Numerical Study of Photo-Induced Dynamics in Double-Exchange Model

Photo-induced spin and charge dynamics in double-exchange model are numerically studied. The Lanczos method and the density-matrix renormalization-group method are applied to one-dimensional finite-size clusters. By photon irradiation in a charge ordered (CO) insulator associated with antiferromagnetic (AFM) correlation, both the CO and AFM correlations collapse rapidly, and appearances of new peaks inside of an insulating gap are observed in the optical spectra and the one-particle excitation spectra. Time evolutions of the spin correlation and the in-gap state are correlated with each other, and are governed by the transfer integral of conduction electrons. Results are interpreted by the charge kink/anti-kink picture and their effective motions which depend on the localized spin correlation. Pump-photon density dependence of spin and charge dynamics are also studied. Roles of spin degree of freedom are remarkable in a case of weak photon density. Implications of the numerical results for the pump-probe experiments in perovskite manganites are discussed.Comment: 16 pages, 16 figure

Photoinduced magnetic bound state in itinerant correlated electron system with spin-state degree of freedom

Photo-excited state in correlated electron system with spin-state degree of freedom is studied. We start from the two-orbital extended Hubbard model where energy difference between the two orbitals is introduced. Photo-excited metastable state is examined based on the effective model Hamiltonian derived by the two-orbital Hubbard model. Spin-state change is induced by photo-irradiation in the low-spin band insulator near the phase boundary. High-spin state is stabilized by creating a ferromagnetic bound state with photo-doped hole carriers. An optical absorption occurs between the bonding and antibonding orbitals inside of the bound state. Time-evolution for photo-excited states is simulated in the time-dependent mean-field scheme. Pair-annihilations of the photo-doped electron and hole generate the high-spin state in a low-spin band insulator. We propose that this process is directly observed by the time-resolved photoemission experiments.Comment: 15 pages, 16 figure

What is the true charge transfer gap in parent insulating cuprates?

A large body of experimental data point towards a charge transfer instability of parent insulating cuprates to be their unique property. We argue that the true charge transfer gap in these compounds is as small as 0.4-0.5\,eV rather than 1.5-2.0\,eV as usually derived from the optical gap measurements. In fact we deal with a competition of the conventional (3d$^9$) ground state and a charge transfer (CT) state with formation of electron-hole dimers which evolves under doping to an unconventional bosonic system. Our conjecture does provide an unified standpoint on the main experimental findings for parent cuprates including linear and nonlinear optical, Raman, photoemission, photoabsorption, and transport properties anyhow related with the CT excitations. In addition we suggest a scenario for the evolution of the CuO$_2$ planes in the CT unstable cuprates under a nonisovalent doping.Comment: 13 pages, 5 figures, submitted to PR

Orbital Compass Model as an Itinerant Electron System

Two-dimensional orbital compass model is studied as an interacting itinerant electron model. A Hubbard-type tight-binding model, from which the orbital compass model is derived in the strong coupling limit, is identified. This model is analyzed by the random-phase approximation (RPA) and the self-consistent RPA methods from the weak coupling. Anisotropy for the orbital fluctuation in the momentum space is qualitatively changed by the on-site Coulomb interaction. This result is explained by the fact that the dominant fluctuation is changed from the intra-band nesting to the inter-band one by increasing the interaction.Comment: 7 pages, 8 figure

Real-space observation of current-driven domain wall motion in submicron magnetic wires

Spintronic devices, whose operation is based on the motion of a magnetic domain wall (DW), have been proposed recently. If a DW could be driven directly by flowing an electric current instead of a magnetic field, the performance and functions of such device would be drastically improved. Here we report real-space observation of the current-driven DW motion by using a well-defined single DW in a micro-fabricated magnetic wire with submicron width. Magnetic force microscopy (MFM) visualizes that a single DW introduced in the wire is displaced back and forth by positive and negative pulsed-current, respectively. We can control the DW position in the wire by tuning the intensity, the duration and the polarity of the pulsed-current. It is, thus, demonstrated that spintronic device operation by the current-driven DW motion is possible.Comment: Accepted and published in PR

Coherent dynamics of photoinduced nucleation processes

We study the dynamics of initial nucleation processes of photoinduced structural change of molecular crystals. In order to describe the nonadiabatic transition in each molecule, we employ a model of localized electrons coupled with a fully quantized phonon mode, and the time-dependent Schr\"odinger equation for the model is numerically solved. We found a minimal model to describe the nucleation induced by injection of an excited state of a single molecule in which multiple types of intermolecular interactions are required. In this model coherently driven molecular distortion plays an important role in the successive conversion of electronic states which leads to photoinduced cooperative phenomena.Comment: 14 pages, 5 figure

Propagation of a magnetic domain wall in magnetic wires with asymmetric notches

The propagation of a magnetic domain wall (DW) in a submicron magnetic wire consisting of a magnetic/nonmagnetic/magnetic trilayered structure with asymmetric notches was investigated by utilizing the giant magnetoresistance effect. The propagation direction of a DW was controlled by a pulsed local magnetic field, which nucleates the DW at one of the two ends of the wire. It was found that the depinning field of the DW from the notch depends on the propagation direction of the DW.Comment: 12 pages, 3 figure

Electronic structure and electric-field gradients analysis in CeIn3CeIn_3

Electric field gradients (EFG's) were calculated for the $CeIn_3$ compound at both $^{115}In$ and $^{140}Ce$ sites. The calculations were performed within the density functional theory (DFT) using the augmented plane waves plus local orbital (APW+lo) method employing the so-called LDA+U scheme. The $CeIn_3$ compound were treated as nonmagnetic, ferromagnetic, and antiferromagnetic cases. Our result shows that the calculated EFG's are dominated at the $^{140}Ce$ site by the Ce-4f states. An approximately linear relation is intuited between the main component of the EFG's and total density of states (DOS) at Fermi level. The EFG's from our LDA+U calculations are in better agreement with experiment than previous EFG results, where appropriate correlations had not been taken into account among 4f-electrons. Our result indicates that correlations among 4f-electrons play an important role in this compound and must be taken into account