Optimal Squeezing in Resonance Fluorescence via Atomic-State Purification

Squeezing of atomic resonance fluorescence is shown to be optimized by a properly designed environment, which can be realized by a quasi-resonant cavity. Optimal squeezing is achieved if the atomic coherence is maximized, corresponding to a pure atomic quantum state. The atomic-state purification is achieved by the backaction of the cavity field on the atom, which increases the atomic coherence and decreases the atomic excitation. For realistic cavities, the coupling of the atom to the cavity field yields a purity of the atomic state of more than 99%. The fragility of squeezing against dephasing is substantially reduced in this scenario, which may be important for various applications.Comment: 6 pages including supplemental information, 3 figures. Accepted for PR

Dephasing of Mollow Triplet Sideband Emission of a Resonantly Driven Quantum Dot in a Microcavity

Detailed properties of resonance fluorescence from a single quantum dot in a micropillar cavity are investigated, with particular focus on emission coherence in dependence on optical driving field power and detuning. Power-dependent series over a wide range could trace characteristic Mollow triplet spectra with large Rabi splittings of $|\Omega| \leq 15$ GHz. In particular, the effect of dephasing in terms of systematic spectral broadening $\propto \Omega^2$ of the Mollow sidebands is observed as a strong fingerprint of excitation-induced dephasing. Our results are in excellent agreement with predictions of a recently presented model on phonon-dressed QD Mollow triplet emission in the cavity-QED regime

All-Optical Depletion of Dark Excitons from a Semiconductor Quantum Dot

Semiconductor quantum dots are considered to be the leading venue for fabricating on-demand sources of single photons. However, the generation of long-lived dark excitons imposes significant limits on the efficiency of these sources. We demonstrate a technique that optically pumps the dark exciton population and converts it to a bright exciton population, using intermediate excited biexciton states. We show experimentally that our method considerably reduces the DE population while doubling the triggered bright exciton emission, approaching thereby near-unit fidelity of quantum dot depletion.Comment: 5 pages, 3 figure

Quantum dot micropillar cavities with quality factors exceeding 250,000

We acknowledge funding the BMBF within the projects QuaHL-Rep (16BQ1042) and Q.com-H project and by the State of Bavaria.We report on the spectroscopic investigation of quantum dot micropillar cavities with unprecedented quality factors. We observe a pronounced dependency of the quality factor on the measurement scheme and find that significantly larger quality factors can be extracted in photoreflectance compared to photoluminescence measurements. While the photoluminescence spectra of the microcavity resonances feature a Lorentzian lineshape and Q-factors up to 184,000 (±10,000), the reflectance spectra have a Fano-shaped asymmetry and feature significantly higher Q-factors in excess of 250,000 resulting from a full saturation of the embedded emitters. The very high quality factors in our cavities promote strong light-matter coupling with visibilities exceeding 0.5 for a single QD coupled to the cavity mode.PostprintPeer reviewe

Spontaneously Localized Photonic Modes Due to Disorder in the Dielectric Constant

We present the first experimental evidence for the existence of strongly localized photonic modes due to random two dimensional fluctuations in the dielectric constant. In one direction, the modes are trapped by ordered Bragg reflecting mirrors of a planar, one wavelength long, microcavity. In the cavity plane, they are localized by disorder, which is due to randomness in the position, composition and sizes of quantum dots located in the anti-node of the cavity. We extend the theory of disorder induced strong localization of electron states to optical modes and obtain quantitative agreement with the main experimental observations.Comment: 6 page

Nonlinear photoluminescence spectra from a quantum dot-cavity system: Direct evidence of pump-induced stimulated emission and anharmonic cavity-QED

We investigate the power-dependent photoluminescence spectra from a strongly coupled quantum dot-cavity system using a quantum master equation technique that accounts for incoherent pumping, pure dephasing, and fermion or boson statistics. Analytical spectra at the one-photon correlation level and the numerically exact multi-photon spectra for fermions are presented. We compare to recent experiments on a quantum dot-micropiller cavity system and show that an excellent fit to the data can be obtained by varying only the incoherent pump rates in direct correspondence with the experiments. Our theory and experiments together show a clear and systematic way of studying stimulated-emission induced broadening and anharmonic cavity-QED.Comment: We have reworked our previous arXiv paper and submitted this latest version for peer revie

Intensity fluctuations in bimodal micropillar lasers enhanced by quantum-dot gain competition

We investigate correlations between orthogonally polarized cavity modes of a bimodal micropillar laser with a single layer of self-assembled quantum dots in the active region. While one emission mode of the microlaser demonstrates a characteristic s-shaped input-output curve, the output intensity of the second mode saturates and even decreases with increasing injection current above threshold. Measuring the photon auto-correlation function g^{(2)}(\tau) of the light emission confirms the onset of lasing in the first mode with g^{(2)}(0) approaching unity above threshold. In contrast, strong photon bunching associated with super-thermal values of g^{(2)}(0) is detected for the other mode for currents above threshold. This behavior is attributed to gain competition of the two modes induced by the common gain material, which is confirmed by photon crosscorrelation measurements revealing a clear anti-correlation between emission events of the two modes. The experimental studies are in excellent qualitative agreement with theoretical studies based on a microscopic semiconductor theory, which we extend to the case of two modes interacting with the common gain medium. Moreover, we treat the problem by an extended birth-death model for two interacting modes, which reveals, that the photon probability distribution of each mode has a double peak structure, indicating switching behavior of the modes for the pump rates around threshold.Comment: 11 pages, 5 figures, submitted to Phys. Rev.

Coherence dynamics and quantum-to-classical crossover in an exciton-cavity system in the quantum strong coupling regime

Interaction between light and matter generates optical nonlinearities, which are particularly pronounced in the quantum strong coupling regime. When a single bosonic mode couples to a single fermionic mode, a Jaynes-Cummings (JC) ladder is formed, which we realize here using cavity photons and quantum dot excitons. We measure and model the coherent anharmonic response of this strongly coupled exciton-cavity system at resonance. Injecting two photons into the cavity, we demonstrate a root 2 larger polariton splitting with respect to the vacuum Rabi splitting. This is achieved using coherent nonlinear spectroscopy, specifically four-wave mixing, where the coherence between the ground state and the first (second) rung of the JC ladder can be interrogated for positive (negative) delays. With increasing excitation intensity and thus rising average number of injected photons, we observe spectral signatures of the quantum-to-classical crossover of the strong coupling regime.Peer reviewe