A random walk description of the heterogeneous glassy dynamics of attracting colloids

We study the heterogeneous dynamics of attractive colloidal particles close to the gel transition using confocal microscopy experiments combined with a theoretical statistical analysis. We focus on single particle dynamics and show that the self part of the van Hove distribution function is not the Gaussian expected for a Fickian process, but that it reflects instead the existence, at any given time, of colloids with widely different mobilities. Our confocal microscopy measurements can be described well by a simple analytical model based on a conventional continuous time random walk picture, as already found in several other glassy materials. In particular, the theory successfully accounts for the presence of broad tails in the van Hove distributions that exhibit exponential, rather than Gaussian, decay at large distance.Comment: 13 pages, 5 figs. Submitted to special issue "Classical and Quantum Glasses" of J. Phys.: Condens. Matter; v2: response to refere

Structure and dynamics in glass-formers: predictability at large length scales

Dynamic heterogeneity in glass-formers has been related to their static structure using the concept of dynamic propensity. We re-examine this relationship by analyzing dynamical fluctuations in two atomistic glass-formers and two theoretical models. We introduce quantitative statistical indicators which show that the dynamics of individual particles cannot be predicted on the basis of the propensity, nor by any structural indicator. However, the spatial structure of the propensity field does have predictive power for the spatial correlations associated with dynamic heterogeneity. Our results suggest that the quest for a connection between static and dynamic properties of glass-formers at the particle level is vain, but they demonstrate that such connection does exist on larger length scales.Comment: 7 pages; 4 figs - Extended, clarified versio

Prediction of transits of solar system objects in Kepler/K2 images: An extension of the Virtual Observatory service SkyBoT

All the fields of the extended space mission Kepler/K2 are located within the ecliptic. Many solar system objects thus cross the K2 stellar masks on a regular basis. We aim at providing to the entire community a simple tool to search and identify solar system objects serendipitously observed by Kepler. The SkyBoT service hosted at IMCCE provides a Virtual Observatory (VO) compliant cone-search that lists all solar system objects present within a field of view at a given epoch. To generate such a list in a timely manner, ephemerides are pre-computed, updated weekly, and stored in a relational database to ensure a fast access. The SkyBoT Web service can now be used with Kepler. Solar system objects within a small (few arcminutes) field of view are identified and listed in less than 10 sec. Generating object data for the entire K2 field of view (14{\deg}) takes about a minute. This extension of the SkyBot service opens new possibilities with respect to mining K2 data for solar system science, as well as removing solar system objects from stellar photometric time-series

Revisiting the slow dynamics of a silica melt using Monte Carlo simulations

We implement a standard Monte Carlo algorithm to study the slow, equilibrium dynamics of a silica melt in a wide temperature regime, from 6100 K down to 2750 K. We find that the average dynamical behaviour of the system is in quantitative agreement with results obtained from molecular dynamics simulations, at least in the long-time regime corresponding to the alpha-relaxation. By contrast, the strong thermal vibrations related to the Boson peak present at short times in molecular dynamics are efficiently suppressed by the Monte Carlo algorithm. This allows us to reconsider silica dynamics in the context of mode-coupling theory, because several shortcomings of the theory were previously attributed to thermal vibrations. A mode-coupling theory analysis of our data is qualitatively correct, but quantitative tests of the theory fail, raising doubts about the very existence of an avoided singularity in this system. We discuss the emergence of dynamic heterogeneity and report detailed measurements of a decoupling between translational diffusion and structural relaxation, and of a growing four-point dynamic susceptibility. Dynamic heterogeneity appears to be less pronounced than in more fragile glass-forming models, but not of a qualitatively different nature.Comment: 13 pages, 10 figures; to be published in Phys. Rev.

