sensing the local field constitutes a two-qubit projective measurement. This entangling operation is remarkably robust to imperfections occurring in an experiment.The third research chapter presents an augmented sensor consisting of a nitrogen-vacancy centre for readout and an `amplifier' spin system that directly senses tiny local magnetic fields. Our calculations show that this hybrid structure has the potential to detect magnetic moments with a sensitivity and spatial resolution far beyond that of a sensor based on only a nitrogen-vacancy centre, and indeed this may be the physical limit for sensors of this class.Finally, the last research chapter investigates measurements of magnetic-field strength using an ensemble of spin-active molecules. Here, we describe a quantum strategy that can beat the common standard strategy. We identify the conditions for which this is possible and find that this crucially depends on the decoherence present in the system.</p
Creating nuclear spin entanglement using an optical degree of freedom
Molecular nanostructures are promising building blocks for future quantum technologies, provided methods of harnessing their multiple degrees of freedom can be identified and implemented. Due to low decoherence rates, nuclear spins are considered ideal candidates for storing quantum information, while optical excitations can give rise to fast and controllable interactions for information processing. A recent paper [M. Schaffry et al., Phys. Rev. Lett. 104, 200501 (2010)] proposed a method for entangling two nuclear spins through their mutual coupling to a transient optically excited electron spin. Building on the same idea, we present here an extended and much more detailed theoretical framework, showing that this method is in fact applicable to a much wider class of molecular structures than previously discussed in the original proposal.</p
Creation and manipulation of quantum states in nanostructures
Nanostructures are promising building blocks for quantum technologies due to their reproducible nature and ability to self-assemble into complex structures. However, the need to control these nanostructures represents a key challenge. Hence, this thesis investigates the manipulation and creation of quantum states in certain nanostructures. The results of this thesis can be applied to quantum information processing and to extremely sensitive magnetic-field measurements. In the first research chapter, we propose and examine methods for entangling two (remote) nuclear spins through their mutual coupling to a transient optically excited electron spin. From our calculations we identify the specific molecular properties that permit high entangling power gates for different protocols. In the next research chapter, we investigate another method to create entanglement; this time between two remote electronic spins. This method uses a very sensitive magnetic-field sensor based on a crystal defect that allows the detection of single magnetic moments. The act of sensing the local field constitutes a two-qubit projective measurement. This entangling operation is remarkably robust to imperfections occurring in an experiment. The third research chapter presents an augmented sensor consisting of a nitrogen-vacancy centre for readout and an `amplifier' spin system that directly senses tiny local magnetic fields. Our calculations show that this hybrid structure has the potential to detect magnetic moments with a sensitivity and spatial resolution far beyond that of a sensor based on only a nitrogen-vacancy centre, and indeed this may be the physical limit for sensors of this class. Finally, the last research chapter investigates measurements of magnetic-field strength using an ensemble of spin-active molecules. Here, we describe a quantum strategy that can beat the common standard strategy. We identify the conditions for which this is possible and find that this crucially depends on the decoherence present in the system.EThOS - Electronic Theses Online ServiceGBUnited Kingdo
Quantum metrology with molecular ensembles
The field of quantum metrology promisesmeasurement devices that are fundamentally superior to conventional technologies. Specifically, when quantum entanglement is harnessed, the precision achieved is supposed to scale more favorably with the resources employed, such as system size and time required. Here, we consider measurement of magnetic-field strength using an ensemble of spin-active molecules. We identify a third essential resource: the change in ensemble polarization (entropy increase) during the metrology experiment. We find that performance depends crucially on the form of decoherence present; for a plausible dephasing model, we describe a quantum strategy, which can indeed beat the standard strategy.</p