Criticality in Dynamic Arrest: Correspondence between Glasses and Traffic

Dynamic arrest is a general phenomenon across a wide range of dynamic systems, but the universality of dynamic arrest phenomena remains unclear. We relate the emergence of traffic jams in a simple traffic flow model to the dynamic slow down in kinetically constrained models for glasses. In kinetically constrained models, the formation of glass becomes a true (singular) phase transition in the limit $T\to 0$. Similarly, using the Nagel-Schreckenberg model to simulate traffic flow, we show that the emergence of jammed traffic acquires the signature of a sharp transition in the deterministic limit \pp\to 1, corresponding to overcautious driving. We identify a true dynamical critical point marking the onset of coexistence between free flowing and jammed traffic, and demonstrate its analogy to the kinetically constrained glass models. We find diverging correlations analogous to those at a critical point of thermodynamic phase transitions.Comment: 4 pages, 4 figure

NMR evidence for the persistence of spin-superlattice above the 1/8 magnetization plateau in SrCu2(BO3)2

We present 11B NMR studies of the 2D frustrated dimer spin system SrCu2(BO3)2 in the field range 27-31 T covering the upper phase boundary of the 1/8 magnetization plateau, identified at 28.4 T. Our data provide a clear evidence that above 28.4 T the spin-superlattice of the 1/8 plateau is modified but does not melt even though the magnetization increases. Although this is precisely what is expected for a supersolid phase, the microscopic nature of this new phase is much more complex. We discuss the field-temperature phase diagram on the basis of our NMR data.Comment: 5 pages, 4 figures, published versio

Facilitated spin models: recent and new results

Facilitated or kinetically constrained spin models (KCSM) are a class of interacting particle systems reversible w.r.t. to a simple product measure. Each dynamical variable (spin) is re-sampled from its equilibrium distribution only if the surrounding configuration fulfills a simple local constraint which \emph{does not involve} the chosen variable itself. Such simple models are quite popular in the glass community since they display some of the peculiar features of glassy dynamics, in particular they can undergo a dynamical arrest reminiscent of the liquid/glass transitiom. Due to the fact that the jumps rates of the Markov process can be zero, the whole analysis of the long time behavior becomes quite delicate and, until recently, KCSM have escaped a rigorous analysis with the notable exception of the East model. In these notes we will mainly review several recent mathematical results which, besides being applicable to a wide class of KCSM, have contributed to settle some debated questions arising in numerical simulations made by physicists. We will also provide some interesting new extensions. In particular we will show how to deal with interacting models reversible w.r.t. to a high temperature Gibbs measure and we will provide a detailed analysis of the so called one spin facilitated model on a general connected graph.Comment: 30 pages, 3 figure

Color changes upon cooling of Lepidoptera scales containing photonic nanoarchitectures, and a method for identifying the changes

The effects produced by the condensation of water vapor from the environment in the various intricate nanoarchitectures occurring in the wing scales of several Lepidoptera species were investigated by controlled cooling (from 23° C, room temperature to -5 to -10° C) combined with in situ measurements of changes in the reflectance spectra. It was determined that all photonic nanoarchitectures giving a reflectance maximum in the visible range and having an open nanostructure exhibited alteration of the position of the reflectance maximum associated with the photonic nanoarchitectures. The photonic nanoarchitectures with a closed structure exhibited little to no alteration in color. Similarly, control specimens colored by pigments did not exhibit a color change under the same conditions. Hence, this method can be used to identify species with open photonic nanoarchitectures in their scales. For certain species, an almost complete disappearance of the reflectance maximum was found. All specimens recovered their original colors following warming and drying. Cooling experiments using thin copper wires demonstrated that color alterations could be limited to a width of a millimeter or less. Dried museum specimens did not exhibit color changes when cooled in the absence of a heat sink due to the low heat capacity of the wings

NMR evidence for a strong modulation of the Bose-Einstein Condensate in BaCuSi2_2O6_6

We present a $^{63,65}$Cu and $^{29}$Si NMR study of the quasi-2D coupled spin 1/2 dimer compound BaCuSi$_2$O$_6$ in the magnetic field range 13-26 T and at temperatures as low as 50 mK. NMR data in the gapped phase reveal that below 90 K different intra-dimer exchange couplings and different gaps ($\Delta_{\rm{B}}/\Delta_{\rm{A}}$ = 1.16) exist in every second plane along the c-axis, in addition to a planar incommensurate (IC) modulation. $^{29}$Si spectra in the field induced magnetic ordered phase reveal that close to the quantum critical point at $H_{\rm{c1}}$ = 23.35 T the average boson density $\bar{n}$ of the Bose-Einstein condensate is strongly modulated along the c-axis with a density ratio for every second plane $\bar{n}_{\rm{A}}/\bar{n}_{\rm{B}} \simeq 5$. An IC modulation of the local density is also present in each plane. This adds new constraints for the understanding of the 2D value $\phi$ = 1 of the critical exponent describing the phase boundary